The Hydrogeologic Environment for a Proposed Deep Geologic Repository in Canada for Low and Intermediate Level Radioactive Waste

Author(s):  
Jonathan F. Sykes ◽  
Stefano D. Normani ◽  
Yong Yin ◽  
Mark R. Jensen

A Deep Geologic Repository (DGR) for low and intermediate level radioactive waste has been proposed by Ontario Power Generation for the Bruce nuclear site in Ontario, Canada. As proposed the DGR would be constructed at a depth of about 680 m below ground surface within the argillaceous Ordovician limestone of the Cobourg Formation. This paper describes the hydrogeology of the DGR site developed through both site characterization studies and regional-scale numerical modelling analysis. The analysis provides a framework for the assembly and integration of the site-specific geoscientific data and examines the factors that influence the predicted long-term performance of the geosphere barrier. Flow system evolution was accomplished using both the density-dependent FRAC3DVS-OPG flow and transport model and the two-phase gas and water flow computational model TOUGH2-MP. In the geologic framework of the Province of Ontario, the DGR is located on the eastern flank of the Michigan Basin. Borehole logs covering Southern Ontario combined with site-specific data from 6 deep boreholes have been used to define the structural contours and hydrogeologic properties at the regional-scale of the modelled 31 sedimentary strata that may be partially present above the Precambrian crystalline basement rock. The regional-scale domain encompasses an approximately 18500km2 region extending from Lake Huron to Georgian Bay. The groundwater zone below the Devonian includes units containing stagnant water having high concentrations of total dissolved solids that can exceed 300g/L. The Ordovician sediments are significantly under-pressured. The horizontal hydraulic conductivity for the Cobourg limestone is estimated to be 2 × 10−14 m/s based on straddle-packer hydraulic tests. The low advective velocities in the Cobourg and other Ordovician units result in solute transport that is diffusion dominant with Peclet numbers less than 0.003 for a characteristic length of unity. Long-term simulations that consider future glaciation scenarios include the impact of ice thickness and permafrost. Solute transport in the Ordovician limestone and shale was diffusion dominant in all simulations. The Salina formations of the Upper Silurian prevented the deeper penetration of basal meltwater.

Author(s):  
Jonathan F. Sykes ◽  
Stefano D. Normani ◽  
Yong Yin ◽  
Eric A. Sykes ◽  
Mark R. Jensen

A Deep Geologic Repository (DGR) for Low and Intermediate Level radioactive waste has been proposed by Ontario Power Generation for the Bruce Nuclear Power Development site in Ontario, Canada. The DGR is to be constructed at a depth of about 680 m below ground surface within the argillaceous Ordovician limestone of the Cobourg Formation. This paper describes a regional-scale geologic conceptual model for the DGR site and analyzes flow system evolution using the FRAC3DVS-OPG flow and transport model. This provides a framework for the assembly and integration of site-specific geoscientific data that explains and illustrates the factors that influence the predicted long-term performance of the geosphere barrier. In the geologic framework of the Province of Ontario, the Bruce DGR is located at the eastern edge of the Michigan Basin. Borehole logs covering Southern Ontario combined with site specific data have been used to define the structural contours at the regional and site scale of the 31 sedimentary strata that may be present above the Precambrian crystalline basement rock. The regional-scale domain encompasses an 18.500km2 region extending from Lake Huron to Georgian Bay. The groundwater zone below the Devonian is characterized by units containing stagnant water having high concentrations of total dissolved solids that can exceed 300g/l. The computational sequence involves the calculation of steady-state density independent flow that is used as the initial condition for the determination of pseudo-equilibrium for a density dependent flow system that has an initial TDS distribution developed from observed data. Long-term simulations that consider future glaciation scenarios include the impact of ice thickness and permafrost. The selection of the performance measure used to evaluate a groundwater system is important. The traditional metric of average water particle travel time is inappropriate for geologic units such as the Ordovician where solute transport is diffusion dominant. The use of life expectancy and groundwater age is a more appropriate metric for such a system. The mean life expectancy for the DGR and base case parameters has been estimated to be in excess of 8 million years.


Author(s):  
A. V. Chambers ◽  
W. R. Rodwell ◽  
M. Kelly ◽  
A. R. Hoch ◽  
A. J. Baker

In the UK, the need for the long-term management of intermediate-level radioactive wastes arises from the absence of an established deep disposal option. As a consequence there is a requirement to demonstrate the ‘passive safety’ of waste packages in stores over a necessarily lengthy period (perhaps 150 years or more). ‘Passive safety’ is taken here to imply that the waste packages themselves would remain safe without intervention; it is assumed however, that the store building and associated infrastructure would need to be actively maintained and that the store may need to be ventilated. Importantly, methods for waste storage also need to ensure that possible future options for disposal are not foreclosed. An extended period of storage suggests that emphasis will need to be placed by waste producers on understanding a number of issues such as: • the impact of corrosion on container integrity; • the assessment of container vents and other features as a pathway for the release of radioactivity; • the extent to which wastes are conditioned for storage and the selection of appropriate methods; • the generation and behaviour of toxic or flammable gases in the storage facility; and the mitigating steps that might be needed to address adverse impacts (e.g. the type of ventilation that the store requires). In this paper, we review the requirements and current state of knowledge relevant to the assessment of operational releases of radioactive, flammable and toxic gases from wastes in long-term interim storage.


Author(s):  
David Horsley ◽  
Bruce McKirdy

Nirex is the organisation responsible for long-term radioactive waste management in the UK. Our Mission is to provide the UK with safe, environmentally sound and publicly acceptable options for the long-term management of radioactive materials. The United Kingdom has a significant legacy of long-lived intermediate level radioactive waste. This has arisen from 50 years of investigation and exploitation of nuclear technology. Some of the waste is stored in old facilities that do not provide the standards of containment that would be incorporated in modern facilities. Also the risk to people and to the environment from the inventory in these facilities will increase with time as the structures age and degrade, increasing the chance of containment failure. There is, therefore, a need to retrieve this raw waste and process and package it to make it demonstrably safe for continued storage, pending a decision on disposal of radioactive waste. This packaging should, as far as is practicable, be compatible with the UK long-term waste management strategy. Nirex has developed its Phased Disposal Concept for intermediate and low-level radioactive waste. Based on that concept, Nirex has developed waste package specifications and carries out assessments of waste packaging proposals. For legacy wastes it may not always practicable to demonstrate full compliance with all Nirex disposal criteria. This paper describes an approach, agreed between Nirex and BNFL, for managing these wastes. The proposed approach takes account of long-term waste management issues whilst recognising the need for timely improvement of storage conditions.


Author(s):  
Ju¨rgen Wollrath ◽  
Ju¨rgen Preuss ◽  
Dirk-A. Becker ◽  
Jo¨rg Mo¨nig

The Morsleben repository has been in operation since 1971 as a repository for low- and intermediate-level radioactive waste. Until the end of the disposal phase in 1998 a waste volume of about 37,000 m3 with a total activity of 4.5·1014 Bq was disposed of. Currently, the German Federal Office for Radiation Protection (BfS) is applying for the licence to finally close the repository. Concerning the possible release of radionuclides to the biosphere, the repository is subject to German radiation protection regulations. Their fulfilment has to be proven by means of numerical calculations as a part of the safety case. A simplified repository model has been developed by GRS and used for calculating the consequences of different scenarios and variants, as well as for a probabilistic uncertainty and sensitivity analysis. The application for licensing is, among others, based on these results. In this paper the main features of the model and the underlying assumptions, as well as the most important calculation results are presented and explained.


1997 ◽  
Vol 506 ◽  
Author(s):  
H. N. Waber ◽  
F. J. Pearson ◽  
A. Scholtis

The Wellenberg area, central Switzerland, is under investigation for a potential low and intermediate level radioactive waste repository. The host rock, the Palfris marl, is bounded on the north by Cretaceous limestone units of the Drusberg nappe and is underlain by a sequence of Tertiary to Jurassic sediments (limestones, marls) of the Wissberg-Firrenband-Equivalent. Chemical and isotopic data on groundwaters and rocks show that three essentially independent groundwater flow regimes occur in the area: (1) groundwaters of the Palfris marl, (2) groundwaters of the limestone units of the Drusberg nappe, and (3) groundwaters of the Wissberg-Firrenband Equivalent.


2016 ◽  
Vol 151 ◽  
pp. 395-403 ◽  
Author(s):  
Ulrik Kautsky ◽  
Peter Saetre ◽  
Sten Berglund ◽  
Ben Jaeschke ◽  
Sara Nordén ◽  
...  

Author(s):  
Regeane Martins de Freitas ◽  
Abir Al-Tabbaa

Although cementation is a widely recognized solidification/stabilization process for immobilisation of Intermediate Level Radioactive Waste (ILRW), the low resistance to hyperalkaline pore waters compromises the effectiveness of the process when Portland Cement (PC) is employed. Moreover the manufacture of PC is responsible for significant CO2 emissions. In this context, low pH cements are environmentally more suitable and have emerged as a potential alternative for obtaining secure waste forms. This paper summarises the achievements on development of low-pH cements and the challenges of using these new materials for the ILRW immobilisation. The performance of waste forms is also discussed in terms of radionuclides release. Reactive magnesium oxide and magnesium phosphate cements are emphasised as they feature important advantages such as consumption of available constituents for controlling acid-base reactions, reduced permeability and higher density. Additionally, in order to identify new opportunities for study, the long-term modelling approach is also briefly discussed.


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