Self-phase modulation in perfluorinated polymer-based GI polymer optical fiber with intense femtosecond laser pulse

Author(s):  
M. Kanai ◽  
M. Obara
2017 ◽  
Vol 26 (04) ◽  
pp. 1750051 ◽  
Author(s):  
Yunxia Huang ◽  
Shuwu Xu ◽  
Shian Zhang

Femtosecond coherent anti-Stokes Raman scattering (CARS) spectra from close Raman levels are indistinguishable due to the large bandwidth of the femtosecond laser pulse. In this paper, we propose a scheme to realize high resolution CARS spectra and further the selective suppression and excitation of the Raman levels by phase shaped femtosecond laser pulse. We show that the CARS signals can be narrowed and differentiated by tailoring only the probe pulse. In addition, one or more of the spectra peaks can be suppressed to realize the selective excitation by further scanning the pump pulse with [Formula: see text] or double reverse [Formula: see text] spectral phase modulation.


2011 ◽  
Vol 84 (1) ◽  
Author(s):  
Shian Zhang ◽  
Chenhui Lu ◽  
Junhui Shi ◽  
Tianqing Jia ◽  
Zugeng Wang ◽  
...  

2018 ◽  
Vol 5 (1) ◽  
pp. 171502
Author(s):  
Yunxia Huang ◽  
Shuwu Xu

We demonstrate that the population of the molecular rotational state through a stimulated impulsive Raman excitation can be controlled by tailoring the femtosecond laser pulse with a V-style phase modulation. The results show that, by precisely manipulating the modulation parameters, both the odd and even populations of the molecular rotational state can be completely suppressed or reconstructed. Meanwhile, the relative excitation between the odd and even populations can be obtained. Finally, we show that field-free molecular alignment can be controlled due to the modulation of the molecular rotational state populations.


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