Two wavelength operation of an acousto-optically tuned quantum cascade laser and direct measurements of quantum cascade laser level lifetimes

2017 ◽  
Vol 110 (3) ◽  
pp. 031104 ◽  
Author(s):  
C. Kumar N. Patel ◽  
Rodolfo Barron-Jimenez ◽  
Ilya Dunayevskiy ◽  
Gene Tsvid ◽  
Arkadiy Lyakh
2013 ◽  
Vol 6 (4) ◽  
pp. 927-936 ◽  
Author(s):  
B. Tuzson ◽  
K. Zeyer ◽  
M. Steinbacher ◽  
J. B. McManus ◽  
D. D. Nelson ◽  
...  

Abstract. A quantum cascade laser based absorption spectrometer for continuous and direct measurements of NO and NO2 was employed at the high-altitude monitoring site Jungfraujoch (3580 m a.s.l., Switzerland) during a three-month campaign in spring/summer 2012. The total reactive nitrogen, NOy, was also measured in the form of NO after conversion on a gold catalyst. The aim was to assess the suitability of the instrument for long-term monitoring of the main reactive nitrogen species under predominantly free tropospheric air conditions. A precision (1σ) of 10 and 3 ppt for NO and NO2 was achieved under field conditions after 180 s averaging time. The linear dynamic range of the instrument has been verified for both species from the detection limit up to 45 ppb. The spectrometer shared a common sampling inlet with a chemiluminescence-based analyzer. The comparison of the time series shows excellent agreement between the two techniques and demonstrates the adequacy of the laser spectroscopic approach for this kind of demanding environmental applications.


2012 ◽  
Vol 5 (6) ◽  
pp. 8969-8993 ◽  
Author(s):  
B. Tuzson ◽  
K. Zeyer ◽  
M. Steinbacher ◽  
J. B. McManus ◽  
D. D. Nelson ◽  
...  

Abstract. A quantum cascade laser based absorption spectrometer for continuous and direct measurements of NO and NO2 was employed at the high-altitude monitoring site Jungfraujoch (3580 m a.s.l., Switzerland) during a three month campaign in Spring/Summer 2012. The total reactive nitrogen, NOy, was also measured in the form of NO after conversion on a gold catalyst. The aim was to assess the suitability of the instrument for long-term monitoring of the main reactive nitrogen species under predominantly free tropospheric air conditions. A precision (1σ) of 10 and 3 ppt for NO and NO2 was achieved with 180 s averaging time under field conditions. The linear dynamic range of the instrument has been verified for both species from the detection limit to ≈45 ppbv. The spectrometer shared a common sampling inlet with a chemiluminescence-based analyzer. The comparison of the time series shows excellent agreement between the two techniques and demonstrates the adequacy of the laser spectroscopic approach for this kind of demanding environmental applications.


AIP Advances ◽  
2021 ◽  
Vol 11 (1) ◽  
pp. 015325
Author(s):  
Yuhong Zhou ◽  
Junqi Liu ◽  
Shenqiang Zhai ◽  
Ning Zhuo ◽  
Jinchuan Zhang ◽  
...  

2020 ◽  
Vol 22 (45) ◽  
pp. 26459-26467
Author(s):  
Jessica L. Klocke ◽  
Tilman Kottke

Flavin photoreduction in H2O is elucidated by developing a quantum cascade laser setup for time-resolved infrared spectroscopy on irreversible reactions.


2011 ◽  
Vol 99 (14) ◽  
pp. 141112 ◽  
Author(s):  
R. Eichholz ◽  
H. Richter ◽  
S. G. Pavlov ◽  
M. Wienold ◽  
L. Schrottke ◽  
...  

2021 ◽  
Vol 143 ◽  
pp. 107346
Author(s):  
Yuan-Yuan Li ◽  
Fang-Yuan Zhao ◽  
Yu Ma ◽  
Wei-Jiang Li ◽  
Jun-Qi Liu ◽  
...  

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