Application of Master Curve Approach to Surveillance Test Data for WWER-1000 Reactor Pressure Vessels

Author(s):  
Volodymyr M. Revka ◽  
Liudmyla I. Chyrko

An important issue in the safety operation of WWER-1000 type reactor is a decrease in fracture toughness for reactor pressure vessel steels due to neutron irradiation. This effect for RPV metal is known as radiation embrittlement. The radiation induced temperature shift of the fracture toughness transition curve is considered as a measure of the embrittlement rate. The Charpy impact and fracture toughness specimens are included in the surveillance program for an assessment of changes in fracture toughness of RPV materials. The present analysis is based on a large data set which includes mostly experimental results for pre-cracked Charpy specimens from a WWER-1000 RPV surveillance program. A Master curve approach is applied to analyze the surveillance test data with respect to a shape of the fracture toughness transition curve and a scatter of KJC values. The RPV base and weld metal in unirradiated, thermally aged and irradiated conditions are considered in this study. The maximum shift in a reference temperature T0 due to irradiation is 107 degree Celsius. It is shown that the Master curve, 5 % and 95 % tolerance bounds describe adequately the temperature dependence and the statistical scatter of KJC values for WWER-1000 RPV steels both in unirradiated condition and after irradiation up to design as well as long term operation neutron fluence. Furthermore, a development of the Weibull plots for considered data sets is shown that the Weibull slope is close to the expected one of 4 on average. Finally, a comparison of the reference temperature T0 and a scatter of KJC values derived from the pre-cracked Charpy and 0,5T C(T) specimens of base and weld metal in unirradiated condition is done. The analysis has shown a significant discrepancy between the T0 values derived from the two different types of specimens for both RPV metals.

Author(s):  
Meifang Yu ◽  
Zhen Luo ◽  
Y. J. Chao

Both Charpy V-notch (CVN) impact energy and fracture toughness are parameters reflecting toughness of the material. Charpy tests are however easy to perform compared to standard fracture toughness tests, especially when the material is irradiated and quantity is limited. Correlations between the two parameters are therefore of great significance, especially for reactor pressure vessel (RPV) structural integrity assessment. In this paper, correlations between CVN impact energy and fracture toughness of three commonly used RPV steels, namely Chinese A508-3 steel, USA A533B steel, Euro 20MnMoNi55 steel, are investigated with two methods. One method applies a direct conversion using empirical formulas and the other adopts the Master Curve method. It is found that when the empirical formula is used, the difference between the predicted fracture toughness (from the CVN impact energy) and actual test data is relatively small in upper shelf, lower shelf and the bottom of transition region, while relatively large in other parts of the transition region. When the Master Curve method is adopted, whether the reference temperature T0 is estimated through temperature at 28J or 41J CVN impact energy, the predicted fracture toughness values of the three steels are consistent with actual test data. The reference temperature T0 is also estimated through the IGC-parameter correlation and through a combination of empirical formula and multi-temperature method. Both procedures show excellent agreement with test results. The mean value of T0 estimated from T28J, T41J, IGC-parameters and the combination method is denoted by TQ-ave and is then used as the final reference temperature T0 for the Master Curve determination. Accuracy of TQ-ave (and therefore the Master Curve method) is demonstrated by comparison with actual test data of the three RPV steels. It is concluded that Master Curve method provides a reliable procedure for predicting fracture toughness in the transition region utilizing limited CVN impact energy data from open literature.


Author(s):  
Udo Rindelhardt ◽  
Hans-Werner Viehrig ◽  
Joerg Konheiser ◽  
Jan Schuhknecht

Between 1973 and 1990 four units of the Russian nuclear power plants type WWER-440/230 were operated in Greifswald (former East Germany). Material probes from the pressure vessels were gained in the frame of the ongoing decommissioning procedure. The investigations of this material started with material from the circumferential core weld of unit 1. First, this paper presents results of the reactor pressure vessel (RPV) fluence calculations depending on different loading schemes and on the axial weld position based on the Monte Carlo code TRAMO. The results show that the use of the dummy assemblies reduces the flux by a factor of 2–5 depending on the azimuthal position. The circumferential core weld (SN0.1.4) received a fluence of 2.4×1019 neutrons/cm2 at the inner surface; it decreases to 0.8×1019 neutrons/cm2 at the outer surface. The material investigations were done using a trepan from the circumferential core weld. The reference temperature T0 was calculated with the measured fracture toughness values, KJc, at brittle failure of the specimen. The KJc values show a remarkable scatter. The highest T0 was about 50°C at a distance of 22 mm from the inner surface of the weld. The Charpy transition temperature TT41J estimated with results of subsized specimens after the recovery annealing was confirmed by the testing of standard Charpy V-notch specimens. The VERLIFE procedure prepared for the integrity assessment of WWER RPV was applied on the measured results. The VERLIFE lower bound curve indexed with the Structural Integrity Assessment Procedures for European Industry (SINTAP) reference temperature, RTT0SINTAP, envelops the KJc values. Therefore for a conservative integrity assessment the fracture toughness curve indexed with a RT representing the brittle fraction of a data set of measured KJc values has to be applied.


Author(s):  
Udo Rindelhardt ◽  
Hans-Werner Viehrig ◽  
Joerg Konheiser ◽  
Jan Schuhknecht

Between 1973 and 1990 4 units of the Russian NPP type WWER-440/230 were operated in Greifswald (former GDR). The operation was stopped after the German reunification, because the units did not completely follow western nuclear safety standards. Material probes from the pressure vessels were gained in the frame of the ongoing decommissioning procedure. The investigations of this material started with material from the circumferential core weld of unit 1. This weld was annealed after 13 cycles and operated further for 2 cycles. Additionally, starting with cycle 11, dummy assemblies were inserted to reduce the neutron fluence in the RPV wall. Firstly this paper presents results of the RPV fluence calculations depending on different loading schemes and on the axial weld position based on the Monte Carlo code TRAMO. The results show, that the use of the dummy assemblies reduces the flux by a factor of 2 – 5 depending on the azimuthal position. The fluence increase is reduced to 1/6 at the position of the maximum fluence. The neutron fluence at the different circumferential welds is closely related to their distance to the core. The circumferential core weld (SN0.1.4) received a fluence of 2.4·1019 neutrons/cm2 at the inner surface, it decreases to 0.8·1019 neutrons/cm2 at the outer surface. The neutron fluences at the both other welds are 2 resp. 4 orders of magnitude smaller according to their distances to the core. It should be mentioned that in this cases the fluence gradient can be negative through the wall. The material investigations were done using a trepan from the circumferential core weld. Master Curve and Charpy V-notch testing were applied. Specimens from 7 locations through the thickness of the welding seam were tested. The reference temperature T0 was calculated with the measured fracture toughness values, KJc, at brittle failure of the specimen. Generally the KJc values measured on pre-cracked and side-grooved Charpy size SE(B) specimens of the investigated weld metal follows the course of the Master Curve. The KJc values show a remarkable scatter. In addition the MC SINTAP procedure was applied to determine T0SINTAP of the brittle fraction of the data set. There are remarkable differences between T0 and T0SINTAP indicating macroscopic inhomogeneous weld metal. The highest T0 was about 50°C at a distance of 22 mm from the inner surface of the weld. It is 40 K higher compared with T0 at the inner surface. This is important for the assessment of ductile-to-brittle temperatures measured with sub size Charpy specimens made of weld metal from the inner RPV wall. This material does not represent the most conservative condition. Nevertheless, the Charpy transition temperature TT41J estimated with results of sub size specimens after the recovery annealing was confirmed by the testing of standard Charpy V-notch specimens. The VERLIFE procedure prepared for the integrity assessment of WWER RPV was applied on the measured results. It enables the determination of a reference temperature, RTT0 to index a lower bound fracture toughness curve. This curve agrees with the MC 5% fractile as specified in ASTM E1921-05. The measured KJc values are not enveloped by this lower bound curve. However, the VERLIFE lower bound curve indexed with the SINTAP reference temperature RTT0SINTAP envelops the KJc values. Therefore for a conservative integrity assessment the fracture toughness curve indexed with a RT representing the brittle fraction of a dataset of measured KJc values has to be applied.


Author(s):  
Volodymyr M. Revka ◽  
Liudmyla I. Chyrko

In this study the analysis of fracture toughness test data has been performed in terms of estimation of the proper T0 value for several WWER-1000 RPV materials in unirradiated condition. The surveillance test data for the standard and reconstituted specimens were included in the analysis. It was found that a reference temperature T0 for reconstituted specimens is 31°C higher on average in comparison to the standard specimens. The possible reason is a high level of the stress intensity factor Kmax during the cycle at the stage of completion of crack tip sharpening for standard specimens. Furthermore, the Charpy impact and fracture toughness test data for standard and reconstituted specimens have been compared considering the known relationship between the reference temperature T0 and the transition temperature T28J which corresponds to the Charpy energy level of 28 J. Another objective of this study was to compare the RPV metal embrittlement rate for the two reactor pressure vessels using surveillance test data from standard and reconstituted fracture toughness specimens. The analysis has shown that test data for the reconstituted specimens is consistent with the test data for the standard specimens with regard to the embrittlement rate.


Author(s):  
Randy K. Nanstad ◽  
Marc Scibetta

There is strong interest from the nuclear industry to use the precracked Charpy single-edge notched bend, SE(B), specimen (PCVN) to enable determination of the reference temperature, T0, with reactor pressure vessel surveillance specimens. Unfortunately, for many different ferritic steels, tests with the PCVN specimen (10×10×55 mm) have resulted in T0 temperatures up to 25°C lower than T0 values obtained using data from 25-mm thick compact specimens [1TC(T)]. This difference in T0 reference temperature has often been designated a specimen bias effect, and the primary focus for explaining this effect is loss of constraint in the PCVN specimen. The International Atomic Energy Agency has developed a three-part coordinated research project (CRP) to evaluate various issues associated with the fracture toughness Master Curve for application to light-water reactor pressure vessels. One part of the CRP is focused on the issue of test specimen geometry effects, with emphasis on the PCVN bias. Participating organizations for this part of the CRP are performing fracture toughness testing of various steels, including the reference steel JRQ (A533-B-1) often used for IAEA studies, with various types of specimens under various conditions. Additionally, many of the participants are taking part in a round robin exercise on finite element modeling of the PCVN specimen. Some preliminary results from fracture toughness tests are compared with regard to effects of specimen size and type on the reference temperature T0. In agreement with a number of published results, the results do generally show lower values of T0 from the PCVN specimen compared with the compact and larger bend specimens. They also clearly show higher apparent fracture toughness for the shallow crack compared with the deep crack configuration. Moreover, the SE(B) specimens exhibit a tendency for decreasing T0 with decreasing specimen size (thickness and/or remaining ligament). Additionally, as shown in previous CRPs, the results also exhibit a dependence on test temperature. Following completion of all testing, the results will be evaluated relative to existing proposed models with a view towards developing an understanding of the reasons for the observed differences.


Author(s):  
Milan Brumovsky ◽  
Milos Kytka ◽  
Petr Novosad ◽  
Jiri Brynda

Lifetime of reactor pressure vessels practically depends on a level of degradation of RPV material properties during operation. The most important degradating mechanism of RPV materials is usually radiation damage, characterized by values on neutron fluence on one side and radiation embrittlement of RPV materials on the second side. WWER reactor pressure vessels in the Czech Republic are a subject of a very thorough and complex monitoring program, that includes: • Standard material surveillance program containing of WWER-440 RPV materials — base metal, weld metal, heat affected zone, but irradiated with high lead factor (13 to 18), • Supplementary surveillance program of WWER-440 RPV materials, including additionally austenitic cladding materials, IAEA reference material JRQ irradiated with low lead factor (2 to 3) with parts subjected to annealing and re-irradiation after annealing, • Modified surveillance program of WWER-1000 RPV materials — base metal, weld metal, heat affected zone, cladding materials, IAEA reference JRQ material irradiated in low lead factor (2 to 3) near RPV inner beltline region, • Integrated surveillance specimen program for WWER-1000 reactor including materials from NPP Temelin (Czech Republic), Belene (Bulgaria), Kalinin (Russia) and Ukranian NPPs, • Continous exvessel monitoring of neutron fluence on outer RPV surface for both WWER-440 and WWER-1000 plants, • Neutron fluence determination on inner RPV surface (austenitic cladding) using special technique for removal of specimens from cladding for Nb activity measurements, • Ex-vessel temperature measurements during RPV operation. All these programs serve for precision of operation conditions and determination of degradation of RPV materials for RPV integrity and lifetime assessment.


Author(s):  
Jan Schuhknecht ◽  
Hans-Werner Viehrig ◽  
Udo Rindelhardt

The investigation of reactor pressure vessel (RPV) materials from decommissioned NPPs offers the unique opportunity to scrutinize the irradiation behaviour under real conditions. Material samples taken from the RPV wall enable a comprehensive material characterisation. The paper describes the investigation of trepans taken from the decommissioned WWER-440 first generation RPVs of the Greifswald NPP. Those RPVs represent different material conditions such as irradiated (I), irradiated and recovery annealed (IA) and irradiated, recovery annealed and re-irradiated (IAI). The working program is focussed on the characterisation of the RPV steels (base and weld metal) through the RPV wall. The key part of the testing is aimed at the determination of the reference temperature T0 following the ASTM Test Standard E1921-05 to determine the fracture toughness of the RPV steel in different thickness locations. In a first step the trepans taken from the RPV Greifswald Unit 1 containing the X-butt multilayer submerged welding seam and from base metal ring 0.3.1 both located in the beltline region were investigated. Unit 1 represents the IAI condition. It is shown that the Master Curve approach as adopted in ASTM E1921 is applicable to the investigated original WWER-440 weld metal. The evaluated T0 varies through the thickness of the welding seam. The lowest T0 value was measured in the root region of the welding seam representing a uniform fine grain ferritic structure. Beyond the welding root T0 shows a wavelike behaviour. The highest T0 of the weld seam was not measured at the inner wall surface. This is important for the assessment of ductile-to-brittle temperatures measured on sub size Charpy specimens made of weld metal compact samples removed from the inner RPV wall. Our findings imply that these samples do not represent the most conservative condition. Nevertheless, the Charpy transition temperature TT41J estimated with results of sub size specimens after the recovery annealing was confirmed by the testing of standard Charpy V-notch specimens. The evaluated Charpy-V TT41J shows a better accordance with the irradiation fluence along the wall thickness than the Master Curve reference temperature T0. The evaluated T0 from the trepan of base metal ring 0.3.1 varies through the thickness of the RPV wall. T0 increases from −120°C at the inner surface to −104°C at a distance of 33 mm from it and again to −115°C at the outer RPV wall. The KJc values generally follow the course of the MC, although the scatter is large. The re-embrittlement during 2 campaigns operation can be assumed to be low for the weld and base metal.


Author(s):  
Naoki Miura ◽  
Naoki Soneda

The fracture toughness Master Curve gives a universal relationship between the median of fracture toughness and temperature in the ductile-brittle transition temperature region of ferritic steels such as reactor pressure vessel (RPV) steels. The Master Curve approach specified in the ASTM standard theoretically provides the confidence levels of fracture toughness in consideration of the inherent scatter of fracture toughness. The authors have conducted a series of fracture toughness tests for typical Japanese RPV steels with various specimen sizes and shapes, and ascertained that the Master Curve can be well applied to the specimens with the thickness of 0.4-inches or larger. Considering the possible application of the Master Curve method coexistent with the present surveillance program for operating RPVs, the utilization of miniature specimens which can be taken from broken halves of surveillance specimens is quite important for the efficient determination of the Master Curve from the limited volume of the materials of concern. In this study, fracture toughness tests were conducted for typical Japanese RPV steels, SFVQ1A forging and SQV2A plate materials, using the miniature C(T) specimens with the thickness of 4 mm following the procedure of the ASTM standard. The results showed that the differences in test temperature, evaluation method, and specimen size did not affect the Master Curves, and the fracture toughness indexed by the reference temperature, T0, obtained from miniature C(T) specimens were consistent with those obtained from standard and larger C(T) specimens. It was also found that valid reference temperature can be determined with the realistic number of miniature C(T) specimens, less than ten, if the test temperature was appropriately selected. Thus, the Master Curve method using miniature C(T) specimens could be a practical method to determine the fracture toughness of actual RPV steels.


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