Enhancement of the second harmonic signal of nonlinear crystals by self-assembled gold nanoparticles

2020 ◽  
Vol 152 (10) ◽  
pp. 104711 ◽  
Author(s):  
Emre Gürdal ◽  
Anke Horneber ◽  
Nadim Shaqqura ◽  
Alfred J. Meixner ◽  
Dieter P. Kern ◽  
...  
2001 ◽  
Vol 707 ◽  
Author(s):  
C. Brands ◽  
P.J. Neyman ◽  
M.T. Guzy ◽  
S. Shah ◽  
K.E Van Cott ◽  
...  

ABSTRACTIonically self-assembled monolayers (ISAMs) have recently been shown to spontaneously exhibit a polar ordering that gives rise to substantial second order nonlinear optical response. The deposition of ISAMs has been studied in situ via second harmonic generation. This is a particularly sensitive probe of the growth of nanometer-thick films since the centrosymmetry of the immersion solutions, the substrate, and the container yields no SHG contribution from these bulk components. Upon immersion in the NLO-active polyelectrolyte solution, the SHG rises sharply over the first minute. When a film is immersed into salt water, the SHG decreases significantly only to be restored when the salt solution is replaced with deionized water.


Open Physics ◽  
2008 ◽  
Vol 6 (3) ◽  
Author(s):  
Robert Fischer ◽  
Solomon Saltiel ◽  
Dragomir Neshev ◽  
Wieslaw Krolikowski ◽  
Yuri Kivshar

AbstractWe investigate the transverse second-harmonic generation in as grown strontium barium niobate (SBN) crystals with a random structure of anti-parallel ferroelectric domains. We consider both, single and counter-propagating pulse geometries. We investigate polarization properties of the second harmonic signal and discuss applications of this process for short pulses characterization.


Nanoscale ◽  
2020 ◽  
Vol 12 (45) ◽  
pp. 23105-23115
Author(s):  
Emre Gürdal ◽  
Anke Horneber ◽  
Alfred J. Meixner ◽  
Dieter P. Kern ◽  
Dai Zhang ◽  
...  

This work fundamentally investigates how the second harmonic generation (SHG) from commercial nonlinear crystals can be boosted by the addition of individual optical nanoantennas.


2001 ◽  
Vol 710 ◽  
Author(s):  
C. Brands ◽  
P.J. Neyman ◽  
M.T. Guzy ◽  
S. Shah ◽  
K.E Van Cott ◽  
...  

ABSTRACTIonically self-assembled monolayers (ISAMs) have recently been shown to spontaneously exhibit a polar ordering that gives rise to substantial second order nonlinear optical response. The deposition of ISAMs has been studied in situ via second harmonic generation. This is a particularly sensitive probe of the growth of nanometer-thick films since the centrosymmetry of the immersion solutions, the substrate, and the container yields no SHG contribution from these bulk components. Upon immersion in the NLO-active polyelectrolyte solution, the SHG rises sharply over the first minute. When a film is immersed into salt water, the SHG decreases significantly only to be restored when the salt solution is replaced with deionized water.


1998 ◽  
Vol 519 ◽  
Author(s):  
David E. Zelmon ◽  
Zewdu Gebeyehu ◽  
David Tomlin ◽  
Thomas M. Cooper

AbstractWe have synthesized several metal xanthate complexes from metal salts and xanthate potassium salts. Powders of several of the materials were sorted and tested for their nonlinear optical properties. Cadmium xanthate demonstrated phase matchability for frequency doubling of 1.06 micron light and generated a very strong second harmonic signal.


2010 ◽  
Vol 19 (03) ◽  
pp. 445-458 ◽  
Author(s):  
MALYAJ DAS ◽  
SHIVANI RANA ◽  
PRATIMA SEN

A comparative study of the second harmonic generation in ZnO micro particles and nanorods has been experimentally studied by Kurtz technique using nanosecond pulsed Nd:YAG laser. The results have been theoretically explained by taking into account the quadrupole moment as well as surface nonlinearity. It was observed that the nanorods yield polarized second harmonic signal while the second harmonic signal obtained from the micro particles was unpolarized.


1989 ◽  
Vol 173 ◽  
Author(s):  
Richard S. Potember ◽  
Robert C. Hoffman ◽  
Karen A. Stetyick

ABSTRACTHydrazone, 1,1-dimethylhydrazone, methylhydrazone, phenylhydrazone and p-nitrophenyl hydrazone derivatives of substituted aromatic aldehydes were prepared and screened for second harmonic generation using the Kurtz powder technique. One compound, 4-nitro-3-methoxybenzaldehyde hydrazone exhibited a second harmonic signal up to 32 times that of ammonium dihydrogen phosphate (ADP) and 4-nitrobenzaldehyde hydrazone exhibited a second harmonic signal five times higher than previously reported, up to 40 times that of ADP. 3-methyl-4-nitrobenzaldehyde hydrazone, 4-nitrobenzaldehyde phenylhydrazone, 1-naphthaldehyde phenylhydrazone, 1-pyrenecarboxaldehyde phenylhydrazone exhibited second harmonic signals 25, 2.5, 5 and 20 times that of an ADP standard.


2006 ◽  
Vol 941 ◽  
Author(s):  
Haibin Zhao ◽  
Diyar Talbayev ◽  
Gunter Luepke ◽  
Aubrey Hanbicki ◽  
Connie Li ◽  
...  

AbstractA large nonlinear magneto-optical effect is observed in a non-centrosymmetric Fe/AlGaAs (001) heterostructure. This effect is a direct consequence of interference between second-harmonic optical waves of magnetic and crystallographic origin, generated at ferromagnetic Fe interface and bulk AlGaAs, respectively. The longitudinal nonlinear Kerr rotation is measured to be 1.6° along the [1-10] hard axis, about two orders of magnitude stronger than the linear equivalent. The rotational second-harmonic signal shows large magnetic contrast along all the in-plane directions, demonstrating a high sensitivity to the magnetization of an anisotropic interface in the longitudinal geometry.


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