scholarly journals Real-time observation of intramolecular proton transfer in the electronic ground state of chloromalonaldehyde: Anab initiostudy of time-resolved photoelectron spectra

2007 ◽  
Vol 126 (5) ◽  
pp. 054303 ◽  
Author(s):  
Márcio T. do N. Varella ◽  
Yasuki Arasaki ◽  
Hiroshi Ushiyama ◽  
Kazuo Takatsuka ◽  
Kwanghsi Wang ◽  
...  
Keyword(s):  
Proton Transfer ◽  
Real Time ◽  
Ground State ◽  
Intramolecular Proton Transfer ◽  
Electronic Ground State ◽  
Photoelectron Spectra ◽  
Time Resolved ◽  
Time Observation ◽  
Real Time Observation ◽  
Electronic Ground

Real-time observation of ground state proton transfer: a model study

2005 ◽  
Vol 311 (3) ◽  
pp. 255-268 ◽  
Author(s):  
Yasuki Arasaki ◽  
Kentaro Yamazaki ◽  
Márcio T. do N. Varella ◽  
Kazuo Takatsuka
Keyword(s):  
Proton Transfer ◽  
Real Time ◽  
Ground State ◽  
Model Study ◽  
Time Observation ◽  
Real Time Observation

Real-Time Observation for the Enzymatic Reaction of Phospholipid Membrane:  Application of the Time-Resolved Quasi-Elastic Laser Scattering Method

2004 ◽  
Vol 76 (8) ◽  
pp. 2314-2320 ◽  
Author(s):  
Toshinori Morisaku ◽  
Hiroharu Yui ◽  
Masanori Iwazumi ◽  
Yasuhiro Ikezoe ◽  
Masanori Fujinami ◽  
...  
Keyword(s):  
Real Time ◽  
Enzymatic Reaction ◽  
Scattering Method ◽  
Phospholipid Membrane ◽  
Laser Scattering ◽  
Time Resolved ◽  
Time Observation ◽  
Real Time Observation

scholarly journals Real-time observation of a correlation-driven sub 3 fs charge migration in ionised adenine

2021 ◽  
Vol 4 (1) ◽  
Author(s):  
Erik P. Månsson ◽  
Simone Latini ◽  
Fabio Covito ◽  
Vincent Wanie ◽  
Mara Galli ◽  
...  
Keyword(s):  
Real Time ◽  
Charge Redistribution ◽  
Many Body ◽  
Charge Migration ◽  
Time Resolved ◽  
Molecular Reactivity ◽  
Time Observation ◽  
A Charge ◽  
Doubly Charged ◽  
Real Time Observation

AbstractSudden ionisation of a relatively large molecule can initiate a correlation-driven process dubbed charge migration, where the electron density distribution is expected to rapidly move along the molecular backbone. Capturing this few-femtosecond or attosecond charge redistribution would represent the real-time observation of electron correlation in a molecule with the enticing prospect of following the energy flow from a single excited electron to the other coupled electrons in the system. Here, we report a time-resolved study of the correlation-driven charge migration process occurring in the nucleic-acid base adenine after ionisation with a 15–35 eV attosecond pulse. We find that the production of intact doubly charged adenine – via a shortly-delayed laser-induced second ionisation event – represents the signature of a charge inflation mechanism resulting from many-body excitation. This conclusion is supported by first-principles time-dependent simulations. These findings may contribute to the control of molecular reactivity at the electronic, few-femtosecond time scale.

Real-time observation of the photoionization-induced water rearrangement dynamics in the 5-hydroxyindole–water cluster by time-resolved IR spectroscopy

2018 ◽  
Vol 20 (5) ◽  
pp. 3079-3091 ◽  
Author(s):  
Mitsuhiko Miyazaki ◽  
Ayumi Naito ◽  
Takamasa Ikeda ◽  
Johanna Klyne ◽  
Kenji Sakota ◽  
...  
Keyword(s):  
Ir Spectroscopy ◽  
Real Time ◽  
Water Cluster ◽  
Time Resolved ◽  
Energy Accumulation ◽  
Time Observation ◽  
Real Time Observation

Climbing the ladder by energy accumulation through IVR takes more than a nanosecond.

scholarly journals Real-time observation of Cooper pair splitting showing strong non-local correlations

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Antti Ranni ◽  
Fredrik Brange ◽  
Elsa T. Mannila ◽  
Christian Flindt ◽  
Ville F. Maisi
Keyword(s):  
Real Time ◽  
Cooper Pair ◽  
Foundations Of Quantum Mechanics ◽  
Direct Access ◽  
Cooper Pairs ◽  
Time Resolved ◽  
Time Observation ◽  
The Individual ◽  
Real Time Observation ◽  
Cooper Pair Splitting

AbstractControlled generation and detection of quantum entanglement between spatially separated particles constitute an essential prerequisite both for testing the foundations of quantum mechanics and for realizing future quantum technologies. Splitting of Cooper pairs from a superconductor provides entangled electrons at separate locations. However, experimentally accessing the individual split Cooper pairs constitutes a major unresolved issue as they mix together with electrons from competing processes. Here, we overcome this challenge with the first real-time observation of the splitting of individual Cooper pairs, enabling direct access to the time-resolved statistics of Cooper pair splitting. We determine the correlation statistics arising from two-electron processes and find a pronounced peak that is two orders of magnitude larger than the background. Our experiment thereby allows to unambiguously pinpoint and select split Cooper pairs with 99% fidelity. These results open up an avenue for performing experiments that tap into the spin-entanglement of split Cooper pairs.

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