Polarization dependent second harmonic generations of equilateral triangular Au nanorods at localized surface plasmon resonances

2017 ◽  
Author(s):  
Atsushi Sugita ◽  
Hirofumi Yogo ◽  
Atsushi Ono ◽  
Yoshimasa Kawata
Keyword(s):  
Surface Plasmon ◽  
Second Harmonic ◽  
Localized Surface Plasmon ◽  
Surface Plasmon Resonances ◽  
Au Nanorods ◽  
Localized Surface Plasmon Resonances ◽  
Plasmon Resonances

scholarly journals Space- and time-resolved second harmonic spectroscopy of coupled plasmonic nanocavities

Nanophotonics ◽  
2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Adi Salomon ◽  
Heiko Kollmann ◽  
Manfred Mascheck ◽  
Slawa Schmidt ◽  
Yehiam Prior ◽  
...  
Keyword(s):  
Optical Properties ◽  
Surface Plasmon ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Hot Spot ◽  
Localized Surface Plasmon ◽  
Surface Plasmon Resonances ◽  
Localized Surface Plasmon Resonances ◽  
Plasmon Resonances ◽  
Linear And Nonlinear

Abstract Localized surface plasmon resonances of individual sub-wavelength cavities milled in metallic films can couple to each other to form a collective behavior. This coupling leads to a delocalization of the plasmon field at the film surface and drastically alters both the linear and nonlinear optical properties of the sample. In periodic arrays of nanocavities, the coupling results in the formation of propagating surface plasmon polaritons (SPP), eigenmodes extending across the array. When artificially introducing dislocations, defects and imperfections, multiple scattering of these SPP modes can lead to hot-spot formation, intense and spatially confined fluctuations of the local plasmonic field within the array. Here, we study the underlying coupling effects by probing plasmonic modes in well-defined individual triangular dimer cavities and in arrays of triangular cavities with and without artificial defects. Nonlinear confocal spectro-microscopy is employed to map the second harmonic (SH) radiation from these systems. Pronounced spatial localization of the SPP field and significant enhancements of the SH intensity in certain, randomly distributed hot spots by more than an order of magnitude are observed from the triangular arrays as compared to a bare silver film by introducing a finite degree of disorder into the array structure. Hot-spot formation and the resulting enhancement of the nonlinear efficiency are correlated with an increase in the lifetime of the localized SPP modes. By using interferometric SH autocorrelation measurements, we reveal lifetimes of hot-spot resonances in disordered arrays that are much longer than the few-femtosecond lifetimes of the localized surface plasmon resonances of individual nanocavity dimers. This suggests that hot spot lifetime engineering provides a path for manipulating the linear and nonlinear optical properties of nanosystems by jointly exploiting coherent couplings and tailored disorder.

scholarly journals Probing the symmetry of the potential of localized surface plasmon resonances with phase-shaped electron beams

2017 ◽  
Vol 8 (1) ◽  
Author(s):  
Giulio Guzzinati ◽  
Armand Béché ◽  
Hugo Lourenço-Martins ◽  
Jérôme Martin ◽  
Mathieu Kociak ◽  
...  
Keyword(s):  
Surface Plasmon ◽  
Electron Beams ◽  
Localized Surface Plasmon ◽  
Surface Plasmon Resonances ◽  
Localized Surface Plasmon Resonances ◽  
Plasmon Resonances

Tunable localized surface plasmon resonances of asymmetric Au/SiO2/Au cross-shape nanobars

2014 ◽  
Vol 28 (17) ◽  
pp. 1450143 ◽  
Author(s):  
M. L. Wan ◽  
H. J. Du ◽  
Y. L. Song ◽  
F. Q. Zhou ◽  
K. J. Dai
Keyword(s):  
Electric Fields ◽  
Surface Plasmon ◽  
Near Infrared ◽  
Dipole Approximation ◽  
Localized Surface Plasmon ◽  
Surface Plasmon Resonances ◽  
Localized Surface Plasmon Resonances ◽  
Plasmon Resonances ◽  
Surface Enhanced Raman ◽  
Infrared Spectral

The plasmonic properties of asymmetric Au / SiO 2/ Au sandwiched cross-shape nanobars are investigated theoretically using the discrete dipole approximation (DDA) method. Two localized surface plasmon resonances are observed in the extinction spectra, which perform extreme sensitivity to the length and width of the nanobar and can be tuned easily throughout visible and into near-infrared spectral regions. The local electric fields around the nanobar are calculated and a pure electromagnetic Raman enhancement factor of about 106 can be achieved. In addition, compared to a monolayer gold nanobar, it exhibits more "hot spots" and stronger localized electric field enhancements. This plasmonic substrate provides potential applications in surface enhanced Raman scattering (SERS) and nonlinear optical devices.

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