Mode Resolved Continuum Mechanics Model of Phonon Scattering From Embedded Cylinders

Author(s):  
Vineet Unni ◽  
Joseph P. Feser

Phonon scattering from media with embedded spherical nanoparticles has been studied extensively over the last decade due to its application to reducing the thermal conductivity of thermoelectric materials. However, similar studies of thermal transport in fiber-embedded media have received little attention. Calculating the thermal conductivity tensor from microscopic principles requires knowledge of the scattering cross section spanning all possible incident elastic wave orientations, polarizations and wavelengths including the transition from Rayleigh to geometric scattering regimes. In this paper, we use continuum mechanics to develop an analytic treatment of elastic wave scattering for an embedded cylinder and show that a classic treatise on the subject contains important errors for oblique angles of incidence, which we correct. We also develop missing equations for the scattering cross section at oblique angles and study the sensitivity of the scattering cross section as a function of elas-todynamic contrast mechanisms. In particular, we find that for oblique angles of incidence, both elastic and density contrast are important mechanisms by which scattering can be controlled, but that their effects can offset one another, similar to the theory of reflection at flat interfaces. The solution developed captures the scattering physics for all possible incident elastic wave orientations, polarizations and wavelengths including the transition from Rayleigh to geometric scattering regimes, so long as the continuum approximation holds. The method thus enables incorporation of coherent scattering models into calculations of the thermal conductivity tensor for media with nanofibers.

2018 ◽  
Vol 141 (1) ◽  
Author(s):  
Vineet Unni ◽  
Joseph P. Feser

In this paper, we use continuum mechanics to develop an analytic treatment of elastic wave scattering from an embedded cylinder and show that a classic treatise on the subject contains important errors for oblique angles of incidence, which we correct. We also develop missing equations for the scattering cross section at oblique angles and study the sensitivity of the scattering cross section as a function of elastodynamic contrast mechanisms. We find that in the Mie scattering regime for oblique angles of incidence, both elastic and density contrast are important mechanisms by which scattering can be controlled, but that their effects can offset one another, similar to the theory of reflection at flat interfaces. In comparison, we find that in the Rayleigh scattering regime, elastic and density contrast are always complimentary toward increasing scattering cross section, but for sufficiently high density contrast, the scattering cross section for incident compressional and y-transverse modes is nearly independent of elastic contrast. The solution developed captures the scattering physics for all possible incident elastic wave orientations, polarizations, and wavelengths including the transition from Rayleigh to geometric scattering regimes, so long as the continuum approximation holds. The method could, for example, enable calculation of the thermal conductivity tensor from microscopic principles which requires knowledge of the scattering cross section spanning all possible incident elastic wave orientations and polarizations at thermally excited wavelengths.


ACS Nano ◽  
2019 ◽  
Vol 13 (7) ◽  
pp. 8347-8355 ◽  
Author(s):  
Junphil Hwang ◽  
Hoon Kim ◽  
Mi-Kyung Han ◽  
Jisook Hong ◽  
Ji-Hoon Shim ◽  
...  

Author(s):  
Ravi S. Prasher

Scattering theory for the scattering of phonons by particulate scatterers is developed in this paper. Recently the author introduced the generalized equation of phonon radiative transport (GEPRT) in particulate media which included a phase function to account for the anisotropic scattering of phonons by particulate scatterer. Solution of the GEPRT showed that scattering cross section is different than the thermal transport cross section. In this paper formulations for the scattering and transport cross section for horizontally shear (SH) wave phonon or transverse wave phonon without mode conversion is developed. The development of the theory of scattering and the transport cross section is exactly analogous to the Mie scattering theory for photon transport in particulate media. Results show that transport cross section is very different than the scattering cross section. It is also shown that for SH (horizontally shear) phonons the scattering and transport cross sections are proportional to ω8 rather than the well accepted value of ω4 in the Rayleigh regime where ω is the frequency of the SH phonons. The theory of phonon scattering developed in this paper will be useful for the predictive modeling of thermal conductivity of practical systems such as nano composites, nano-micro particle laden systems and etc.


Author(s):  
M. K. Lamvik ◽  
A. V. Crewe

If a molecule or atom of material has molecular weight A, the number density of such units is given by n=Nρ/A, where N is Avogadro's number and ρ is the mass density of the material. The amount of scattering from each unit can be written by assigning an imaginary cross-sectional area σ to each unit. If the current I0 is incident on a thin slice of material of thickness z and the current I remains unscattered, then the scattering cross-section σ is defined by I=IOnσz. For a specimen that is not thin, the definition must be applied to each imaginary thin slice and the result I/I0 =exp(-nσz) is obtained by integrating over the whole thickness. It is useful to separate the variable mass-thickness w=ρz from the other factors to yield I/I0 =exp(-sw), where s=Nσ/A is the scattering cross-section per unit mass.


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