Reconstruction of microstructure parameters of the coarsely dispersed aerosol from spectral measurements of the aerosol optical thickness during a one-year observation period from their regression relations using a finite sample

2017 ◽  
Author(s):  
Victor V. Veretennikov
Keyword(s):  
Optical Thickness ◽  
Aerosol Optical Thickness ◽  
Finite Sample ◽  
Spectral Measurements ◽  
Microstructure Parameters ◽  
Regression Relations ◽  
One Year ◽  
Observation Period

scholarly journals Retrieval of stratospheric and tropospheric BrO columns from multi-axis DOAS measurements at Reunion Island (21° S, 56° E)

2007 ◽  
Vol 7 (3) ◽  
pp. 8261-8308 ◽  
Author(s):  
N. Theys ◽  
M. Van Roozendael ◽  
F. Hendrick ◽  
C. Fayt ◽  
C. Hermans ◽  
...  
Keyword(s):  
Measurement Data ◽  
Retrieval Algorithm ◽  
Reunion Island ◽  
Spectral Measurements ◽  
Réunion Island ◽  
One Year ◽  
Chemical Fields ◽  
Latitudinal Band ◽  
Observation Period ◽  
Good Agreement

Abstract. Spectral measurements of BrO using zenith-sky and off-axis viewing geometries are combined in a linear multiple regression retrieval algorithm to provide stratospheric and tropospheric BrO vertical columns. One year of measurement data are investigated over Reunion-Island (20.9° S, 55.5° E), from July 2004 to July 2005. No seasonal variations of the retrieved BrO columns could be observed, in line with previous studies. A comparison between the stratospheric columns retrieved at 45°, 80°, 85°, 87.5° and 92.5° solar zenith angles and photochemical simulations initialized by chemical fields from the 3-D-CTM SLIMCAT and further constrained by observed NO2 profiles shows a good agreement only by considering a contribution from the very short-lived organic bromine substances to the stratospheric inorganic bromine budget, of 6 to 8 pptv. Furthermore, stratospheric BrO profiles retrieved from late twilight zenith-sky observations are consistent with a total inorganic bromine (Bry) loading of approximately 23 pptv. This represents 6 to 7 pptv more than can be supplied by long-lived organic bromine sources, and therefore supports an added contribution from very short-lived organic bromine substances as recently suggested in several other studies. Moreover strong evidences are presented for the existence of a substantial amount of BrO in the tropical free-troposphere, around 6 km altitude, possibly supplied by the decomposition of short-lived biogenic bromine organic compounds. Tropospheric BrO vertical columns of 1.1±0.45×1013 molec/cm2 are derived for the entire observation period. Comparisons between ground-based BrO vertical columns and total BrO columns derived from SCIAMACHY (onboard the ENVISAT satellite) nadir observations in a latitudinal band centered around 21° S present a good level of consistency, which further strengthens the conclusions of our study.

scholarly journals Retrieval of stratospheric and tropospheric BrO columns from multi-axis DOAS measurements at Reunion Island (21° S, 56° E)

2007 ◽  
Vol 7 (18) ◽  
pp. 4733-4749 ◽  
Author(s):  
N. Theys ◽  
M. Van Roozendael ◽  
F. Hendrick ◽  
C. Fayt ◽  
C. Hermans ◽  
...  
Keyword(s):  
Measurement Data ◽  
Retrieval Algorithm ◽  
Reunion Island ◽  
Spectral Measurements ◽  
Réunion Island ◽  
One Year ◽  
Chemical Fields ◽  
Latitudinal Band ◽  
Observation Period ◽  
Good Agreement

Abstract. Spectral measurements of BrO using zenith-sky and off-axis viewing geometries are combined in a linear multiple regression retrieval algorithm to provide stratospheric and tropospheric BrO vertical columns. One year of measurement data are investigated over Reunion-Island (20.9° S, 55.5° E), from August 2004 to June 2005. A comparison between the stratospheric columns retrieved at 45°, 80°, 85°, 87.5° and 92.5° solar zenith angles and photochemical simulations initialized by chemical fields from the 3-D-CTM SLIMCAT and further constrained by observed NO2 profiles shows a good agreement only by considering a contribution from the very short-lived organic bromine substances to the stratospheric inorganic bromine budget, of 6 to 8 pptv. Furthermore, stratospheric BrO profiles retrieved from late twilight zenith-sky observations are consistent with a total inorganic bromine (Bry) loading of approximately 23 pptv. This represents 6 to 7 pptv more than can be supplied by long-lived organic bromine sources, and therefore supports an added contribution from very short-lived organic bromine substances as recently suggested in several other studies. Moreover strong evidences are presented for the existence of a substantial amount of BrO in the tropical free-troposphere, around 6 km altitude, possibly supplied by the decomposition of short-lived biogenic bromine organic compounds. Tropospheric BrO vertical columns of 1.1±0.45×1013 molec/cm² are derived for the entire observation period. Comparisons between ground-based BrO vertical columns and total BrO columns derived from SCIAMACHY (onboard the ENVISAT satellite) nadir observations in a latitudinal band centered around 21° S present a good level of consistency, which further strengthens the conclusions of our study.

scholarly journals Simultaneous determination of aerosol optical thickness and water leaving radiance from multispectral measurements in coastal waters

2017 ◽  
Author(s):  
Chong Shi ◽  
Teruyuki Nakajima
Keyword(s):  
Simultaneous Determination ◽  
Optical Thickness ◽  
Coastal Waters ◽  
Atmospheric Correction ◽  
Ocean Surface ◽  
Aerosol Optical Thickness ◽  
Surface Model ◽  
Spectral Measurements ◽  
Mean Square Errors

Abstract. Retrieval of aerosol optical properties and water leaving radiance over ocean is changeling since the latter mostly accounts for ~10% of satellite observed signal and can be easily contaminated by the atmospheric scattering. Such an effort would be more difficulty in turbid coastal waters due to the existence of optically complex oceanic substances or high aerosol loading. In an effort to solve such problems, we present an optimization approach for the simultaneous determination of aerosol optical thickness (AOT) and normalized water leaving radiance (nLw) from multi-spectral measurements. In this algorithm, a coupled atmosphere-ocean radiative transfer model combined with a comprehensive bio-optical oceanic module is used to jointly simulate the satellite observed reflectance at the top of atmosphere and water leaving radiance just above the ocean surface. Then a full-physical nonlinear optimization method is adopted to retrieve AOT and nLw in one step. The algorithm is validated using Aerosol Robotic Network Ocean Color (AERONET-OC) products selected from eight OC sites distributed over different waters, consisting of observation cases covered both in and out of sun glint from the Moderate Resolution Imaging Spectroradiometer (MODIS) instrument. Results show a good consistency between retrieved and in situ measurements in each site. It is demonstrated that more accurate AOT are determined based on the simultaneous retrieval method, particularly in shorter wavelengths and sun glint conditions, where the averaged percentage difference (APD) of retrieved AOT generally reduce by approximate 10 % in visible bands compared with those derived from the standard atmospheric correction (AC) scheme. It is caused that all the spectral measurements can be used jointly to increase the information content in the inversion of AOT and the wind speed is also simultaneously retrieved to compensate the specular reflectance error estimated from the rough ocean surface model. For the retrieval of nLw, over atmospheric correction can be avoided to have a significant improvement for the inversion of nLw at 412 nm. Furthermore, generally better estimates of band ratios of nLw(443)/nLw(554) and nLw(488)/nLw(554), which are employed in the inversion of chlorophyll a concentration (Chl), are obtained using simultaneous retrieval approach with less root mean square errors and relative differences than those derived from the standard AC approach in comparison to the AERONET-OC products, as a result that the APD value of retrieved Chl decreases by about 5 %. On the other hand, the standard AC scheme yields a more accurate retrieval of nLw at 488 nm, prompting a further optimization of oceanic bio-optical module of current model.

scholarly journals Temporal consistency of lidar observations during aerosol transport events in the framework of the ChArMEx/ADRIMED campaign at Minorca in June 2013

2016 ◽  
Vol 16 (5) ◽  
pp. 2863-2875 ◽  
Author(s):  
Patrick Chazette ◽  
Julien Totems ◽  
Gérard Ancellet ◽  
Jacques Pelon ◽  
Michaël Sicard
Keyword(s):  
Remote Sensing ◽  
Biomass Burning ◽  
Optical Thickness ◽  
Forest Fires ◽  
Atmospheric Transport ◽  
Extinction Ratio ◽  
Aerosol Optical Thickness ◽  
Dust Particles ◽  
Temporal Consistency ◽  
Observation Period

Abstract. We performed synergetic daytime and nighttime active and passive remote-sensing observations at Minorca (Balearic Islands, Spain), over more than 3 weeks during the Chemistry-Aerosol Mediterranean Experiment/Aerosol Direct Radiative Effect in the Mediterranean (ChArMEx/ADRIMED) special observation period (SOP 1a, June–July 2013). We characterized the aerosol optical properties and type in the low and middle troposphere using an automated procedure combining Rayleigh–Mie–Raman lidar (355, 387 and 407 nm) with depolarization (355 nm) and AERONET Cimel® sun-photometer data. Results show a high variability due to varying dynamical forcing. The mean column-averaged lidar backscatter-to-extinction ratio (BER) was close to 0.024 sr−1 (lidar ratio of  ∼ 41.7 sr), with a large dispersion of ±33 % over the whole observation period due to changing atmospheric transport regimes and aerosol sources. The ground-based remote-sensing measurements, coupled with satellite observations, allowed the documentation of (i) dust particles up to 5 km (above sea level) in altitude originating from Morocco and Algeria from 15 to 18 June with a peak in aerosol optical thickness (AOT) of 0.25 ± 0.05 at 355 nm, (ii) a long-range transport of biomass burning aerosol (AOT  =  0.18 ± 0.16) related to North American forest fires detected from 26 to 28 June 2013 by the lidar between 2 and 7 km and (iii) mixture of local sources including marine aerosol particles and pollution from Spain. During the biomass burning event, the high value of the particle depolarization ratio (8–14 %) may imply the presence of dust-like particles mixed with the biomass burning aerosols in the mid-troposphere. For the field campaign period, we also show linearity with SEVIRI retrievals of the aerosol optical thickness despite 35 % relative bias, which is discussed as a function of aerosol type.

scholarly journals Temporal consistency of lidar observables during aerosol transport events in the framework of the ChArMEx/ADRIMED campaign at Menorca Island in June 2013

2015 ◽  
Vol 15 (22) ◽  
pp. 32723-32757 ◽  
Author(s):  
P. Chazette ◽  
J. Totems ◽  
G. Ancellet ◽  
J. Pelon ◽  
M. Sicard
Keyword(s):  
Remote Sensing ◽  
Biomass Burning ◽  
Optical Thickness ◽  
Forest Fires ◽  
Extinction Ratio ◽  
Aerosol Optical Thickness ◽  
Dust Particles ◽  
Temporal Consistency ◽  
Night Time ◽  
Observation Period

Abstract. We performed synergetic daytime and night-time active and passive remote sensing observations at Menorca (Balearic Island, Spain), over more than 3 weeks during the Chemistry–Aerosol Mediterranean Experiment/Aerosol Direct Radiative Effect in the Mediterranean (ChArMEx/ADRIMED) special observation period (SOP 1a, June–July 2013). We characterized the aerosol optical properties and type in the low and middle troposphere using an automated procedure combining Rayleigh–Mie–Raman lidar (355, 387 and 407 nm) with depolarization (355 nm) and AERONET Cimel® sun-photometer data. Results show a high variability due to varying dynamical forcing. The mean column-averaged lidar backscatter-to-extinction ratio (BER) was close to 0.024 sr-1 (lidar ratio of ∼ 41.7 sr), with a large dispersion of ±33 % over the whole observation period due to changing atmospheric transport regimes and aerosol sources. The ground-based remote sensing measurements, coupled with satellite observations, allowed to document (i) dust particles up to 5 km a.s.l. in altitude originating from Morocco and Algeria from 15 to 18 June with a peak in aerosol optical thickness (AOT) of 0.25 ± 0.05 at 355 nm, (ii) a long-range transport of biomass burning aerosol (AOT = 0.18 ± 0.16) related to North American forest fires detected from 26 to 28 June 2013 by the lidar between 2 and 7 km and (iii) mixture of local sources including marine aerosol particles and pollution from Spain. During the biomass burning event, the high value of the particle depolarization ratio (8–14 %) may imply the presence of dust-like particles mixed with the biomass burning aerosols in the mid troposphere. We show also linearity with SEVIRI retrievals of the aerosol optical thickness within 35 % relative bias, which is discussed as a function of aerosol type.

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