GridFTP based real-time data movement architecture for x-ray photon correlation spectroscopy at the Advanced Photon Source

2012 ◽  
Author(s):  
S. Narayanan ◽  
T. J. Madden ◽  
A. R. Sandy ◽  
Raj Kettimuthu ◽  
Michael Link
Keyword(s):  
Real Time ◽  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
Time Data ◽  
Photon Correlation ◽  
Data Movement ◽  
X Ray ◽  
Real Time Data ◽  
Photon Source

scholarly journals Distributed X-ray photon correlation spectroscopy data reduction using Hadoop MapReduce

2018 ◽  
Vol 25 (4) ◽  
pp. 1135-1143 ◽  
Author(s):  
Faisal Khan ◽  
Suresh Narayanan ◽  
Roger Sersted ◽  
Nicholas Schwarz ◽  
Alec Sandy
Keyword(s):  
Real Time ◽  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
Frame Rate ◽  
Computational Techniques ◽  
Complex Materials ◽  
Photon Correlation ◽  
X Ray ◽  
Wide Range ◽  
Recent Developments

Multi-speckle X-ray photon correlation spectroscopy (XPCS) is a powerful technique for characterizing the dynamic nature of complex materials over a range of time scales. XPCS has been successfully applied to study a wide range of systems. Recent developments in higher-frame-rate detectors, while aiding in the study of faster dynamical processes, creates large amounts of data that require parallel computational techniques to process in near real-time. Here, an implementation of the multi-tau and two-time autocorrelation algorithms using the Hadoop MapReduce framework for distributed computing is presented. The system scales well with regard to the increase in the data size, and has been serving the users of beamline 8-ID-I at the Advanced Photon Source for near real-time autocorrelations for the past five years.

Nanoparticle suspensions studied by x-ray photon correlation spectroscopy

2007 ◽  
Vol 1027 ◽  
Author(s):  
Xinhui Lu ◽  
Simon G. J. Mochrie ◽  
S. Narayanan ◽  
Alec R. Sandy ◽  
Michael Sprung
Keyword(s):  
Silica Nanoparticles ◽  
Binary Mixtures ◽  
Photon Correlation Spectroscopy ◽  
National Laboratory ◽  
Argonne National Laboratory ◽  
Correlation Spectroscopy ◽  
Photon Correlation ◽  
X Ray ◽  
Nanoparticle Suspensions ◽  
Photon Source

AbstractMultispeckle x-ray photon correlation spectroscopy measurements, carried out at beamline 8-ID at the Advanced Photon Source at Argonne National Laboratory, of opaque suspensions of silica nanoparticles in water and lutidine-water binary mixtures are presented.

scholarly journals 20 µs-resolved high-throughput X-ray photon correlation spectroscopy on a 500k pixel detector enabled by data-management workflow

2021 ◽  
Vol 28 (1) ◽  
pp. 259-265
Author(s):  
Qingteng Zhang ◽  
Eric M. Dufresne ◽  
Yasukazu Nakaye ◽  
Pete R. Jemian ◽  
Takuto Sakumura ◽  
...  
Keyword(s):  
Data Management ◽  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
Frame Rate ◽  
Pixel Detector ◽  
Photon Correlation ◽  
X Ray ◽  
Area Detector ◽  
Workflow System ◽  
Photon Source

The performance of the new 52 kHz frame rate Rigaku XSPA-500k detector was characterized on beamline 8-ID-I at the Advanced Photon Source at Argonne for X-ray photon correlation spectroscopy (XPCS) applications. Due to the large data flow produced by this detector (0.2 PB of data per 24 h of continuous operation), a workflow system was deployed that uses the Advanced Photon Source data-management (DM) system and high-performance software to rapidly reduce area-detector data to multi-tau and two-time correlation functions in near real time, providing human-in-the-loop feedback to experimenters. The utility and performance of the workflow system are demonstrated via its application to a variety of small-angle XPCS measurements acquired from different detectors in different XPCS measurement modalities. The XSPA-500k detector, the software and the DM workflow system allow for the efficient acquisition and reduction of up to ∼109 area-detector data frames per day, facilitating the application of XPCS to measuring samples with weak scattering and fast dynamics.

Creating coherent x-rays and putting them to use: X-ray photon correlation spectroscopy at beamline 8-1d at the advanced photon source

2000 ◽  
Vol 13 (2) ◽  
pp. 28-37 ◽  
Author(s):  
L. B. Lurio ◽  
D. Lumma ◽  
M. A. Borthwick ◽  
P. Falus ◽  
S. G. J. Mochrie ◽  
...  
Keyword(s):  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
X Rays ◽  
Photon Correlation ◽  
X Ray ◽  
Photon Source

scholarly journals From Femtoseconds to Hours–Measuring Dynamics over 18 Orders of Magnitude with Coherent X-rays

2021 ◽  
Vol 11 (13) ◽  
pp. 6179
Author(s):  
Felix Lehmkühler ◽  
Wojciech Roseker ◽  
Gerhard Grübel
Keyword(s):  
Time Scales ◽  
Free Electron Laser ◽  
Photon Correlation Spectroscopy ◽  
Signal To Noise Ratio ◽  
Coherent Scattering ◽  
Correlation Spectroscopy ◽  
X Rays ◽  
Photon Correlation ◽  
X Ray ◽  
Scattering Technique

X-ray photon correlation spectroscopy (XPCS) enables the study of sample dynamics between micrometer and atomic length scales. As a coherent scattering technique, it benefits from the increased brilliance of the next-generation synchrotron radiation and Free-Electron Laser (FEL) sources. In this article, we will introduce the XPCS concepts and review the latest developments of XPCS with special attention on the extension of accessible time scales to sub-μs and the application of XPCS at FELs. Furthermore, we will discuss future opportunities of XPCS and the related technique X-ray speckle visibility spectroscopy (XSVS) at new X-ray sources. Due to its particular signal-to-noise ratio, the time scales accessible by XPCS scale with the square of the coherent flux, allowing to dramatically extend its applications. This will soon enable studies over more than 18 orders of magnitude in time by XPCS and XSVS.

scholarly journals Grain Growth and Coarsening Dynamics in a Compositionally Asymmetric Block Copolymer Revealed by X-ray Photon Correlation Spectroscopy

2020 ◽  
Vol 53 (19) ◽  
pp. 8233-8243
Author(s):  
Ronald M. Lewis ◽  
Grayson L. Jackson ◽  
Michael J. Maher ◽  
Kyungtae Kim ◽  
Suresh Narayanan ◽  
...  
Keyword(s):  
Block Copolymer ◽  
Grain Growth ◽  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
Photon Correlation ◽  
X Ray ◽  
Coarsening Dynamics

scholarly journals Atomic Migration Studies with X-Ray Photon Correlation Spectroscopy

2014 ◽  
Vol 2 ◽  
pp. 73-94 ◽  
Author(s):  
Markus Stana ◽  
Manuel Ross ◽  
Bogdan Sepiol
Keyword(s):  
Low Temperatures ◽  
Short Range ◽  
Short Range Order ◽  
Photon Correlation Spectroscopy ◽  
Condensed Matter ◽  
Correlation Spectroscopy ◽  
Atomic Scale ◽  
Photon Correlation ◽  
X Ray ◽  
Amorphous Systems

The new technique of atomic-scale X-ray Photon Correlation Spectroscopy (aXPCS) makesuse of a coherent X-ray beam to study the dynamics of various processes in condensed matter systems.Particularly atomistic migration mechanisms are still far from being understood in most of intermetallicalloys and in amorphous systems. Special emphasis must be given to the opportunity to measureatomistic diffusion at relatively low temperatures where such measurements were far out of reach withpreviously established methods. The importance of short-range order is demonstrated on the basis ofMonte Carlo simulations.

scholarly journals Demonstration of 3D Photon Correlation Spectroscopy in the hard X-ray regime

2021 ◽  
Author(s):  
Wonhyuk Jo ◽  
Rustam Rysov ◽  
FABIAN WESTERMEIER ◽  
Michael Walther ◽  
Leonard Mueller ◽  
...  
Keyword(s):  
Photon Correlation Spectroscopy ◽  
Correlation Spectroscopy ◽  
Photon Correlation ◽  
X Ray
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