Measurements of moisture in smoldering smoke and implications for fog

2006 ◽  
Vol 15 (4) ◽  
pp. 517 ◽  
Author(s):  
Gary L. Achtemeier

Smoke from wildland burning in association with fog has been implicated as a visibility hazard over roadways in the southern United States. A project began in 2002 to determine whether moisture released during the smoldering phases of southern prescribed burns could contribute to fog formation. Temperature and relative humidity measurements were taken from 27 smoldering ‘smokes’ during 2002 and 2003. These data were converted to a measure of the mass of water vapor present to the mass of dry air containing the vapor (smoke mixing ratio). Some smokes were dry with almost no moisture beyond ambient. Other smokes were moist with moisture excesses as large as 39 g kg–1. Calculations show that ground-level smoke moisture excesses have no impact on ambient relative humidity during the day. However, the impact at night can be large enough to increase the ambient relative humidity to 100%. Therefore smoke moisture may be a contributing factor to the location and timing of fog formation.

2016 ◽  
Vol 16 (2) ◽  
pp. 927-932 ◽  
Author(s):  
M. L. López ◽  
E. E. Ávila

Abstract. This study reports measurements of deposition-mode ice-nucleating particle (INP) concentrations at ground level during the period July–December 2014 in Córdoba, Argentina. Ambient air was sampled into a cloud chamber where the INP concentration was measured at a temperature of −25 °C and a 15 % supersaturation over ice. Measurements were performed on days with different thermodynamic conditions, including rainy days. The effect of the relative humidity at ground level (RHamb) on the INP concentration was analyzed. The number of INPs activated varied from 1 L−1 at RHamb of 25 % to 30 L−1 at RHamb of 90 %. In general, a linear trend between the INP concentration and the RHamb was found, suggesting that this variability must be related to the effectiveness of the aerosols acting as INPs. From the backward trajectories analysis, it was found that the link between INP concentration and RHamb is independent of the origin of the air masses. The role of biological INPs and nucleation occurring in pores and cavities was discussed as a possible mechanism to explain the increase of the INP concentration during high ambient relative humidity events. This work provides valuable measurements of deposition-mode INP concentrations from the Southern Hemisphere where INP data are sparse so far.


1931 ◽  
Vol 5 (6) ◽  
pp. 625-635
Author(s):  
D. C. Rose

The Gerdian type of atmospheric ionization measuring apparatus was attached to a cabin aeroplane so that the state of ionization of the atmosphere could be studied. The limitations of the apparatus for aeroplane use are discussed. Measurements were taken from ground level to heights of 15000 ft. The results are plotted in number of ions per cc. (separate curves for positive and negative) at different altitudes.The results indicate that at the cloud level there is an abnormal excess of small positive ions and a minimum in the excess of positive ions over negative ions from 4000–6000 ft. higher. This does not include large ions such as charged water drops or dust particles. The observations were taken in regions free from clouds, the cloud level being determined by observation on clouds in the sky, and by relative humidity measurements taken at the same time.


2008 ◽  
Vol 47 (5) ◽  
pp. 1287-1296 ◽  
Author(s):  
Gary L. Achtemeier

Abstract Smoke from wildland burning in association with fog has been implicated as a visibility hazard over roadways in the United States. Visibilities at accident sites have been estimated in the range from 1 to 3 m (extinction coefficients between 1000 and 4000). Temperature and relative humidity measurements were taken from 29 “smokes” during 2002 and 2003. These data were converted to a measure of the mass of water vapor present to the mass of dry air containing the vapor (smoke mixing ratio). Smoke temperatures were processed through a simple radiation model before smokes were mixed with ambient air with temperature and moisture observed during the early morning on the days following the burns. Calculations show supersaturations implying liquid water contents (LWC) up to 17 times as large as LWC found in natural fog. Simple models combining fog droplet number density, droplet size, and LWC show that the supersaturation LWC of smokes is capable of reducing visibility to the ranges observed.


2015 ◽  
Vol 15 (12) ◽  
pp. 16697-16714
Author(s):  
M. L. López ◽  
E. E. Ávila

Abstract. This study reports measurements of deposition ice nuclei (IN) concentration at ground level during the period July–December 2014 in Córdoba, Argentina. The measurements were carried out at temperature of −25 °C and at 15 % supersaturation over ice. They were performed on days with different thermodynamic conditions, including rainy days. The effect of the relative humidity at ground level (RHamb) on the IN concentration was analyzed. The number of IN activated varied from 1 −1 at RHamb of 25 % to 30 L−1 at RHamb of 90 %. In general, a linear trend between the IN concentration and the RHamb was found, suggesting that this variable must be related to the ability of the aerosols acting as IN. These results are consistent with previous results. From the backward trajectories analysis, it was found that the link between IN concentration and RHamb is independent of the origin of the air masses. The role of nucleation occurring in pores and cavities was discussed as possible mechanism to explain the increase on the IN concentration during high ambient relative humidity events.


2007 ◽  
Vol 135 (10) ◽  
pp. 3405-3428 ◽  
Author(s):  
Greg M. McFarquhar ◽  
Michael S. Timlin ◽  
Robert M. Rauber ◽  
Brian F. Jewett ◽  
Joseph A. Grim ◽  
...  

Abstract During the Bow Echo and Mesoscale Convective Vortex Experiment, the NOAA P-3 research aircraft executed 17 spiral descents to the rear of convective lines to document the vertical variability of hydrometeors above, within, and below the stratiform melting layer. Ten spirals were behind lines that exhibited bowing at some stage in their evolution. Although quick descents on some spirals forced sampling of different particle zones, clear trends with respect to temperature were seen. For 16 spirals, the ambient relative humidity with respect to ice was in the range of 100% ± 4% at temperatures between −10°C and the melting layer, but exhibited steady decreases below the melting layer to an average relative humidity with respect to water of 77% ± 15% at 9°C. In contrast, one spiral conducted on 29 June 2003 directly behind a developing bow echo had a relative humidity with respect to ice averaging 85% at heights above the 0°C level and relative humidity with respect to ice further decreased below the 0°C level to a minimum relative humidity with respect to water of 48% at 9°C. Vertical profiles of particle shapes, size distributions (SDs), total mass contents (TMC), number concentrations, and parameters of gamma distributions fit to SDs were computed using optical array probe data in conjunction with measurements of radar reflectivity from the P-3 X-band tail radar. For spirals with humidity at or near saturation above the melting layer, melting particles occurred through about 300 m of cloud depth between 0° and 2° or 3°C. Above the melting layer, number concentrations, dominated by smaller crystals, decreased at 19% ± 10% °C−1, faster than the 10% ± 7% °C−1 decrease of TMC dominated by larger particles. Increases in the numbers of crystals with a maximum dimension <2 mm (N<2) and in the slope parameter with temperature also occurred. To the extent that in-cloud heterogeneity did not complicate observed trends, these trends suggest aggregation dominated the evolution of SDs. Observations on 29 June differ from other days and are explained by the unique position and timing of the spiral in subsaturated air behind a developing bow. On 29 June the presence of an isothermal layer at 2.5°C suggested that sublimative cooling delayed the onset of melting. Ice at 7°C showed that melting particles were present through 500 m of cloud depth. A slight decrease in N<2, but no decrease in the slope parameter, with temperature suggested that sublimation modified the impact of aggregation. Sublimative cooling would only have been significant at the location of the 29 June spiral. For other spirals, evaporative cooling below the melting layer in subsaturated regions was the most important diabatic processes in the stratiform regions at the time of the observations.


2016 ◽  
Vol 16 (24) ◽  
pp. 15451-15460 ◽  
Author(s):  
Yang Hua ◽  
Shuxiao Wang ◽  
Jiandong Wang ◽  
Jingkun Jiang ◽  
Tianshu Zhang ◽  
...  

Abstract. During the APEC (Asia-Pacific Economic Cooperation) Economic Leaders' 2014 Summit in Beijing, strict regional air emission controls were implemented, providing a unique opportunity to investigate the transport and formation mechanism of fine particulate matter (PM2.5). This study explores the use of vertical observation methods to investigate the influence of regional transport on PM2.5 pollution in Beijing before and during the APEC Summit. Vertical profiles of extinction coefficient, wind, temperature and relative humidity were monitored at a rural site on the border of Beijing and Hebei Province. Three PM2.5 pollution episodes were analyzed. In episode 1 (27 October to 1 November), regional transport accompanied by the accumulation of pollutants under unfavorable meteorological conditions led to the pollution. In episode 2 (2–5 November), pollutants left from episode 1 were retained in the boundary layer of the region for 2 days and then settled down to the surface, leading to an explosive increase of PM2.5. The regional transport of aged aerosols played a crucial role in the heavy PM2.5 pollution. In episode 3 (6–11 November), emissions from large point sources had been controlled for several days while primary emissions from diesel vehicles might have led to the pollution. It is found that ground-level observation of meteorological conditions and air quality could not fully explain the pollution process, while vertical parameters (aerosol optical properties, winds, relative humidity and temperature) improved the understanding of regional transport influence on heavy pollution processes. Future studies may consider including vertical observations to aid investigation of pollutant transport, especially during episodic events of rapidly increasing concentrations.


2007 ◽  
Vol 20 (22) ◽  
pp. 5629-5641 ◽  
Author(s):  
Thomas M. Seidel ◽  
Andrea N. Grant ◽  
Alexander A. P. Pszenny ◽  
Daniel J. Allman

Abstract Meteorological conditions have been recorded at the summit of Mount Washington, New Hampshire, (44°16′N, 71°18′W, 1914 m ASL) since November 1932. Use of consistent instrumentation allows analysis of humidity measurements as calculated from error-checked dry bulb temperature, wet bulb temperature, and pressure during the period 1935–2004. This paper presents seasonally and annually averaged dewpoint temperature, mixing ratio, and relative humidity means and trends, including clear-air and fog subsets and, beginning in 1939, day and night subsets. The majority of linear trends are negative over the full study period, although these decreases are not constant, with relatively large (small) values in the mid-1950s (late 1970s). Annual mean dewpoint (water vapor mixing ratio) over the 70-yr period has decreased by 0.06°C decade−1 (0.01 g kg−1 decade−1). During this period the annual frequency of fog increased by 0.5% decade−1. Dewpoint and mixing ratio trends, both generally decreasing, differ by season; they are smallest in spring and greatest in fall. Relative humidity has decreased most in winter. The clear-air subset shows significant decreases in both dewpoint and mixing ratio for all seasons except spring.


2013 ◽  
Vol 6 (2) ◽  
pp. 387-396 ◽  
Author(s):  
D. Sakaizawa ◽  
S. Kawakami ◽  
M. Nakajima ◽  
T. Tanaka ◽  
I. Morino ◽  
...  

Abstract. Simultaneous measurements of the partial column-averaged dry air mixing ratio of CO2 (XCO2) and target range were demonstrated using airborne amplitude-modulated 1.57 μm differential laser absorption spectrometer (LAS). The LAS system is useful for discriminating between ground and cloud return signals and has a demonstrated ability to suppress the impact of integrated aerosol signals on atmospheric CO2 measurements. A high correlation coefficient (R) of 0.987 between XCO2 observed by LAS and XCO2 calculated from in situ measurements was obtained. The averaged difference in XCO2 obtained from LAS and validation data was within 1.5 ppm for all spiral measurements. An interesting vertical profile was observed for both XCO2LAS and XCO2val, in which lower altitude CO2 decreases compared to higher altitude CO2 attributed to the photosynthesis over grassland in the summer. In the case of an urban area where there are boundary-layer enhanced CO2 and aerosol in the winter, the difference of XCO2LAS to XCO2val is a negative bias of 1.5 ppm, and XCO2LAS is in agreement with XCO2val within the measurement precision of 2.4 ppm (1 SD).


2012 ◽  
Vol 5 (4) ◽  
pp. 4851-4880
Author(s):  
D. Sakaizawa ◽  
S. Kawakami ◽  
M. Nakajima ◽  
T. Tanaka ◽  
I. Morino ◽  
...  

Abstract. Simultaneous measurements of the partial column-averaged dry air mixing ratio of CO2 (q) and target range were demonstrated using airborne amplitude-modulated 1.57 μm differential laser absorption spectrometry (LAS). The LAS system is useful for discriminating between ground and cloud return signals and has a demonstrated ability to suppress the impact of integrated aerosol signals on differential absorption optical depth (Δτ) measurements. A high correlation coefficient (R) of 0.99 between Δτ observed by LAS and Δτ calculated from in-situ measurements of CO2 was obtained. The averaged difference in q obtained from LAS (qLAS) and validation data (qval) was within 1.5 ppm for all spiral measurements. A significant profile was observed for both qLAS and qval, in which lower altitude CO2 decreases compared to higher altitude CO2 attributed to the photosynthesis over grassland in the summer. In the case of an urban area where CO2 and aerosol are highly distributed in the lower atmosphere in the winter, the difference of qLAS to qval is −1.5 ppm, and evaluated qLAS is in agreement with qval within the measurement precision of 2.4 ppm (1σ).


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