Raman pump/probe measurements of state‐to‐state energy transfer rates in the v=1 state of H2

1988 ◽  
Vol 89 (4) ◽  
pp. 1994-1998 ◽  
Author(s):  
R. L. Farrow ◽  
D. W. Chandler
Keyword(s):  
Energy Transfer ◽  
State Energy ◽  
Pump Probe ◽  
Transfer Rates ◽  
Probe Measurements ◽  
Raman Pump

Pump-Probe Measurements Using Silicon Nanocrystal Waveguides

2003 ◽  
Vol 770 ◽  
Author(s):  
Nathanael Smith ◽  
Max J. Lederer ◽  
Marek Samoc ◽  
Barry Luther-Davies ◽  
Robert G. Elliman
Keyword(s):  
Probe Beam ◽  
Time Resolution ◽  
Pump Beam ◽  
Silicon Nanocrystals ◽  
Continuous Wave ◽  
Optical Gain ◽  
Optical Pump ◽  
Time Resolved ◽  
Pump Probe ◽  
Probe Measurements

AbstractOptical pump-probe measurements were performed on planar slab waveguides containing silicon nanocrystals in an attempt to measure optical gain from photo-excited silicon nanocrystals. Two experiments were performed, one with a continuous-wave probe beam and a pulsed pump beam, giving a time resolution of approximately 25 ns, and the other with a pulsed pump and probe beam, giving a time resolution of approximately 10 ps. In both cases the intensity of the probe beam was found to be attenuated by the pump beam, with the attenuation increasing monotonically with increasing pump power. Time-resolved measurements using the first experimental arrangement showed that the probe signal recovered its initial intensity on a time scale of 45-70 μs, a value comparable to the exciton lifetime in Si nanocrystals. These data are shown to be consistent with an induced absorption process such as confined carrier absorption. No evidence for optical gain was observed.

Origin of the Red Sites and Energy Transfer Rates in Single MEH-PPV Chains at Low Temperature

ChemPhysChem ◽  
2011 ◽  
Vol 12 (8) ◽  
pp. 1499-1508 ◽  
Author(s):  
Florian A. Feist ◽  
Martin F. Zickler ◽  
Thomas Basché
Keyword(s):  
Energy Transfer ◽  
Low Temperature ◽  
Transfer Rates

scholarly journals Ultrafast Electron/Energy Transfer and Intersystem Crossing Mechanisms in BODIPY-Porphyrin Compounds

Processes ◽  
2021 ◽  
Vol 9 (2) ◽  
pp. 312
Author(s):  
Yusuf Tutel ◽  
Gökhan Sevinç ◽  
Betül Küçüköz ◽  
Elif Akhuseyin Yildiz ◽  
Ahmet Karatay ◽  
...  
Keyword(s):  
Energy Transfer ◽  
Fluorescence Spectra ◽  
Visible Region ◽  
Energy Transfer Mechanism ◽  
Free Base ◽  
Pump Probe ◽  
Harvesting Efficiency ◽  
Probe Spectroscopy ◽  
Absorption Features ◽  
Transfer Mechanisms

Meso-substituted borondipyrromethene (BODIPY)-porphyrin compounds that include free base porphyrin with two different numbers of BODIPY groups (BDP-TTP and 3BDP-TTP) were designed and synthesized to analyze intramolecular energy transfer mechanisms of meso-substituted BODIPY-porphyrin dyads and the effect of the different numbers of BODIPY groups connected to free-base porphyrin on the energy transfer mechanism. Absorption spectra of BODIPY-porphyrin conjugates showed wide absorption features in the visible region, and that is highly valuable to increase light-harvesting efficiency. Fluorescence spectra of the studied compounds proved that BODIPY emission intensity decreased upon the photoexcitation of the BODIPY core, due to the energy transfer from BODIPY unit to porphyrin. In addition, ultrafast pump-probe spectroscopy measurements indicated that the energy transfer of the 3BDP-TTP compound (about 3 ps) is faster than the BDP-TTP compound (about 22 ps). Since the BODIPY core directly binds to the porphyrin unit, rapid energy transfer was seen for both compounds. Thus, the energy transfer rate increased with an increasing number of BODIPY moiety connected to free-base porphyrin.

scholarly journals Giant Photoluminescence Enhancement and Carrier Dynamics in MoS2 Bilayers with Anomalous Interlayer Coupling

Nanomaterials ◽  
2021 ◽  
Vol 11 (8) ◽  
pp. 1994
Author(s):  
Han Li ◽  
Yating Ma ◽  
Zhongjie Xu ◽  
Xiang’ai Cheng ◽  
Tian Jiang
Keyword(s):  
Optical Properties ◽  
Transition Metal Dichalcogenides ◽  
Interlayer Coupling ◽  
Carrier Dynamics ◽  
Probe Signal ◽  
Exciton Resonance ◽  
Pump Probe ◽  
Metal Dichalcogenides ◽  
Photoluminescence Enhancement ◽  
Probe Measurements

Fundamental researches and explorations based on transition metal dichalcogenides (TMDCs) mainly focus on their monolayer counterparts, where optical densities are limited owing to the atomic monolayer thickness. Photoluminescence (PL) yield in bilayer TMDCs is much suppressed owing to indirect-bandgap properties. Here, optical properties are explored in artificially twisted bilayers of molybdenum disulfide (MoS2). Anomalous interlayer coupling and resultant giant PL enhancement are firstly observed in MoS2 bilayers, related to the suspension of the top layer material and independent of twisted angle. Moreover, carrier dynamics in MoS2 bilayers with anomalous interlayer coupling are revealed with pump-probe measurements, and the secondary rising behavior in pump-probe signal of B-exciton resonance, originating from valley depolarization of A-exciton, is firstly reported and discussed in this work. These results lay the groundwork for future advancement and applications beyond TMDCs monolayers.

Coherent coupling effects in pump–probe measurements with collinear, copropagating beams

1984 ◽  
Vol 9 (8) ◽  
pp. 359 ◽  
Author(s):  
T. F. Heinz ◽  
K. B. Eisenthal ◽  
S. L. Palfrey
Keyword(s):  
Coupling Effects ◽  
Pump Probe ◽  
Coherent Coupling ◽  
Probe Measurements
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