Time-resolved experimental and computational study of two-photon laser-induced fluorescence in a hydrogen plasma

2000 ◽  
Vol 61 (4) ◽  
pp. 4402-4409 ◽  
Author(s):  
H. W. P. van der Heijden ◽  
M. G. H. Boogaarts ◽  
S. Mazouffre ◽  
J. A. M. van der Mullen ◽  
D. C. Schram
Keyword(s):  
Computational Study ◽  
Hydrogen Plasma ◽  
Laser Induced Fluorescence ◽  
Time Resolved ◽  
Two Photon

Imaging hydrogen flames by two-photon, laser-induced fluorescence

1991 ◽  
Author(s):  
R. MILES ◽  
W. LEMPERT ◽  
V. KUMAR ◽  
G. DISKIN
Keyword(s):  
Laser Induced Fluorescence ◽  
Two Photon

scholarly journals Progresses on the Use of Two-Photon Absorption Laser Induced Fluorescence (TALIF) Diagnostics for Measuring Absolute Atomic Densities in Plasmas and Flames

Plasma ◽  
2021 ◽  
Vol 4 (1) ◽  
pp. 145-171
Author(s):  
Kristaq Gazeli ◽  
Guillaume Lombardi ◽  
Xavier Aubert ◽  
Corinne Y. Duluard ◽  
Swaminathan Prasanna ◽  
...  
Keyword(s):  
Optical Transition ◽  
Thin Film Deposition ◽  
Laser Induced Fluorescence ◽  
Film Deposition ◽  
Stimulated Emission ◽  
Photon Absorption ◽  
Collisional Quenching ◽  
Two Photon Absorption ◽  
Two Photon ◽  
Wide Range

Recent developments in plasma science and technology have opened new areas of research both for fundamental purposes (e.g., description of key physical phenomena involved in laboratory plasmas) and novel applications (material synthesis, microelectronics, thin film deposition, biomedicine, environment, flow control, to name a few). With the increasing availability of advanced optical diagnostics (fast framing imaging, gas flow visualization, emission/absorption spectroscopy, etc.), a better understanding of the physicochemical processes taking place in different electrical discharges has been achieved. In this direction, the implementation of fast (ns) and ultrafast (ps and fs) lasers has been essential for the precise determination of the electron density and temperature, the axial and radial gradients of electric fields, the gas temperature, and the absolute density of ground-state reactive atoms and molecules in non-equilibrium plasmas. For those species, the use of laser-based spectroscopy has led to their in situ quantification with high temporal and spatial resolution, with excellent sensitivity. The present review is dedicated to the advances of two-photon absorption laser induced fluorescence (TALIF) techniques for the measurement of reactive species densities (particularly atoms such as N, H and O) in a wide range of pressures in plasmas and flames. The requirements for the appropriate implementation of TALIF techniques as well as their fundamental principles are presented based on representative published works. The limitations on the density determination imposed by different factors are also discussed. These may refer to the increasing pressure of the probed medium (leading to a significant collisional quenching of excited states), and other issues originating in the high instantaneous power density of the lasers used (such as photodissociation, amplified stimulated emission, and photoionization, resulting to the saturation of the optical transition of interest).

Measurements of the Collisionally Quenched Lifetime of CO in Hydrocarbon Flames

1994 ◽  
Vol 48 (9) ◽  
pp. 1118-1124 ◽  
Author(s):  
Sara Agrup ◽  
Marcus Aldén
Keyword(s):  
Laser Induced Fluorescence ◽  
Polyaromatic Hydrocarbon ◽  
Time Decay ◽  
Collisional Quenching ◽  
Time Resolved ◽  
Hydrocarbon Flames ◽  
Effective Lifetime ◽  
Ethylene Flame ◽  
Oxygen Flame ◽  
Different Parts

Time-resolved laser-induced fluorescence (LIF) from CO molecules in hydrocarbon flames was studied. Collisional quenching constants were evaluated on the basis of the exponential decays. Effective lifetime in a methane/oxygen flame was observed to vary between 250 and 400 ps depending on the position within the flame, and from 400 to 600 ps in the non-sooty parts of an ethylene/air flame. Fluorescence, constituting simultaneous spatially and temporally resolved decays, was also registered from various sections along a laser beam that probed different parts of the flame. Spectral recordings revealed not only the expected CO peaks but also, in the ethylene flame, laser-induced emission from C2 Swan bands and from polyaromatic hydrocarbon (PAH) emission that affected the fluorescence time decay in the sooty part of the flame.

Time-resolved two-photon photoemission at metal-dielectric interfaces

2005 ◽  
Vol 45 (1-2) ◽  
pp. 181-194 ◽  
Author(s):  
Wolfram Berthold ◽  
Ulrich Höfer
Keyword(s):  
Time Resolved ◽  
Two Photon ◽  
Dielectric Interfaces
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