Theory of gas-phase time-resolved ultrafast electron diffraction

1997 ◽  
Vol 55 (1) ◽  
pp. 641-647 ◽  
Author(s):  
W. -K. Liu ◽  
S. H. Lin
Keyword(s):  
Electron Diffraction ◽  
Gas Phase ◽  
Ultrafast Electron Diffraction ◽  
Time Resolved ◽  
Phase Time

scholarly journals Femtosecond gas-phase mega-electron-volt ultrafast electron diffraction

2019 ◽  
Vol 6 (5) ◽  
pp. 054305 ◽  
Author(s):  
X. Shen ◽  
J. P. F. Nunes ◽  
J. Yang ◽  
R. K. Jobe ◽  
R. K. Li ◽  
...  
Keyword(s):  
Electron Diffraction ◽  
Gas Phase ◽  
Ultrafast Electron Diffraction ◽  
Electron Volt

Diffraction, crystallography and microscopy beyond three dimensions: structural dynamics in space and time

2004 ◽  
Vol 363 (1827) ◽  
pp. 315-329 ◽  
Author(s):  
Ahmed H. Zewail
Keyword(s):  
Electron Microscopy ◽  
Electron Diffraction ◽  
Gas Phase ◽  
Structural Dynamics ◽  
Research Area ◽  
Three Dimensions ◽  
Ultrafast Electron Diffraction ◽  
Major Research ◽  
Condensed Media ◽  
Recent Developments

In this article we highlight recent developments of ultrafast electron diffraction and crystallography at Caltech. These developments have made it possible to resolve transient structures, both spatially (0.01 Å) and temporally (picosecond and now femtosecond), in the gas phase and condensed media—surfaces, interfaces, and crystals—with wide-ranging applications. With the extension to ultrafast electron microscopy, discussed here and elsewhere, we present an overview of one major research area at our centre, the Laboratory for Molecular Sciences.

Relativistic ultrafast electron diffraction from molecules in the gas phase (Conference Presentation)

2016 ◽  
Author(s):  
Jie Yang ◽  
Markus Guehr ◽  
Theodore Vecchione ◽  
Matthew S. Robinson ◽  
Renkai Li ◽  
...  
Keyword(s):  
Electron Diffraction ◽  
Gas Phase ◽  
Ultrafast Electron Diffraction

scholarly journals A compact streak camera for 150 fs time resolved measurement of bright pulses in ultrafast electron diffraction

2010 ◽  
Vol 81 (10) ◽  
pp. 105103 ◽  
Author(s):  
G. H. Kassier ◽  
K. Haupt ◽  
N. Erasmus ◽  
E. G. Rohwer ◽  
H. M. von Bergmann ◽  
...  
Keyword(s):  
Electron Diffraction ◽  
Streak Camera ◽  
Ultrafast Electron Diffraction ◽  
Time Resolved

scholarly journals Quantum state tomography of molecules by ultrafast diffraction

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Ming Zhang ◽  
Shuqiao Zhang ◽  
Yanwei Xiong ◽  
Hankai Zhang ◽  
Anatoly A. Ischenko ◽  
...  
Keyword(s):  
Electron Diffraction ◽  
Quantum State ◽  
Degrees Of Freedom ◽  
Molecular Structures ◽  
Electron Diffraction Data ◽  
Ultrafast Electron Diffraction ◽  
Time Resolved ◽  
Quantum State Tomography ◽  
New Variant ◽  
State Tomography

AbstractUltrafast electron diffraction and time-resolved serial crystallography are the basis of the ongoing revolution in capturing at the atomic level of detail the structural dynamics of molecules. However, most experiments capture only the probability density of the nuclear wavepackets to determine the time-dependent molecular structures, while the full quantum state has not been accessed. Here, we introduce a framework for the preparation and ultrafast coherent diffraction from rotational wave packets of molecules, and we establish a new variant of quantum state tomography for ultrafast electron diffraction to characterize the molecular quantum states. The ability to reconstruct the density matrix, which encodes the amplitude and phase of the wavepacket, for molecules of arbitrary degrees of freedom, will enable the reconstruction of a quantum molecular movie from experimental x-ray or electron diffraction data.

Ultrafast Imaging of Molecules with Electron Diffraction

2021 ◽  
Vol 73 (1) ◽  
Author(s):  
Martin Centurion ◽  
Thomas J.A. Wolf ◽  
Jie Yang
Keyword(s):  
Electron Diffraction ◽  
Gas Phase ◽  
Structural Dynamics ◽  
Mechanical Energy ◽  
Annual Review ◽  
Publication Date ◽  
Ultrafast Electron Diffraction ◽  
Ultrafast Imaging ◽  
Ideal Tool ◽  
Nuclear Geometry

Photoexcited molecules convert light into chemical and mechanical energy through changes in electronic and nuclear structure that take place on femtosecond timescales. Gas phase ultrafast electron diffraction (GUED) is an ideal tool to probe the nuclear geometry evolution of the molecules and complements spectroscopic methods that are mostly sensitive to the electronic state. GUED is a passive probing tool that does not alter the molecular properties during the probing process and is sensitive to the spatial distribution of charge in the molecule, including both electrons and nuclei. Improvements in temporal resolution have enabled GUED to capture coherent nuclear motions in molecules in the excited and ground electronic states with femtosecond and subangstrom resolution. Here we present the basic theory of GUED and explain what information is encoded in the diffraction signal, review how GUED has been used to observe coherent structural dynamics in recent experiments, and discuss the advantages and limitations of the method. Expected final online publication date for the Annual Review of Physical Chemistry, Volume 73 is April 2022. Please see http://www.annualreviews.org/page/journal/pubdates for revised estimates.

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