Novel optoelectronic technique for direct tracking of ultrafast triplet excitons in polymeric semiconductor

2021 ◽  
Vol 8 (3) ◽  
pp. 031415
Author(s):  
Gangadhar Banappanavar ◽  
Sumukh Vaidya ◽  
Urvashi Bothra ◽  
Lohitha R. Hegde ◽  
Kamendra P. Sharma ◽  
...  
Keyword(s):  
Polymeric Semiconductor ◽  
Direct Tracking ◽  
Triplet Excitons

TRIPLET EXCITONS IN MEM(TCNQ)2

1983 ◽  
Vol 44 (C3) ◽  
pp. C3-1383-C3-1385
Author(s):  
S. Oostra ◽  
P. De Lange ◽  
R. J.J. Visser
Keyword(s):  
Triplet Excitons

Enhanced efficacy of defect passivation and charge extraction for efficient perovskite photovoltaics with a small open circuit voltage loss

2019 ◽  
Vol 7 (15) ◽  
pp. 9025-9033 ◽  
Author(s):  
Jin-Feng Liao ◽  
Wu-Qiang Wu ◽  
Jun-Xing Zhong ◽  
Yong Jiang ◽  
Lianzhou Wang ◽  
...  
Keyword(s):  
Grain Boundary ◽  
Power Conversion Efficiency ◽  
Conversion Efficiency ◽  
Open Circuit Voltage ◽  
Power Conversion ◽  
Charge Recombination ◽  
Open Circuit ◽  
Polymeric Semiconductor ◽  
Voltage Loss ◽  
Defect Passivation

A multifunctional 2D polymeric semiconductor was incorporated to provide surprisingly robust efficacy in grain boundary functionalization and defect passivation of perovskite, which suppresses charge recombination and thus affording an illustrious photovoltage of 1.16 V and power conversion efficiency of 21.1%.

A Fully Coplanar D‐A Polymeric Semiconductor with Promoted Charge Separation Kinetics for Photochemistry

2021 ◽  
Author(s):  
Zhi-An Lan ◽  
Meng Wu ◽  
Zhongpu Fang ◽  
Xu Chi ◽  
Xiong Chen ◽  
...  
Keyword(s):  
Charge Separation ◽  
Polymeric Semiconductor ◽  
Separation Kinetics

Why Triage the Materials with Low Luminescence Quantum Efficiency: The Use of 35Cbz4BzCN as a Universal Host for Organic Light Emitting Diode through Effective Triplet Energy Transfer

2021 ◽  
Author(s):  
Yi-Mei Huang ◽  
Tse-Ying Chen ◽  
Deng-Gao Chen ◽  
Hsuan-Chi Liang ◽  
Cheng-Ham Wu ◽  
...  
Keyword(s):  
Light Emitting Diode ◽  
Delayed Fluorescence ◽  
Triplet Energy ◽  
Thermally Activated Delayed Fluorescence ◽  
Light Emitting ◽  
Organic Light Emitting Diode ◽  
Thermally Activated ◽  
Triplet Energy Transfer ◽  
Triplet Lifetime ◽  
Triplet Excitons

35Cbz4BzCN, a novel universal host with long triplet lifetime, has been developed. The triplet excitons in 35Cbz4BzCN can be effectively harvested by phosphorescence and thermally activated delayed fluorescence emitters. In...

scholarly journals Broccoli Fluorets: Split Aptamers as a User-Friendly Fluorescent Toolkit for Dynamic RNA Nanotechnology

Molecules ◽  
2018 ◽  
Vol 23 (12) ◽  
pp. 3178 ◽  
Author(s):  
Morgan Chandler ◽  
Tatiana Lyalina ◽  
Justin Halman ◽  
Lauren Rackley ◽  
Lauren Lee ◽  
...  
Keyword(s):  
Real Time ◽  
Logic Gates ◽  
Rna Aptamers ◽  
One Pot ◽  
Rna Nanotechnology ◽  
Close Proximity ◽  
Direct Tracking ◽  
Displacement Approach ◽  
User Friendly ◽  
In Cells

RNA aptamers selected to bind fluorophores and activate their fluorescence offer a simple and modular way to visualize native RNAs in cells. Split aptamers which are inactive until the halves are brought within close proximity can become useful for visualizing the dynamic actions of RNA assemblies and their interactions in real time with low background noise and eliminated necessity for covalently attached dyes. Here, we design and test several sets of F30 Broccoli aptamer splits, that we call fluorets, to compare their relative fluorescence and physicochemical stabilities. We show that the splits can be simply assembled either through one-pot thermal annealing or co-transcriptionally, thus allowing for direct tracking of transcription reactions via the fluorescent response. We suggest a set of rules that enable for the construction of responsive biomaterials that readily change their fluorescent behavior when various stimuli such as the presence of divalent ions, exposure to various nucleases, or changes in temperature are applied. We also show that the strand displacement approach can be used to program the controllable fluorescent responses in isothermal conditions. Overall, this work lays a foundation for the future development of dynamic systems for molecular computing which can be used to monitor real-time processes in cells and construct biocompatible logic gates.

Polarons and Triplet Excitons in C60: An Optically Detected Magnetic Resonance (Odmr) and Light-Induced Esr (Lesr) Study

1992 ◽  
Vol 270 ◽  
Author(s):  
P. A. Lane ◽  
L. S. Swanson ◽  
Q.-X. Ni ◽  
J. Shinar ◽  
J Engel ◽  
...  
Keyword(s):  
Magnetic Resonance ◽  
Conjugated Polymers ◽  
Glass Matrix ◽  
Membered Ring ◽  
X Band ◽  
Optically Detected Magnetic Resonance ◽  
Optically Detected ◽  
Triplet Excitons

ABSTRACTThe photoluminescence (PL), X-band ODMR. and LESR of C60 films and C60 isolated in a toluene/polystyrene glass matrix (C60:T/PS) is described. The delocalized triplet LESR and ODMR of C60:T/PS are similar to previously reported LESR. In films, however, the ODMR indicates that the delocalized triplet is larger and distorted by neighboring molecules. In addition, another, localized triplet, and a narrow PL-enhancing line at g = 2.0017 ± 0.0005 are observed. These features are similar to those observed in several π-conjugated polymers. The former is attributed to a localized triplet of size similar to a 5- or 6-membered ring, tentatively on a face adjacent to another C60 molecule; the latter is believed to result from intermolecular polaron recombination.

The Binding Energy of Charge-Transfer Excitons Localized at Polymeric Semiconductor Heterojunctions

2011 ◽  
Vol 115 (14) ◽  
pp. 7114-7119 ◽  
Author(s):  
Simon Gélinas ◽  
Olivier Paré-Labrosse ◽  
Colin-Nadeau Brosseau ◽  
Sebastian Albert-Seifried ◽  
Christopher R. McNeill ◽  
...  
Keyword(s):  
Charge Transfer ◽  
Binding Energy ◽  
Polymeric Semiconductor ◽  
Semiconductor Heterojunctions ◽  
Charge Transfer Excitons

Diffusion of Triplet Excitons in Anthracene

1965 ◽  
Vol 15 (2) ◽  
pp. 56-59 ◽  
Author(s):  
R. G. Kepler ◽  
A. C. Switendick
Keyword(s):  
Triplet Excitons
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