Tropospheric ozone from space: tracking pollution with the TOMS (Total Ozone Mapping Spectrometer) instrument

Author(s):  
A.M. Thompson ◽  
R.D. Hudson ◽  
A.D. Frolov ◽  
J.C. Witte ◽  
T.L. Kucsera
2003 ◽  
Vol 3 (1) ◽  
pp. 225-252 ◽  
Author(s):  
M. J. Newchurch ◽  
D. Sun ◽  
J. H. Kim ◽  
X. Liu

Abstract. Using TOMS total-ozone measurements over high-altitude cloud locations and nearby paired clear locations, we describe the Clear-Cloudy Pairs (CCP) method for deriving tropical tropospheric ozone. The high-altitude clouds are identified by measured 380 nm reflectivities greater than 80% and Temperature Humidity InfraRed (THIR) measured cloud-top pressures less than 200 hPa. To account for locations without high-altitude clouds, we apply a zonal sine fitting to the stratospheric ozone derived from available cloudy points, resulting in a wave-one amplitude of about 4 DU. THIR data is unavailable after November 1984, so we extend the CCP method by using a reflectivity threshold of 90% to identify high-altitude clouds and remove the influence of high-reflectivity-but-low-altitude clouds with a lowpass frequency filter. We correct ozone retrieval errors associated with clouds, and ozone retrieval errors due to sun glint and aerosols. Comparing CCP results with Southern Hemisphere ADditional OZonesondes (SHADOZ) tropospheric ozone indicates that CCP tropospheric ozone and ozonesonde measurements are highly consistent. The most significant difference between CCP and ozonesonde tropospheric ozone can be explained by the low Total Ozone Mapping Spectrometer (TOMS) retrieval efficiency of ozone in the lower troposphere.


2010 ◽  
Vol 10 (9) ◽  
pp. 20887-20920
Author(s):  
J. Kar ◽  
M. N. Deeter ◽  
J. Fishman ◽  
Z. Liu ◽  
A. Omar ◽  
...  

Abstract. The Bihar pollution pool is a large wintertime increase in pollutants over the eastern parts of the Indo Gangetic basin. We use improved carbon monoxide (CO) retrievals from the recent Measurements of Pollution in the Troposphere (MOPITT) version 4 data along with the aerosol data from the latest version 3 of the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) lidar instrument and the tropospheric ozone residual products from the Total Ozone Mapping Spectrometer (TOMS)/Solar Backscattered Ultraviolet (SBUV) and Ozone Monitoring Instrument (OMI)/Microwave Limb Sounder (MLS) database to characterize this pollution pool. The feature is seen primarily in the lower troposphere from about November to February with strong concomitant increase in CO, aerosol optical depth and tropospheric ozone columns. The height resolved aerosol data from CALIPSO confirm the trapping of the pollution pool at the lowest altitudes. The observations indicate that MOPITT can capture this low altitude phenomenon even in winter conditions as indicated by the averaging kernels.


2009 ◽  
Vol 9 (16) ◽  
pp. 6255-6271 ◽  
Author(s):  
A. Boynard ◽  
C. Clerbaux ◽  
P.-F. Coheur ◽  
D. Hurtmans ◽  
S. Turquety ◽  
...  

Abstract. In this paper, we present measurements of total and tropospheric ozone, retrieved from infrared radiance spectra recorded by the Infrared Atmospheric Sounding Interferometer (IASI), which was launched on board the MetOp-A European satellite in October 2006. We compare IASI total ozone columns to Global Ozone Monitoring Experiment-2 (GOME-2) observations and ground-based measurements from the Dobson and Brewer network for one full year of observations (2008). The IASI total ozone columns are shown to be in good agreement with both GOME-2 and ground-based data, with correlation coefficients of about 0.9 and 0.85, respectively. On average, IASI ozone retrievals exhibit a positive bias of about 9 DU (3.3%) compared to both GOME-2 and ground-based measurements. In addition to total ozone columns, the good spectral resolution of IASI enables the retrieval of tropospheric ozone concentrations. Comparisons of IASI tropospheric columns to 490 collocated ozone soundings available from several stations around the globe have been performed for the period of June 2007–August 2008. IASI tropospheric ozone columns compare well with sonde observations, with correlation coefficients of 0.95 and 0.77 for the [surface–6 km] and [surface–12 km] partial columns, respectively. IASI retrievals tend to overestimate the tropospheric ozone columns in comparison with ozonesonde measurements. Positive average biases of 0.15 DU (1.2%) and 3 DU (11%) are found for the [surface–6 km] and for the [surface–12 km] partial columns respectively.


1975 ◽  
Vol 14 (4) ◽  
Author(s):  
D. F. Heath ◽  
A. J. Krueger ◽  
H. A. Roeder ◽  
B. D. Henderson

2021 ◽  
Author(s):  
Jerry Ziemke ◽  
Natalya Kramarova ◽  
Dave Haffner ◽  
Pawan Bhartia

<p>The NASA TOMS V9 (TOMS-V9) total ozone retrieval algorithm is tested<br>for sensitvity to boundary-layer ozone and suitability to make daily<br>maps of tropospheric ozone residual (TOR).  Daily maps of TOR are<br>derived by differencing co-located MERRA-2 assimilated MLS<br>stratospheric column ozone (SCO) from total column ozone from the Aura<br>Ozone Monitoring Instrument (OMI).  The TOMS-V9 algorithm uses a few<br>discrete channels with an order of magnitude range in ozone<br>senstivity. We compare the TOR results from TOMS-V9 with results from<br>several hyper-spectral total ozone retrievals: GODFIT v4 (BIRA-IASB),<br>OMI-DOAS (KNMI), and total ozone from the SAO PROFOZ algorithm. We<br>compare all satellite-retrieved TOR with TOR derived from ozonesondes,<br>lidar, and the Goddard Modeling Initiative (GMI) model simulation.</p><p> </p><p> </p>


2016 ◽  
Vol 9 (10) ◽  
pp. 5037-5051 ◽  
Author(s):  
Klaus-Peter Heue ◽  
Melanie Coldewey-Egbers ◽  
Andy Delcloo ◽  
Christophe Lerot ◽  
Diego Loyola ◽  
...  

Abstract. In preparation of the TROPOMI/S5P launch in early 2017, a tropospheric ozone retrieval based on the convective cloud differential method was developed. For intensive tests we applied the algorithm to the total ozone columns and cloud data of the satellite instruments GOME, SCIAMACHY, OMI, GOME-2A and GOME-2B. Thereby a time series of 20 years (1995–2015) of tropospheric column ozone was generated. To have a consistent total ozone data set for all sensors, one common retrieval algorithm, namely GODFITv3, was applied and the L1 reflectances were also soft calibrated. The total ozone columns and the cloud data were input into the tropospheric ozone retrieval. However, the tropical tropospheric column ozone (TCO) for the individual instruments still showed small differences and, therefore, we harmonised the data set. For this purpose, a multilinear function was fitted to the averaged difference between SCIAMACHY's TCO and those from the other sensors. The original TCO was corrected by the fitted offset. GOME-2B data were corrected relative to the harmonised data from OMI and GOME-2A. The harmonisation leads to a better agreement between the different instruments. Also, a direct comparison of the TCO in the overlapping periods proves that GOME-2A agrees much better with SCIAMACHY after the harmonisation. The improvements for OMI were small. Based on the harmonised observations, we created a merged data product, containing the TCO from July 1995 to December 2015. A first application of this 20-year record is a trend analysis. The tropical trend is 0.7 ± 0.12 DU decade−1. Regionally the trends reach up to 1.8 DU decade−1 like on the African Atlantic coast, while over the western Pacific the tropospheric ozone declined over the last 20 years with up to 0.8 DU decade−1. The tropical tropospheric data record will be extended in the future with the TROPOMI/S5P data, where the TCO is part of the operational products.


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