scholarly journals Revision of forensics-relevant nuclear data in Sb127 β decay

2019 ◽  
Vol 99 (3) ◽  
Author(s):  
B. Bucher ◽  
M. S. Snow ◽  
E. S. Cárdenas ◽  
K. P. Carney ◽  
M. R. Finck ◽  
...  
Keyword(s):  
2020 ◽  
Vol 27 ◽  
pp. 189
Author(s):  
Zinovia Eleme ◽  
... Et al.

The condition for the safe design and operation of fast neutron reactors and energy boosters (Generation-IV reactors, ADS systems [1]) is the accuracy of nuclear data. The 241Am isotope (T1/2 = 433 years) is highly present in nuclear waste, accounting for about 1.8% of the actinide mass in PWR UOx nuclear reactors’ waste [2]. In addition, the 241Am isotope is further produced by the β decay of the 241Pu isotope (T1/2 = 14.3 years). Given the high production rate of 241Am isotope, its incineration with concurrent energy production is considered to be of utmost importance for the design and implementation of the recycling of existing nuclear waste. Sensitivity studies of the proposed systems for energy production showed that high-precision measurements of the cross section of the 241Am(n,f) reaction are required. In the present work, the 241Am(n,f) reaction cross section was measured in the Second Experimental Area of the n_TOF facility at CERN, using an array of Micromegas detectors. For the measurement, six targets of 241Am with average activity of 17 MBq per sample were coupled with an equal number of detectors in a common chamber. Additionally two 235U and two 238U samples were coupled with Micromegas detectors utilizing the neutron flux determination. Within this work, an overview of the experimental set-up and the adopted data analysis technique is presented along with preliminary results.


2017 ◽  
Author(s):  
Karl-Ludwig Kratz ◽  
Khalil Farouqi ◽  
Bernd Pfeiffer

2020 ◽  
Vol 15 ◽  
pp. 210
Author(s):  
N. Costiris ◽  
E. Mavrommatis ◽  
K. A. Gernoth ◽  
J. W. Clark

Statistical modeling of nuclear data using artificial neural networks (ANNs) and, more re- cently, support vector machines (SVMs), is providing novel approaches to systematics that are complementary to phenomenological and semi-microscopic theories. We present a global model of β−-decay halflives of the class of nuclei that decay 100% by β− mode in their ground states. A fully-connected multilayered feed forward network has been trained using the Levenberg- Marquardt algorithm, Bayesian regularization, and cross-validation. The halflife estimates gen- erated by the model are discussed and compared with the available experimental data, with previous results obtained with neural networks, and with estimates coming from traditional global nuclear models. Predictions of the new neural-network model are given for nuclei far from stability, with particular attention to those involved in r-process nucleosynthesis. This study demonstrates that in the framework of the β−-decay problem considered here, global models based on ANNs can at least match the predictive performance of the best conventional global models rooted in nuclear theory. Accordingly, such statistical models can provide a valuable tool for further mapping of the nuclidic chart.


Author(s):  
I. P. Korenkov ◽  
A. I. Ermakov ◽  
A. B. Mayzik ◽  
T. N. Laschenova ◽  
V. N. Klochkov ◽  
...  

The aim of the study is to evaluate the volume activity of radioactive waste (RW) by surface and specific alpha contamination using portable gamma-spectrometry.Materials and methods. Methods of rapid assessment of the content of α-emitting radionuclides in solid waste of various morphologies using gamma-spectrometers based on germanium detectors are considered. Computational methods for determining the effectiveness of radionuclide registration are presented.Results. The possibility of using portable gamma-ray spectrometry to assess the surface and specific activity of various materials contaminated with α-emitters (232Th, 235U, 238U, 237Np, 239Pu, 240Pu and 241Am) is shown. The calculated values of the registration efficiency of low-energy gamma-emitters obtained by modeling the spatial-energy parameters of the detector are given.To simplify the solution of this problem, the calculation program used 20 standard templates of various geometries (rectangular, cylindrical, conical, spherical, etc.). The main sources of error in the survey of contaminated surfaces, largesized equipment and building structures were investigated.Conclusions. The possibilities of portable γ-spectrometry for estimating the volume of RW based on the surface density of contamination of materials with radionuclides of uranium and transuranic elements are investigated. When using γ-spectrometer with a high-purity germanium detector with a range of γ-quanta extended in the low-energy region, radionuclides such as 232Th, 235U,238U, 237Np, 241Am were determined by their own radiation or by the radiation of their daughter products.The “problem” element is plutonium, for rapid evaluation of which it is proposed, in accordance with the radionuclide vector methodology, to use 241Am, which accumulates during the β-decay of 241Pu.According to calculations, the most likely value of the activity ratio 239Pu/241Am for the object where the work was performed (scaling factor) varies in the range from 5.0 to 9.0.Based on the results of calculations and experimental studies, the parameters of the efficiency of registration of various α-emitting radionuclides by portable γ-spectrometers. It has been found that for germanium detectors with an absolute efficiency of registering a point source of 7÷15%, it is n×10–5÷n×10–4%.


Kerntechnik ◽  
2011 ◽  
Vol 76 (3) ◽  
pp. 174-178 ◽  
Author(s):  
M. Klein ◽  
L. Gallner ◽  
B. Krzykacz-Hausmann ◽  
A. Pautz ◽  
W. Zwermann
Keyword(s):  

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