scholarly journals Nuclear dynamics in electronic ground and excited states probed by spectrally resolved four wave mixing

2002 ◽  
Vol 116 (24) ◽  
pp. 10801-10808 ◽  
Author(s):  
June-Sik Park ◽  
Taiha Joo
2018 ◽  
Vol 4 (9) ◽  
pp. eaau3783 ◽  
Author(s):  
Hugo J. B. Marroux ◽  
Ashley P. Fidler ◽  
Daniel M. Neumark ◽  
Stephen R. Leone

Dynamics following excitation with attosecond extreme ultraviolet (XUV) pulses arise from enormous numbers of accessible excited states, complicating the retrieval of state-specific time evolutions. We develop attosecond XUV multidimensional spectroscopy here to separate interfering pathways on a near-infrared (NIR) energy axis, retrieving single state dynamics in argon atoms in a two-dimensional (2D) XUV-NIR spectrum. In this experiment, we measure four-wave mixing signal arising from the interaction of XUV attosecond pulses centered around 15 eV with two few-cycle NIR pulses. The 2D spectrum is created by measuring the emitted XUV signal field spectrum while applying narrowband amplitude and phase modulations to one of the NIR pulses. Application of such a technique to systems of high dimensionality will provide for the observation of state-resolved pure electronic dynamics, in direct analogy to phenomena unraveled by multidimensional spectroscopies at optical frequencies.


1994 ◽  
Vol 9 (5S) ◽  
pp. 419-421 ◽  
Author(s):  
P Leisching ◽  
P Haring Bolivar ◽  
R Schwedler ◽  
K Leo ◽  
H Kurz ◽  
...  

2003 ◽  
Vol 72 (8) ◽  
pp. 1863-1866 ◽  
Author(s):  
Osamu Arimoto ◽  
Mieko Sakamoto ◽  
Yutaka Imai ◽  
Shunsuke Nakanishi ◽  
Hiroshi Itoh

2012 ◽  
Vol 20 (6) ◽  
pp. 6204 ◽  
Author(s):  
Utsab Khadka ◽  
Huaibin Zheng ◽  
Min Xiao

1996 ◽  
Vol 13 (5) ◽  
pp. 977 ◽  
Author(s):  
M. U. Wehner ◽  
D. Steinbach ◽  
M. Wegener ◽  
T. Marschner ◽  
W. Stolz

1998 ◽  
Vol 07 (01) ◽  
pp. 153-159 ◽  
Author(s):  
J. Ishi ◽  
M. Mizuno ◽  
H. Kunugita ◽  
K. Ema ◽  
S. Iwamoto ◽  
...  

Third-order optical nonlinearity around the exciton resonance in (C6H13NH3)2PbI4 was measured using time-integrated and spectrally-resolved four-wave-mixing (FWM) techniques. For excitation below the exciton resonance, biexciton contribution to the FWM signals was observed. The dephasing energy of the biexcitons was estimated to be larger than 10 meV.


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