Third order ab initio calculations of amplitudes of two‐photon absorption for ions across the lanthanide series

1989 ◽  
Vol 90 (3) ◽  
pp. 1390-1395 ◽  
Author(s):  
Lidia Smentek‐Mielczarek ◽  
B.Andes Hess
Keyword(s):  
Ab Initio Calculations ◽  
Ab Initio ◽  
Photon Absorption ◽  
Third Order ◽  
Two Photon Absorption ◽  
Two Photon ◽  
Lanthanide Series

Third-order nonlinear optical properties and two-photon absorption in branched oligothienylenevinylenes

2002 ◽  
Vol 209 (4-6) ◽  
pp. 461-466 ◽  
Author(s):  
I. Fuks-Janczarek ◽  
J-M. Nunzi ◽  
B. Sahraoui ◽  
I.V. Kityk ◽  
J. Berdowski ◽  
...  
Keyword(s):  
Optical Properties ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Photon Absorption ◽  
Third Order ◽  
Two Photon Absorption ◽  
Two Photon

scholarly journals The Influence of Quantum Confinement on Third-Order Nonlinearities in Porous Silicon Thin Films

2018 ◽  
Vol 8 (10) ◽  
pp. 1810 ◽  
Author(s):  
Rihan Wu ◽  
Jack Collins ◽  
Leigh Canham ◽  
Andrey Kaplan
Keyword(s):  
Refractive Index ◽  
Nonlinear Refractive Index ◽  
Quantum Confinement ◽  
Nonlinear Refraction ◽  
Photon Absorption ◽  
Third Order ◽  
Two Photon Absorption ◽  
Two Photon ◽  
Silicon Thin Films ◽  
Gaussian Decomposition

We present an experimental investigation into the third-order nonlinearity of conventional crystalline (c-Si) and porous (p-Si) silicon with Z-scan technique at 800-nm and 2.4- μ m wavelengths. The Gaussian decomposition method is applied to extract the nonlinear refractive index, n 2 , and the two-photon absorption (TPA) coefficient, β , from the experimental results. The nonlinear refractive index obtained for c-Si is 7 ± 2 × 10 − 6 cm 2 /GW and for p-Si is − 9 ± 3 × 10 − 5 cm 2 /GW. The TPA coefficient was found to be 2.9 ± 0.9 cm/GW and 1.0 ± 0.3 cm/GW for c-Si and p-Si, respectively. We show an enhancement of the nonlinear refraction and a suppression of TPA in p-Si in comparison to c-Si, and the enhancement gets stronger as the wavelength increases.

Third-order nonlinear optical properties and two-photon absorption in polymers doped withp-phenyl sydnone

2008 ◽  
Vol 108 (5) ◽  
pp. 3218-3224 ◽  
Author(s):  
Seetharam Shettigar ◽  
G. Umesh ◽  
K. Chandrasekharan ◽  
Ganesh Rai ◽  
B. Kalluraya
Keyword(s):  
Optical Properties ◽  
Nonlinear Optical ◽  
Nonlinear Optical Properties ◽  
Photon Absorption ◽  
Third Order ◽  
Two Photon Absorption ◽  
Two Photon

Two-Photon Absorption and Degenerate Four-Wave Mixing Studies of Sulfide Semiconductor Nanoparticles in Polymeric Solutions

2008 ◽  
Vol 8 (3) ◽  
pp. 1364-1370 ◽  
Author(s):  
Wenling Jia ◽  
Fengqi Guo ◽  
Elliot P. Douglas ◽  
Wenfang Sun
Keyword(s):  
Four Wave Mixing ◽  
Semiconductor Nanoparticles ◽  
Photon Absorption ◽  
Wave Mixing ◽  
Absorption Coefficients ◽  
Third Order ◽  
Two Photon Absorption ◽  
Two Photon ◽  
The Third ◽  
Degenerate Four Wave Mixing

The two-photon absorption coefficients (β) and the third-order nonlinear susceptibilities (χ(3)) of several semiconductor nanoparticles (CdS, CdxAg1–xS, and core–shell CdS/Ag2S) that are confined and stabilized by random and block ionomers have been measured by nonlinear transmission and degenerate four-wave mixing techniques using 21 picosecond laser pulses at near-infrared spectral region. The imaginary part of the third-order nonlinear susceptibility that is related to the two-photon absorption coefficient was then calculated. The absorptive nonlinearity of the nanoparticles (2∼9 nm) was found to be dependent on the particle size, composition and wavelength, i.e., larger CdS particles exhibit higher two-photon absorption coefficients and the presence of Ag improves two-photon absorption of CdS nanoparticles. The obtained two-photon absorption coefficients of nanoparticles corrected for their volume fraction in solution are significantly greater that those of corresponding bulk semiconductors.

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