Ab initio study of the one- and two-photon circular dichroism of R-(+)-3-methyl-cyclopentanone

2008 ◽  
Vol 128 (16) ◽  
pp. 164312 ◽  
Author(s):  
Antonio Rizzo ◽  
Na Lin ◽  
Kenneth Ruud
2010 ◽  
Vol 114 (19) ◽  
pp. 6500-6512 ◽  
Author(s):  
Maxime Guillaume ◽  
Kenneth Ruud ◽  
Antonio Rizzo ◽  
Susanna Monti ◽  
Zijing Lin ◽  
...  

Author(s):  
В.Р. Расулов ◽  
Р.Я. Расулов ◽  
Б.Б. Ахмедов ◽  
И.А. Муминов

Interband two-photon optical transitions are classified and expressions are obtained for the matrix elements in a narrow-gap semiconductor depending on the band parameters, degree of polarization, and light frequency. It is shown that the main contribution to two-photon linear-circular dichroism in narrow-gap semiconductors is made by optical transitions proceeding from the subband of light holes to the conduction band. The dependences of the partial coefficients of interband two-photon absorption of light, which differ from each other by the types of optical transitions, are analyzed depending on the degree of polarization of the light, and a quantitative analysis of the coefficient of linear-circular dichroism of two-photon absorption of light is carried out. Expressions are obtained for the spectral dependence of the coefficient of interband two-photon absorption of light in narrow-gap semiconductors in the Kane model.


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