Depolarized Rayleigh scattering in liquids. Molecular reorientation and orientation pair correlations in a nematic liquid crystal: MBBA

1974 ◽  
Vol 61 (6) ◽  
pp. 2231-2239 ◽  
Author(s):  
T. D. Gierke ◽  
W. H. Flygare
2018 ◽  
Vol 10 (4) ◽  
pp. 109
Author(s):  
Filip Sala

By lunching the beam into the chiral nematic liquid crystals it is possible to achieve a non-diffractive beam similar to a soliton. This effect is caused by the molecular reorientation i.e. nonlinear response of the material forming the areas of higher refractive index. Diffraction is suppressed by the focusing effect. For appropriate launching conditions it is also possible to achieve a beam which splits into two or more separate beams. Such phenomenon is discussed in this article and analyzed theoretical. To model this effect Fully Vectorial Beam Propagation Method coupled with the Frank-Oseen elastic theory is used. Simulations are performed for various input beam powers, widths, polarization angles and launching positions. Full Text: PDF ReferencesG. Assanto and M. A. Karpierz, "Nematicons: self-localised beams in nematic liquid crystals", Liq. Cryst. 36, 1161–1172 (2009) CrossRef G. Assanto, Nematicons: Spatial Optical Solitons in Nematic Liquid Crystals, John Wiley & Sons Inc. Hoboken, New Jersey (2013) DirectLink A. Piccardi, A. Alberucci, U. Bortolozzo, S. Residori, and G. Assanto, "Soliton gating and switching in liquid crystal light valve", Appl. Phys. Lett. 96, 071104 (2010). CrossRef D. Melo, I. Fernandes, F. Moraes, S. Fumeron, and E. Pereira, "Thermal diode made by nematic liquid crystal", Phys. Lett. A 380, 3121 – 3127 (2016). CrossRef U. Laudyn, M. Kwaśny, F. A. Sala, M. A. Karpierz, N. F. Smyth, G. Assanto, "Curved optical solitons subject to transverse acceleration in reorientational soft matter", Sci. Rep. 7, 12385 (2017) CrossRef M. Kwaśny, U. A. Laudyn, F. A. Sala, A. Alberucci, M. A. Karpierz, G. Assanto, "Self-guided beams in low-birefringence nematic liquid crystals", Phys. Rev. A 86, 013824 (2012) CrossRef F. A. Sala, M. M. Sala-Tefelska, "Optical steering of mutual capacitance in a nematic liquid crystal cell", J. Opt. Soc. Am. B. 35, 133-139 (2018) CrossRef U. A. Laudyn, A. Piccardi, M. Kwasny, M. A. Karpierz, G. Assanto, "Thermo-optic soliton routing in nematic liquid crystals", Opt. Lett. 43, 2296-2299 (2018) CrossRef F. A. Sala, M. M. Sala-Tefelska, M. J. Bujok, J. "Influence of temperature diffusion on molecular reorientation in nematic liquid crystals", Nonlinear Opt. Phys. Mater. 27, 1850011 (2018) CrossRef I-C Khoo Liquid crystals John Wiley & Sons, Inc (2007) DirectLink P. G. de Gennes, J. Prost, The Physics of Liquid Crystals, Clarendon Press (1995) DirectLink U. A. Laudyn, P. S. Jung, M. A. Karpierz, G. Assanto, "Quasi two-dimensional astigmatic solitons in soft chiral metastructures", Sci. Rep. 6, 22923 (2016) CrossRef J. Beeckman, A. Madani, P. J. M. Vanbrabant, P. Henneaux, S-P. Gorza, M. Haelterman, "Switching and intrinsic position bistability of soliton beams in chiral nematic liquid crystals", Phys. Rev. A 83, 033832 (2011) CrossRef A. Madani, J. Beeckman, K. Neyts, "An experimental observation of a spatial optical soliton beam and self splitting of beam into two soliton beams in chiral nematic liquid crystal", Opt. Commun. 298–299, 222-226, (2013) CrossRef G. D. Ziogos, E. E. Kriezis, "Modeling light propagation in liquid crystal devices with a 3-D full-vector finite-element beam propagation method", Opt. Quant. Electron 40, 10 (2008) CrossRef F. A. Sala, M. A. Karpierz, "Chiral and nonchiral nematic liquid-crystal reorientation induced by inhomogeneous electric fields", J. Opt. Soc. Am. B 29, 1465-1472 (2012) CrossRef F. A. Sala, M. A. Karpierz, "Modeling of molecular reorientation and beam propagation in chiral and non-chiral nematic liquid crystals", Opt. Express 20, 13923-13938 (2012) CrossRef F. A. Sala, "Design of false color palettes for grayscale reproduction", Displays, 46, 9-15 (2017) CrossRef


2021 ◽  
Vol 118 (22) ◽  
pp. e2104092118
Author(s):  
Xi Chen ◽  
Eva Korblova ◽  
Matthew A. Glaser ◽  
Joseph E. Maclennan ◽  
David M. Walba ◽  
...  

We show that surface interactions can vectorially structure the three-dimensional polarization field of a ferroelectric fluid. The contact between a ferroelectric nematic liquid crystal and a surface with in-plane polarity generates a preferred in-plane orientation of the polarization field at that interface. This is a route to the formation of fluid or glassy monodomains of high polarization without the need for electric field poling. For example, unidirectional buffing of polyimide films on planar surfaces to give quadrupolar in-plane anisotropy also induces macroscopic in-plane polar order at the surfaces, enabling the formation of a variety of azimuthal polar director structures in the cell interior, including uniform and twisted states. In a π-twist cell, obtained with antiparallel, unidirectional buffing on opposing surfaces, we demonstrate three distinct modes of ferroelectric nematic electro-optic response: intrinsic, viscosity-limited, field-induced molecular reorientation; field-induced motion of domain walls separating twisted states of opposite chirality; and propagation of polarization reorientation solitons from the cell plates to the cell center upon field reversal. Chirally doped ferroelectric nematics in antiparallel-rubbed cells produce Grandjean textures of helical twist that can be unwound via field-induced polar surface reorientation transitions. Fields required are in the 3-V/mm range, indicating an in-plane polar anchoring energy of wP ∼3 × 10−3 J/m2.


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