Interface engineering in inorganic hybrid structures towards improved photocatalysis (Conference Presentation)

Author(s):  
Yujie Xiong
2018 ◽  
Vol MA2018-01 (31) ◽  
pp. 1833-1833
Author(s):  
Yujie Xiong

Considering the excessive emission of atmospheric carbon dioxide (CO2) caused by the combustion of fossil fuels, the sunlight-driven CO2 reduction into higher energy chemicals, such as carbon monoxide, formic acid, methanol or methane, offers a more promising approach to alleviate both global warming and energy crisis. Designing new photocatalytic materials for improving the photoconversion efficiency is a promising route to achieve this goal. Despite the invention of a large number of catalytic materials with well-defined structures, their overall efficiency in photocatalysis is still quite limited as the three key steps - light harvesting, charge generation and separation, and charge transfer to surface for redox reactions - have not been substantially improved. To improve each step in the complex process, there is a major trend to develop materials based on inorganic hybrid structures, in which surface and interface engineering holds the promise for boosting the overall efficiency. In this talk, I will demonstrate several different approaches to designing inorganic hybrid structures with improved photocatalytic performance via surface and interface engineering. It is anticipated that this series of works open a new window to rationally designing inorganic hybrid materials for photo-induced applications.


2013 ◽  
Vol 103 (15) ◽  
pp. 151116 ◽  
Author(s):  
Hyung Keun Yoo ◽  
Sun-Goo Lee ◽  
Chul Kang ◽  
Chul-Sik Kee ◽  
Joong Wook Lee

2014 ◽  
Vol 54 (2S) ◽  
pp. 02BC03
Author(s):  
Feifei Wu ◽  
Lian Hu ◽  
Bingpo Zhang ◽  
Ruifeng Li ◽  
Huizhen Wu

2015 ◽  
Vol 51 (51) ◽  
pp. 10261-10271 ◽  
Author(s):  
Song Bai ◽  
Yujie Xiong

This feature article outlines recent progress in the surface and interface design of inorganic hybrid structures, which offers the possibilities to tune their catalytic performance, with a focus on the fundamentals behind each synthesis and catalytic application.


2011 ◽  
Vol 391-392 ◽  
pp. 409-417 ◽  
Author(s):  
Yu Ping Liu ◽  
Lei Huang ◽  
Wang Zhou Shi

Cover scales and ground scales are found to be responsible for the greenish blue color of Morpho menelaus. From simulation predictions, different colors can be engineered by controlled thickness coatings on surface of scales. By replicating the morphologies of scales with low-temperature atomic layer deposition (ALD) methods, tunable colors are achieved successful by regulations of deposition cycles of Al2O3in the organic-inorganic hybrid structures. After removal of original structures by means of high temperatures, inverted nanostructures exhibiting colors sealed by Al2O3shell are fabricated. Simulation results of the hybrid and inverted structures are in accordance with experimental results well. The predictable spectra and the executable precisely controlled deposition by ALD provide us the potential of designing and constructing diversified structural colors.


2019 ◽  
Vol 7 (40) ◽  
pp. 23105-23120 ◽  
Author(s):  
Eluri Pavitra ◽  
Ganji Seeta Rama Raju ◽  
Seyed Majid Ghoreishian ◽  
L. Krishna Bharat ◽  
Sreekantha Reddy Dugasani ◽  
...  

Protein–inorganic hybrid CaMoO4:Eu3+ microstructures were unveiled as an efficient photocatalyst for water purification.


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