Viscoelectric Effect on the Electroosmotic Flow in Nanochannels With Heterogeneous Zeta Potentials

Author(s):  
Edson M. Jimenez ◽  
Federico Méndez ◽  
Juan P. Escandón

In the present work, we realize a study about the influence of viscoelectric effect on the electroosmotic flow of Newtonian fluids in nanochannels formed by two parallel flat plates. In the problem, the channel walls have heterogeneous zeta potentials which follow a sinusoidal distribution; moreover, viscoelectric effects appear into the electric double layers when high zeta potentials are considered at the channel walls, modifying the fluid viscosity and the fluid velocity. To find the solution of flow field, the modified Poisson-Boltzmann, mass conservation and momentum governing equations, are solved numerically. In the results, combined effects from the zeta potential heterogeneities and viscosity changes yields different kind of flow recirculations controlled by the dephasing angle, amplitude and number of waves of the heterogeneities at the walls. The viscoelectric effect produces a decrease in the magnitude of velocity profiles and volumetric flow rate when the high zeta potentials are magnified. Additionally, the heterogeneous zeta potentials at the walls generate an induced pressure on the flow. This investigation extend the knowledge of electroosmotic flows under field effects for future mixing applications.

2020 ◽  
Vol 66 (6 Nov-Dec) ◽  
pp. 761
Author(s):  
J. Arcos ◽  
O. Bautista ◽  
F. Méndez ◽  
M. Peralta

We present the analysis of an electroosmotic flow (EOF) of a Newtonian fluid in a wavy-wall microchannel. In order to describe the flow and electrical fields, the lubrication and Debye-Hückel approximations are used. The simplified governing equations of continuity, momentum and Poisson-Boltzmann, together with the boundary conditions are presented in dimensionless form. For solving the mathematical problem, numerical and asymptotic techniques were applied. The asymptotic solution is obtained in the limit of very thin electric double layers (EDLs). We show that the lubrication theory is a powerful technique for solving the hydrodynamic field in electroosmotic flows in microchannels where the amplitude of the waviness changes on the order of the  mean semi-channel height. Approximate analytical expressions for the velocity components and pressure distribution are derived, and a closed formula for the volumetric flow rate is obtained.  The results show that the principal parameters that govern this EOF are the geometrical parameter, ε, which characterizes the waviness of the microchannel and the ratio of the mean semi-channel height to the thickness of the EDL, κ.


Author(s):  
Juan P. Escandón ◽  
David A. Torres

Abstract This paper presents the 2-D numerical solution of the flow and concentration field of an electrokinetic T-type micromixer, under heterogeneous zeta potentials modulated via sinusoidal functions and interfacial viscoelectric effects. Here, the viscoelectric effects appear to modify the fluid viscosity due to the high voltages within the electric double layer. The mathematical model is based on the Poisson-Boltzmann, mass conservation, momentum, and species concentration equations. In the steady-state analysis, two electrolytes with known ionic concentration and an imposed velocity profile are considered at the inlet of the micromixer. The results demonstrate that by using heterogeneous zeta potentials, at the mixer walls, generated flow recirculations along the mixer channel, promoting the rise in mixing efficiency; however, for high zeta potential values, this is counteracted by the viscoelectric effects. The present investigation shows how the viscoelectric condition deteriorates the mixing performance and how with the correct selection of modulated zeta potential parameters as the wave number, and the phase angle can improve it. Therefore, the performance of the mixer studied here should be considered for the design of microfluidic devices in the future.


RSC Advances ◽  
2017 ◽  
Vol 7 (12) ◽  
pp. 7274-7286 ◽  
Author(s):  
Gan-Jun Cen ◽  
Chien-Cheng Chang ◽  
Chang-Yi Wang

Optimal EO pumping rates on the plane of zeta potentials with distribution of the inner radius of annular tube.


Author(s):  
Wu Zhong ◽  
Yunfei Chen

The governing equations of electroosmotic flow, including the Navier-Stokes (N-S) equations, Laplace equation and Poisson-Boltzmann equation, are set up in a straight microchannel. The meshless method is employed as a discrete scheme for the solution domain. The semi-implicit multistep (SIMS) method is used to solve the Navier-Stokes equations. The simulation results demonstrated that different patterns of the zeta potential over the channel surface could induce different flow profiles for the vortex. The rotational direction of the vortex is determined by the electroosmotic driving force.


Author(s):  
Juan P. Escandón ◽  
Eduardo G. Merino ◽  
Clara G. Hernández

This paper presents an analytical study of the transient electroosmotic flow for Newtonian fluids through a parallel flat plate microchannel with heterogeneous zeta potentials. The dimensionless mathematical model is based on the Poisson-Boltzmann, mass and momentum conservation governing equations together with the lubrication theory. The distribution of the zeta potentials at the walls obeys to a sinusoidal function, which includes dimensional parameters as Δζ that controls the magnitude and polarity of the zeta potentials, being capable to produce slanted velocity profiles and inverse flows. On the other hand, the combination of the phase angle between the sinusoidal functions of the zeta potentials ω, the dimensionless parameter of their amplitude Δζ, and the parameter that controls the frequency of the sinusoidal functions m, induce additional perturbations on the flow, which is directly related to the dimensionless pressure distribution and to the transient flow field. The transient behavior characteristics of the electroosmotic flow are discussed in terms of the zeta potential variations. It is demonstrated that the results for the transient electroosmotic flow, predict the influence of the main dimensionless parameters above mentioned on the velocity profiles and the streamlines. This work about the perturbations on the electroosmotic flow by heterogeneous zeta potentials, contributes to a better understanding of the transport phenomena in microfluidic devices for future mixing applications.


2000 ◽  
Author(s):  
Mehrdad Massoudi ◽  
Tran X. Phuoc

Abstract In this paper we study the flow of granular materials between two horisontal flat plates where the top plate is moving with a constant speed. The constitutive relation used for the stress is based on the continuum model proposed by Rajagopal and Massoudi (1990), where the material parameters are derived using the kinetic theory model proposed by Boyle and Massoudi (1990). The governing equations are non-dimensionalized and the resulting system of non-linear differential equations is solved numerically using finite difference technique.


1997 ◽  
Vol 52 (4) ◽  
pp. 358-368 ◽  
Author(s):  
Michio Nishida ◽  
Masashi Matsumotob

Abstract • This paper describes a computational study of the thermal and chemical nonequilibrium occuring in a rapidly expanding flow of high-temperature air transported as a free jet from an orifice into low-density stationary air. Translational, rotational, vibrational and electron temperatures are treated separately, and in particular the vibrational temperatures are individually treated; a multi-vibrational temperature model is adopted. The governing equations are axisymmetric Navier-Stokes equations coupled with species vibrational energy, electron energy and species mass conservation equations. These equations are numerically solved, using the second order upwind TVD scheme of the Harten-Yee type. The calculations were carried out for two different orifice temperatures and also two different orifice diameters to investigate the effects of such parameters on the structure of a nonequilibrium free jet.


2015 ◽  
Vol 138 (3) ◽  
Author(s):  
Morteza Sadeghi ◽  
Arman Sadeghi ◽  
Mohammad Hassan Saidi

Adopting the Navier slip conditions, we analyze the fully developed electroosmotic flow in hydrophobic microducts of general cross section under the Debye–Hückel approximation. The method of analysis includes series solutions which their coefficients are obtained by applying the wall boundary conditions using the least-squares matching method. Although the procedure is general enough to be applied to almost any arbitrary cross section, eight microgeometries including trapezoidal, double-trapezoidal, isosceles triangular, rhombic, elliptical, semi-elliptical, rectangular, and isotropically etched profiles are selected for presentation. We find that the flow rate is a linear increasing function of the slip length with thinner electric double layers (EDLs) providing higher slip effects. We also discover that, unlike the no-slip conditions, there is not a limit for the electroosmotic velocity when EDL extent is reduced. In fact, utilizing an analysis valid for very thin EDLs, it is shown that the maximum electroosmotic velocity in the presence of surface hydrophobicity is by a factor of slip length to Debye length higher than the Helmholtz–Smoluchowski velocity. This approximate procedure also provides an expression for the flow rate which is almost exact when the ratio of the channel hydraulic diameter to the Debye length is equal to or higher than 50.


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