Infrared profile of single molecules adsorbed on ionic substrates: Relaxational mechanism for the homogeneous linewidth

1996 ◽  
Vol 105 (6) ◽  
pp. 2471-2486 ◽  
Author(s):  
A. Lakhlifi ◽  
C. Girardet
Keyword(s):  
Single Molecules ◽  
Homogeneous Linewidth

Single molecules in the dark

2009 ◽  
Vol 11 (S1) ◽  
pp. S19-S19 ◽  
Author(s):  
Daniel Evanko
Keyword(s):  
Single Molecules

Multifunctional far-field luminescence nanoscope for studying single molecules and quantum dots

2018 ◽  
Vol 189 (03) ◽  
pp. 312-322 ◽  
Author(s):  
Ivan Yu. Eremchev ◽  
M.Yu. Eremchev ◽  
Andrei V. Naumov
Keyword(s):  
Quantum Dots ◽  
Single Molecules ◽  
Far Field

Nanopore detection of DNA damage in single molecules

2011 ◽  
Author(s):  
N. An ◽  
Aaron M. Fleming ◽  
Cynthia J. Burrows
Keyword(s):  
Dna Damage ◽  
Single Molecules

scholarly journals Effect of elastic colored noise in the hopping dynamics of single molecules in stretching experiments

2015 ◽  
Vol 92 (6) ◽  
Author(s):  
M. Hidalgo-Soria ◽  
A. Pérez-Madrid ◽  
I. Santamaría-Holek
Keyword(s):  
Colored Noise ◽  
Single Molecules

Single Molecules in Strong Optical Fields: A Variable-Temperature Molecular Junction Spectroscopy Setup

2021 ◽  
Author(s):  
Hai Bi ◽  
Chao Jing ◽  
Peter Hasch ◽  
Yuxiang Gong ◽  
Daniel Gerster ◽  
...  
Keyword(s):  
Variable Temperature ◽  
Single Molecules ◽  
Molecular Junction ◽  
Optical Fields

scholarly journals One-Dimensional Lateral Force Anisotropy at the Atomic Scale in Sliding Single Molecules on a Surface

Nano Letters ◽  
2021 ◽  
Author(s):  
Yuan Zhang ◽  
Daniel J. Trainer ◽  
Badri Narayanan ◽  
Yang Li ◽  
Anh T. Ngo ◽  
...  
Keyword(s):  
Single Molecules ◽  
Lateral Force ◽  
Atomic Scale ◽  
One Dimensional

scholarly journals Optical spin-state polarization in a binuclear europium complex towards molecule-based coherent light-spin interfaces

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Kuppusamy Senthil Kumar ◽  
Diana Serrano ◽  
Aline M. Nonat ◽  
Benoît Heinrich ◽  
Lydia Karmazin ◽  
...  
Keyword(s):  
Ground State ◽  
Quantum Information Processing ◽  
Optical Transition ◽  
Molecular Engineering ◽  
Coherent Light ◽  
Nuclear Spins ◽  
Rare Earth Ion ◽  
Molecular Systems ◽  
Homogeneous Linewidth ◽  
State Spin

AbstractThe success of the emerging field of solid-state optical quantum information processing (QIP) critically depends on the access to resonant optical materials. Rare-earth ion (REI)-based molecular systems, whose quantum properties could be tuned taking advantage of molecular engineering strategies, are one of the systems actively pursued for the implementation of QIP schemes. Herein, we demonstrate the efficient polarization of ground-state nuclear spins—a fundamental requirement for all-optical spin initialization and addressing—in a binuclear Eu(III) complex, featuring inhomogeneously broadened 5D0 → 7F0 optical transition. At 1.4 K, long-lived spectral holes have been burnt in the transition: homogeneous linewidth (Γh) = 22 ± 1 MHz, which translates as optical coherence lifetime (T2opt) = 14.5 ± 0.7 ns, and ground-state spin population lifetime (T1spin) = 1.6 ± 0.4 s have been obtained. The results presented in this study could be a progressive step towards the realization of molecule-based coherent light-spin QIP interfaces.

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