Measurement of Selected Differential Cross Sections in 235U Spectrum

2019 ◽  
Vol 5 (3) ◽  
Author(s):  
Nicola Burianová ◽  
Michal Košt´ál ◽  
Martin Schulc ◽  
Jan Šimon ◽  
Martin Mareček ◽  
...  

This paper describes the measurement of 55Mn(n,2n) and 127I(n,2n) reaction rates in a well-defined reactor field in a special core of LR-0 reactor. The reaction rates were derived using gamma-spectrometry by measuring gamma activities of irradiated MnO2 and NaI samples at a high purity germanium (HPGe) detector. The spectral average cross section (SACS) in 235U prompt fission neutron spectrum (PFNS) was experimentally determined to be 0.2393 ± 0.015 × 10−3 b for 55Mn and 1.2087 ± 0.052 × 10−3 b for 127I. These obtained results were compared with calculations by MCNP6 code using ENDF/B VII.1, ENDF/B VII, JEFF-3.1, JEFF-3.2, JENDL-3.3, JENDL-4, ROSFOND- 2010, CENDL-3.1, and IRDFF nuclear data libraries. In a case of 55Mn, a good agreement with ENDF/B VII.1, JEFF 3.1, JENDL 3.3, JENDL 4, ROSFOND, and CENDL 3.1 nuclear data libraries was found, where C/E−1 is 0.1%, while IRDFF underestimated by about 15.8%. In the case of 127I, more significant discrepancies were found, where JENDL 3.3 and JENDL 4 overestimate the result by about 31.3%.

2018 ◽  
Vol 4 ◽  
pp. 35 ◽  
Author(s):  
Eric Bauge ◽  
Dimitri A. Rochman

Most recent evaluated nuclear data files exhibit excellent integral performance, as shown by the very good agreement between experimental and calculated keff values over a wide range of benchmark integral experiments. However, the propagation of the uncertainties associated with those nuclear data to integral observables, generally produces calculated distribution which are much (3–5 times) wider than the experimental uncertainties. Reducing the variances of the evaluated data to achieve consistency at the integral level would lead to unreasonably narrow variances in the light of differential experimental data. One way of solving that paradox could be to allow, for different observables like fission cross-sections (σf), the prompt fission neutron spectra (χ), and the average multiplicity of fission neutrons ([see formula in PDF]) to be correlated in a Bayesian-like, Total Monte-Carlo approach, under constraints from integral experiments from the ICSBEP (International International Criticality Safety Benchmark Evaluation Project) benchmark compilation. Future developments will be highlighted and restrictions imposed by the current formatting of nuclear data will be discussed.


Author(s):  
Martin Schulc ◽  
Michal Košťál ◽  
Evžen Novák ◽  
Jan Šimon ◽  
Nicola Burianová

This work deals with 23Na(n,2n)22Na and 127I(n,2n)126I reactions in the 252Cf spontaneous fission neutron source. 252Cf neutron source with approximate emission of 6·× 108 n/s was employed for the irradiation of sodium iodide. The spectrum-averaged cross sections (SACS) were then inferred from experimentally determined reaction rates and compared with calculations in MCNP6 using various nuclear data libraries. The experimental reaction rates were derived from the net peak areas (NPAs) measured using the high purity germanium spectroscopy. The measured SACS for the 23Na(n,2n)22Na reaction in the 252Cf spectrum was determined as equal to (8.98±0.32)·× 10−6 b. The resulting SACS for the 127I(n,2n)126I reaction in the 252Cf spectrum was derived as (2.044±0.0072)·× 10−3 b. These experimental data can be used for nuclear data libraries validation and to specify high energy tail of the 252Cf neutron spectrum.


Metrology ◽  
2021 ◽  
Vol 2 (1) ◽  
pp. 1-18
Author(s):  
Nikolay V. Kornilov ◽  
Vladimir G. Pronyaev ◽  
Steven M. Grimes

Each experiment provides new information about the value of some physical quantity. However, not only measured values but also the uncertainties assigned to them are an important part of the results. The metrological guides provide recommendations for the presentation of the uncertainties of the measurement results: statistics and systematic components of the uncertainties should be explained, estimated, and presented separately as the results of the measurements. The experimental set-ups, the models of experiments for the derivation of physical values from primary measured quantities, are the product of human activity, making it a rather subjective field. The Systematic Distortion Factor (SDF) may exist in any experiment. It leads to the bias of the measured value from an unknown “true” value. The SDF appears as a real physical effect if it is not removed with additional measurements or analysis. For a set of measured data with the best evaluated true value, their differences beyond their uncertainties can be explained by the presence of Unrecognized Source of Uncertainties (USU) in these data. We can link the presence of USU in the data with the presence of SDF in the results of measurements. The paper demonstrates the existence of SDF in Prompt Fission Neutron Spectra (PFNS) measurements, measurements of fission cross sections, and measurements of Maxwellian spectrum averaged neutron capture cross sections for astrophysical applications. The paper discusses introducing and accounting for the USU in the data evaluation in cases when SDF cannot be eliminated. As an example, the model case of 238U(n,f)/235U(n,f) cross section ratio evaluation is demonstrated.


1961 ◽  
Vol 123 (6) ◽  
pp. 2140-2142 ◽  
Author(s):  
A. B. Smith ◽  
R. K. Sjoblom ◽  
J. H. Roberts

2016 ◽  
Vol 111 ◽  
pp. 05004 ◽  
Author(s):  
D. Neudecker ◽  
P. Talou ◽  
T. Kawano ◽  
A.C. Kahler ◽  
M.E. Rising ◽  
...  

2020 ◽  
Vol 239 ◽  
pp. 05010
Author(s):  
Keegan J. Kelly ◽  
Jaime A. Gomez ◽  
John M. O'Donnell ◽  
Matthew Devlin ◽  
Robert C. Haight ◽  
...  

Prompt fission neutron spectrum (PFNS) evaluations use provide nuclear data for the PFNS across a wide range of incident and outgoing neutron energies. However, experimental data underlying the evaluation are sparse, inconsistent, and incomplete with respect to the desired incident and outgoing energy coverage. As such, evaluations sometimes predict features of the PFNS, such those relating to multi-chance fission and pre-equilibrium pre-fission neutron emission, without any experimental validation. The Chi-Nu experiment at Los Alamos National Laboratory has recently obtained high-precision results for the 239Pu and 235U PFNS which, for the first time in both cases, have shed light on multi-chance fission and pre-equilibrium contributions to the observed fission neutron spectrum. In addition to providing the first experimental data on some of these fission properties, the angular coverage of the Chi-Nu experiment allows for the extraction of angular distributions of pre-equilibrium pre-fission neutrons. PFNS results of multi-chance fission and pre-equilibrium pre-fission neutron emission are discussed in this proceedings in terms of the observed neutron spectrum and the average PFNS energies.


2014 ◽  
Vol 119 ◽  
pp. 205-208 ◽  
Author(s):  
R.C. Haight ◽  
H.Y. Lee ◽  
T.N. Taddeucci ◽  
J.M. O'Donnell ◽  
B.A. Perdue ◽  
...  

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