Testing and Numerical Simulation of Elastomeric Seals Under Consideration of Time Dependent Effects

Author(s):  
Mike Weber ◽  
Anja Kömmling ◽  
Matthias Jaunich ◽  
Dietmar Wolff ◽  
Uwe Zencker ◽  
...  

Due to delays in the siting procedure to establish a deep geological repository for spent nuclear fuel and high level waste and in construction of the already licensed Konrad repository for low and intermediate level waste, extended periods of interim storage will become more relevant in Germany. BAM is involved in most of the cask licensing procedures and is responsible for the evaluation of cask-related long-term safety issues. Elastomeric seals are widely used as barrier seals for containers for low and intermediate level radioactive waste. In addition they are also used as auxiliary seals in spent fuel storage and transportation casks (dual purpose casks (DPC)). To address the complex requirements resulting from the described applications, BAM has initiated several test programs for investigating the behavior of elastomeric seals. These include experiments concerning the hyperelastic and viscoelastic behavior at different temperatures and strain rates, the low temperature performance down to −40°C, the influence of gamma irradiation and the aging behavior. The first part of the paper gives an overview of these tests, their relevant results and their possible impact on BAM’s work as a consultant in the framework of approval and licensing procedures. The second part presents an approach of the development of a finite element model using the finite element code ABAQUS®. The long-term goal is to simulate the complex elastomeric behavior in a complete lid closure system under specific operation and accident conditions.

Author(s):  
Mike Weber ◽  
Anja Kömmling ◽  
Matthias Jaunich ◽  
Dietmar Wolff ◽  
Uwe Zencker ◽  
...  

Extended periods of interim storage are more relevant in Germany due to delays in the siting procedure to establish a deep geological repository for spent nuclear fuel, high level radioactive waste and in low/intermediate level waste container storage designated for the Konrad repository. BAM is involved in national cask licensing procedures and responsible for the evaluation of cask-related long-term safety issues. The long-term performance of elastomer seals for lid systems of transport and storage casks, whether used as auxiliary seals in spent fuel casks or as primary seals for low and intermediate level waste packages, is an important issue in this context. The polymeric structure of these seals causes a complex mechanical behavior with time-dependent sealing force reduction. The results of a comprehensive purpose-designed test program consisting of basic compression and tension tests as well as relaxation tests on unaged specimens of representative types of elastomers (fluorocarbon rubber (FKM) and ethylene propylene diene rubber (EPDM)) at different temperatures and strain rates are presented. They were used to identify the constitutive behavior and to obtain parameters for finite element material models provided by the computer code ABAQUS®. After estimating the influence of parameters such as Poisson’s ratio and friction coefficient by sensitivity analyses, the chosen values for the finite element simulation were validated by comparison with specimen test results. Based on this preliminary work the simulation of a specific laboratory test configuration containing a typical elastomer seal with circular cross section is presented. The chosen finite element material model and the related parameters had to show that they are able to represent not only the specimen behavior under predominantly uniaxial load but also the more complex stress states in real components. Deviations between the measured and calculated results are pointed out and discussed. The results from this work will be utilized in future simulations of aged elastomer behavior.


Author(s):  
Matthias Jaunich ◽  
Anja Kömmling ◽  
Jutta Horn ◽  
Holger Völzke ◽  
Dietmar Wolff

Elastomers show a high versatility which makes them ideal materials for sealing applications in various fields. Especially under changing application conditions the high recovery potential of this class of material is beneficial to compensate temperature or pressure fluctuation, and geometrical changes resulting from mechanical loads in e.g. accident conditions. Out of these reasons elastomers are also used in containers for low and intermediate level radioactive waste and for spent fuel transportation casks. In casks designed for low and intermediate level waste elastomer seals can act as primary seal responsible for the containment function whereas in spent fuel storage and transportation casks (dual purpose casks (DPC)) elastomer seals are used as auxiliary seals to allow leakage rate measurements of metal barrier seals. An inherent prerequisite for this kind of application is the long time-scale of operation without or with limited possibility of seal replacement. In Germany an interim storage license for DPC’s is typically issued for 40 years, a timeframe which might increase in the future due to challenges of the final repository siting procedure. For low and intermediate level waste, also long time periods are required before final disposal can be achieved. Therefore, the performance of elastomer seals over extended time periods is, as for other applications, of high importance. A typical approach to ensure long-term functionality is to perform accelerated aging tests to calculate an estimated lifetime by assuming e.g. Arrhenius like equations for the timetemperature relationship. This approach requires a suitable end of life criterion considering the application of interest. This often can represent a challenge on its own. As BAM is involved in most of the cask licensing procedures and especially responsible for the evaluation of cask-related long-term safety issues we initiated several test programs for investigating the behavior of elastomer seals. Experiments concerning the low temperature performance down to −40 °C and the influence of gamma irradiation have been started first. Currently the thermal aging behavior of elastomer seals, which is the topic of this contribution, is examined. For our aging investigations we use a broad approach to first determine the property changes in different elastomer materials due to thermo-oxidative aging at elevated temperatures and secondly, we test how the typical methods of lifetime extrapolation can be applied to these results. This approach enables us to detect and exclude undesired side effects which very often influence lifetime estimations. In this contribution, our recent results are extended. The results show that lifetime estimation based on single material properties can be misleading and therefore a combination of several methods is recommended.


2021 ◽  
Vol 1 ◽  
pp. 263-264
Author(s):  
Dirk Mallants ◽  
John Phalen ◽  
Hef Griffiths

Abstract. Around the world, deep borehole disposal is being evaluated for intermediate-level waste (ILW), high-level waste (HLW), spent nuclear fuel (SNF), separated plutonium waste and some very high specific activity fission product waste. In Australia, long-lived ILW from research reactors and radiopharmaceutical production represents the principal waste stream that requires deep geologic disposal. Whilst the Australian government has not yet made a decision on its preferred strategy for ILW disposal, deep borehole disposal of small volumes of ILW would be a more cost-effective and modular solution compared to a conventional geologic disposal facility (GDF). CSIRO, ANSTO and SANDIA have created an international partnership to execute a full-scale borehole research, development and demonstration (RD&D) project in Australia. The project will demonstrate the technical feasibility of the long-term safety of borehole disposal in deep geological formations. The execution of this project could also demonstrate options for nuclear waste disposal that would reduce proliferation risks, potentially up to the termination of compliance with international safeguards requirements. The RD&D includes demonstration of surface handling and waste/seal emplacement capabilities, basic research on foundational science areas, and full-scale field testing in both a deep characterization borehole and a larger-diameter (0.7 m or 27.5 inch) 2000 m deep demonstration borehole. The multi-barrier system designed for such a deep disposal borehole concept places much less reliance on engineered barriers at the disposal zone to achieve safety as compared to a conventional GDF. It rather relies on geological features for waste containment. The concept being explored uses disposal containers with primary waste packages, such as vitrified waste canisters, inside; to be both cost effective and fit for purpose, such a container could have a mild steel-based structural component with copper coating. A critical review of six coating technologies showed that cold spray has the greatest advantages, such as minimal porosity and compressive residual stress. The RD&D has delivered novel enabling tools that assist with site screening, borehole design and post-closure safety assessments. For instance, an automated geological fault mapping and meshing tool was developed that assists with ranking the suitability of potential disposal sites based on proximity to faults. New codes were developed for better representation of fault zones in 2D/3D numerical flow and transport models, while also being more efficient to execute. Post-closure safety assessments tested the sensitivity of long-term safety with respect to disposal depth, rock permeability and sorption. Heat transport calculations explored the sensitivity of temperature evolution within the borehole to parameters such as heat load, borehole depth, geothermal gradients and rock thermal conductivity. For verification of host rock tightness while also demonstrating the absence of recent groundwater, a new noble gas analytical facility has been established for measuring rare noble gases in mineral fluid inclusions as indicators of very old pore fluids.


Author(s):  
Ievgen Levadnyi ◽  
Jan Awrejcewicz ◽  
Yan Zhang ◽  
Yaodong Gu

Bone fracture, formation and adaptation are related to mechanical strains in bone. Assessing bone stiffness and strain distribution under different loading conditions may help predict diseases and improve surgical results by determining the best conditions for long-term functioning of bone-implant systems. In this study, an experimentally wide range of loading conditions (56) was used to cover the directional range spanned by the hip joint force. Loads for different stance configurations were applied to composite femurs and assessed in a material testing machine. The experimental analysis provides a better understanding of the influence of the bone inclination angle in the frontal and sagittal planes on strain distribution and stiffness. The results show that the surface strain magnitude and stiffness vary significantly under different loading conditions. For the axial compression, maximal bending is observed at the mid-shaft, and bone stiffness is also maximal. The increased inclination leads to decreased stiffness and increased magnitude of maximum strain at the distal end of the femur. For comparative analysis of results, a three-dimensional, finite element model of the femur was used. To validate the finite element model, strain gauges and digital image correlation system were employed. During validation of the model, regression analysis indicated robust agreement between the measured and predicted strains, with high correlation coefficient and low root-mean-square error of the estimate. The results of stiffnesses obtained from multi-loading conditions experiments were qualitatively compared with results obtained from a finite element analysis of the validated model of femur with the same multi-loading conditions. When the obtained numerical results are qualitatively compared with experimental ones, similarities can be noted. The developed finite element model of femur may be used as a promising tool to estimate proximal femur strength and identify the best conditions for long-term functioning of the bone-implant system in future study.


2003 ◽  
Vol 807 ◽  
Author(s):  
Paul Wersin ◽  
Lawrence H. Johnson ◽  
Bernhard Schwyn

ABSTRACTRedox conditions were assessed for a spent fuel and high-level waste (SF/HLW) and an intermediate-level waste (ILW) repository. For both cases our analysis indicates permanently reducing conditions after a relatively short oxic period. The canister-bentonite near field in the HLW case displays a high redox buffering capacity because of expected high activity of dissolved and surface-bound Fe(II). This is contrary to the cementitious near field in the ILW case where concentrations of dissolved reduced species are low and redox reactions occur primarily via solid phase transformation processes.For the bentonite-canister near field, redox potentials of about -100 to -300 mV (SHE) are estimated, which is supported by recent kinetic data on U, Tc and Se interaction with reduced iron systems. For the cementitious near field, redox potentials of about -200 to -800 mV are estimated, which reflects the large uncertainties related to this alkaline environment.


Author(s):  
Zekai Ceylan ◽  
Mohamed B. Trabia

Abstract Welded cylindrical containers usually experience stress corrosion cracking (SCC) in the closure-weld area. Induction coil heating technique may be used to relieve the residual stresses from the closure-weld. This technique involves localized heating of the material by the surrounding coils. The material is then cooled to the room temperature by quenching. A two-dimensional axisymmetric finite element model is developed to study the effects of induction coil heating and subsequent quenching. The finite element results are validated through an experimental test. The parameters of the design are tuned to maximize the compressive stress within a layer of thickness from the outer surface that is equal to the long-term general corrosion of Alloy 22 (Appendix A). The problem is subject to geometrical and stress constraints. Two different solution methods are implemented for this purpose. First, an off-the-shelf optimization software is used to obtain an optimum solution. These results are not satisfactory because of the highly nonlinear nature of the problem. The paper proposes a novel alternative: the Successive Heuristic Quadratic Approximation (SHQA) technique. This algorithm combines successive quadratic approximation with an adaptive random search. Examples and discussion are included.


2012 ◽  
Vol 1475 ◽  
Author(s):  
Aku Itälä ◽  
Arto Muurinen

ABSTRACTThe Finnish spent nuclear fuel disposal is based on the Swedish KBS-3 concept in crystalline bedrock. The concept aims at long-term isolation and containment of spent fuel in copper canisters surrounded by bentonite buffer which mostly consists of montmorillonite. For the long-term modelling of the chemical processes in the buffer, the cation-exchange selectivity coefficients have to be known at different temperatures. In this work, the cation-exchange selectivity coefficients and cation-exchange isotherms were determined in batch experiments for montmorillonite at three different temperatures (25 °C, 50 °C and 75 °C). Five different ratios of NaClO4/Ca(ClO4)2 were used in the experimental solutions. After equilibration the solution and montmorillonite were separated and the solution analysed to get the desired exchange parameters. The experiments were modelled with a computational model capable of taking into account the physicochemical processes that take place in the experiment.


Author(s):  
Xiang Liu ◽  
Yue Li ◽  
Jinhua Wang ◽  
Bin Wu

The spent nuclear fuel of HTR-PM (High Temperature Reactor–Pebblebed Modules) will be dry stored in wells. In the mouth of each well, there is a cover weighing 11 tons. A lifting appliance with three hooks is used to open and close the covers. The hooks are L-shaped with fillet at the inside corner. The stress concentration at the corner has a significant impact on the strength and fatigue life of hooks. For optimizing the structure of the hook, the stress concentration factor related to the radius of fillet is calculated by both theoretical and numerical methods. The theoretical calculation is based on the Saint-Venant’s Principle and the analytical solution of a curved beam. The result is consistent with the numerical calculation performed by the finite element method.


Sign in / Sign up

Export Citation Format

Share Document