scholarly journals Computer simulation of the linear and nonlinear optical properties of liquid benzene: Its local fields, refractive index, and second nonlinear susceptibility

1999 ◽  
Vol 110 (13) ◽  
pp. 6463-6474 ◽  
Author(s):  
R. H. C. Janssen ◽  
J.-M. Bomont ◽  
D. N. Theodorou ◽  
S. Raptis ◽  
M. G. Papadopoulos
Keyword(s):  
Computer Simulation ◽  
Refractive Index ◽  
Optical Properties ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Local Fields ◽  
Nonlinear Susceptibility ◽  
Liquid Benzene ◽  
Linear And Nonlinear

scholarly journals Linear and nonlinear optical properties of hybrid metallic–dielectric plasmonic nanoantennas

2016 ◽  
Vol 7 ◽  
pp. 111-120 ◽  
Author(s):  
Mario Hentschel ◽  
Bernd Metzger ◽  
Bastian Knabe ◽  
Karsten Buse ◽  
Harald Giessen
Keyword(s):  
Refractive Index ◽  
Optical Properties ◽  
Nonlinear Optical ◽  
Nonlinear Response ◽  
High Efficiency ◽  
Dielectric Materials ◽  
Nonlinear Optical Properties ◽  
Linear Optical Properties ◽  
Linear And Nonlinear ◽  
Linear Optical

We study the linear and nonlinear optical properties of hybrid metallic–dielectric plasmonic gap nanoantennas. Using a two-step-aligned electron beam lithography process, we demonstrate the ability to selectively and reproducibly fill the gap region of nanoantennas with dielectric nanoparticles made of lithium niobate (LiNbO3) with high efficiency. The linear optical properties of the antennas are modified due to the large refractive index of the material. This leads to a change in the coupling strength as well as an increase of the effective refractive index of the surrounding. The combination of these two effects causes a red- or blue-shift of the plasmonic modes, respectively. We find that the nonlinear optical properties of the combined system are only modified in the range of one order of magnitude. The observed changes in our experiments in the nonlinear emission can be traced to the changed dielectric environment and thus the modified linear optical properties. The intrinsic nonlinearity of the dielectric used is in fact small when compared to the nonlinearity of the metallic part of the hybrid antennas. Thus, the nonlinear signals generated by the antenna itself are dominant in our experiments. We demonstrate that the well-known nonlinear response of bulk dielectric materials cannot always straightforwardly be used to boost the nonlinear response of nanoscale antenna systems. Our results significantly deepen the understanding of these interesting hybrid systems and offer important guidelines for the design of nanoscale, nonlinear light sources.

A DFT investigation of 45 wurtzite (B4)-type compounds: Structural, electronic, linear and nonlinear optical properties

2020 ◽  
Vol 34 (04) ◽  
pp. 2050010
Author(s):  
A. P. Gazhulina
Keyword(s):  
Optical Properties ◽  
Density Functional ◽  
Nonlinear Optical ◽  
Structural Type ◽  
Nonlinear Optical Properties ◽  
Nonlinear Susceptibility ◽  
Full Potential ◽  
Computational Data ◽  
Linear And Nonlinear ◽  
The Relationship

This work is a part of a series of investigations devoted to the study of the relationship between nonlinear optical properties and pseudosymmetric features of some groups of crystal compounds [A. P. Gazhulina and M. O. Marychev, Cryst. Struct. Theory Appl. 2, 106 (2013). doi.org/10.4236/csta.2013.23015 ; A. P. Gazhulina and M. O. Marychev, J. Alloys Compd. 623, 413 (2015). doi.org/10.1016/j.jallcom.2014.11.028 ; A. P. Gazhulina and M. O. Marychev, J. Solid State Chem. 239, 170 (2016). doi.org/10.1016/j.jssc.2016.04.034 ]. Crystals of the wurtzite ([Formula: see text]4) structural type (45 crystals) have been considered. In the framework of density functional theory, the structural, electronic, linear and nonlinear optical properties were investigated using the full-potential linearized augment plane wave (FP-LAPW) method. The obtained results are compared to available experimental and computational data. Diagrams “Second-order Nonlinear Susceptibility–Degree of Pseudoinversion” at 1.064 and 0.634 [Formula: see text]m wavelengths were constructed.

Linear and Nonlinear Optical Properties of Small Silicon Clusters

1990 ◽  
Author(s):  
Tapio T. Rantala ◽  
Mark I. Stockman ◽  
Daniel A. Jelski ◽  
Thomas F. George
Keyword(s):  
Optical Properties ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Silicon Clusters ◽  
Linear And Nonlinear

Mechanochemical synthesis, linear and nonlinear optical properties of a new oligophenyleneimine with indole terminal moiety for optoelectronic application

2021 ◽  
Author(s):  
Francisco Germán Mejía-Hernández ◽  
Oscar Javier Hernández-Ortíz ◽  
Francisco Misael Muñoz-Pérez ◽  
Armando Irving Martínez-Pérez ◽  
Rosa Angeles Vázquez-García ◽  
...  
Keyword(s):  
Optical Properties ◽  
Mechanochemical Synthesis ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Optoelectronic Application ◽  
Linear And Nonlinear

Integrity in linear and nonlinear optical properties of L-tyrosine doped bis thiourea cadmium acetate single crystal

2021 ◽  
Vol 573 (1) ◽  
pp. 52-62
Author(s):  
Siddique Aneesa-Fatema ◽  
Y. B. Rasal ◽  
R. N. Shaikh ◽  
M. D. Shirsat ◽  
S. S. Hussaini ◽  
...  
Keyword(s):  
Optical Properties ◽  
Single Crystal ◽  
Nonlinear Optical ◽  
Cadmium Acetate ◽  
Nonlinear Optical Properties ◽  
Linear And Nonlinear

scholarly journals Flexible Methyl Cellulose/Polyaniline/Silver Composite Films with Enhanced Linear and Nonlinear Optical Properties

Polymers ◽  
2021 ◽  
Vol 13 (8) ◽  
pp. 1225
Author(s):  
Ali Atta ◽  
Mostufa M. Abdelhamied ◽  
Ahmed M. Abdelreheem ◽  
Mohamed R. Berber
Keyword(s):  
Refractive Index ◽  
Optical Properties ◽  
Band Gap ◽  
Nonlinear Optical ◽  
Composite Films ◽  
Methyl Cellulose ◽  
Carbon Cluster ◽  
Nonlinear Susceptibility ◽  
Optical Parameters ◽  
Flexible Polymer

In order to potentiate implementations in optical energy applications, flexible polymer composite films comprising methyl cellulose (MC), polyaniline (PANI) and silver nanoparticles (AgNPs) were successfully fabricated through a cast preparation method. The composite structure of the fabricated film was confirmed by X-ray diffraction and infrared spectroscopy, indicating a successful incorporation of AgNPs into the MC/PANI blend. The scanning electron microscope (SEM) images have indicated a homogenous loading and dispersion of AgNPs into the MC/PANI blend. The optical parameters such as band gap (Eg), absorption edge (Ed), number of carbon cluster (N) and Urbach energy (Eu) of pure MC polymer, MC/PANI blend and MC/PANI/Ag films were determined using the UV optical absorbance. The effects of AgNPs and PANI on MC polymer linear optical (LO) and nonlinear optical (NLO) parameters including reflection extinction coefficient, refractive index, dielectric constant, nonlinear refractive index, and nonlinear susceptibility are studied. The results showed a decrease in the band gap of MC/PANI/AgNPs compared to the pure MC film. Meanwhile, the estimated carbon cluster number enhanced with the incorporation of the AgNPs. The inclusion of AgNPs and PANI has enhanced the optical properties of the MC polymer, providing a new composite suitable for energy conversion systems, solar cells, biosensors, and nonlinear optical applications.

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