Mass-Yield Curve of First-Chance Fission from Proton- and Deuteron-Induced Fission ofRa226

1971 ◽  
Vol 4 (3) ◽  
pp. 977-989 ◽  
Author(s):  
D. G. Perry ◽  
A. W. Fairhall
1978 ◽  
Vol 56 (10) ◽  
pp. 1340-1352 ◽  
Author(s):  
Masako Shima ◽  
H. G. Thode ◽  
R. H. Tomlinson

The relative cumulative yields of nine stable and long-lived isotopes of ruthenium and palladium (masses 101 to 110) produced in the thermal neutron fission of 233U and in the thermal and epicadmium neutron fission of 235U and 239Pu have been measured using a solid source mass spectrometer and isotope dilution techniques. Absolute yields of these isotopes for the thermal neutron fission of 233U, 235U, and 239Pu are obtained using normalization procedures. These yields provide the first experimentally determined yields of the palladium masses 105, 106, 107, 108, and 110.In the thermal fission of 233U and 235U the ruthenium isotope yields obtained are in general agreement with previously determined values, although discrepancies exist of the order of 10% at masses 103, 104, and 106 for thermal fission of 235U.A plot of the ruthenium and palladium isotope mass yields together with the previously determined yields for the cadmium and tin isotopes indicate a significant depression in the mass yield curve at masses 111 and 114 for 233U and 235U thermal fission, respectively. In the 235U epicadmium fission, yields at even mass numbers are relatively higher than those at odd numbers, resulting in a zigzag yield curve in the 101 to 110 mass region.


1957 ◽  
Vol 35 (8) ◽  
pp. 969-979 ◽  
Author(s):  
T. J. Kennett ◽  
H. G. Thode

The relative fission yields for mass chains ending in stable krypton and xenon isotopes have been measured for the fast neutron-induced fission of Th232. Isotope dilution techniques were used to determine the krypton/xenon ratio to assist in obtaining the absolute fission yields for these mass chains. The absolute yields were determined by the use of two methods, both giving results which were in excellent agreement. The fine structure observed for the Th232 mass–yield curve is compared with that of heavier fissile nuclides.


2018 ◽  
Vol 4 ◽  
pp. 26 ◽  
Author(s):  
Brieuc Voirin ◽  
Grégoire Kessedjian ◽  
Abdelaziz Chebboubi ◽  
Sylvain Julien-Laferrière ◽  
Olivier Serot

Studies on fission yields have a major impact on the characterization and the understanding of the fission process and are mandatory for reactor applications. Fission yield evaluation represents the synthesis of experimental and theoretical knowledge to perform the best estimation of mass, isotopic and isomeric yields. Today, the output of fission yield evaluation is available as a function of isotopic yields. Without the explicitness of evaluation covariance data, mass yield uncertainties are greater than those of isotopic yields. This is in contradiction with experimental knowledge where the abundance of mass yield measurements is dominant. These last years, different covariance matrices have been suggested but the experimental part of those are neglected. The collaboration between the LPSC Grenoble and the CEA Cadarache starts a new program in the field of the evaluation of fission products in addition to the current experimental program at Institut Laue-Langevin. The goal is to define a new methodology of evaluation based on statistical tests to define the different experimental sets in agreement, giving different solutions for different analysis choices. This study deals with the thermal neutron induced fission of 235U. The mix of data is non-unique and this topic will be discussed using the Shannon entropy criterion in the framework of the statistical methodology proposed.


1955 ◽  
Vol 33 (11) ◽  
pp. 693-706 ◽  
Author(s):  
J. A. Petruska ◽  
H. G. Thode ◽  
R. H. Tomlinson

Twenty-eight absolute fission yields totalling 78% of the heavy and 16% of the light fragments have been determined using the mass spectrometer and isotope dilution techniques. The precision of the values obtained is in most cases better than 2% and the absolute accuracy is estimated to be about 3%. Fine structure in the mass–yield curve is discussed in terms of structural preference and various chain branching mechanisms.


1962 ◽  
Vol 40 (8) ◽  
pp. 1017-1026 ◽  
Author(s):  
H. Farrar ◽  
H. R. Fickel ◽  
R. H. Tomlinson

A mass spectrometric study of the relative yields of the strontium, yttrium, zirconium, and molybdenum isotopes formed in the thermal neutron fission of U235 has made possible a detailed examination of structure of the light mass region of the mass–yield curve. The relative yields of this work have been normalized to 5.77% for Sr90, and when literature and extrapolated values are taken for the remaining chains, the fission yields total 100.8%.


1963 ◽  
Vol 25 (5) ◽  
pp. 465-472 ◽  
Author(s):  
R.H. Iyer ◽  
C.K. Mathews ◽  
N. Ravindran ◽  
K. Rengan ◽  
D.V. Singh ◽  
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