Progress towards fundamental symmetry tests with nonlinear optical rotation

Author(s):  
D. F. Kimball
Crystals ◽  
2018 ◽  
Vol 9 (1) ◽  
pp. 8 ◽  
Author(s):  
Johannes Buchen ◽  
Volker Wesemann ◽  
Steffen Dehmelt ◽  
Andreas Gross ◽  
Daniel Rytz

Many borate crystals feature nonlinear optical properties that allow for efficient frequency conversion of common lasers down into the ultraviolet spectrum. Twinning may degrade crystal quality and affect nonlinear optical properties, in particular if crystals are composed of twin domains with opposing polarities. Here, we use measurements of optical activity to demonstrate the existence of inversion twins within single crystals of YAl 3 (BO 3 ) 4 (YAB) and K 2 Al 2 B 2 O 7 (KABO). We determine the optical rotatory dispersion of YAB and KABO throughout the visible spectrum using a spectrophotometer with rotatable polarizers. Space-resolved measurements of the optical rotation can be related to the twin structure and give estimates on the extent of twinning. The reported dispersion relations for the rotatory power of YAB and KABO may be used to assess crystal quality and to select twin-free specimens.


2017 ◽  
Vol 8 (1) ◽  
Author(s):  
M. Ahmadi ◽  
B. X. R. Alves ◽  
C. J. Baker ◽  
W. Bertsche ◽  
E. Butler ◽  
...  

2018 ◽  
Vol 49 (3) ◽  
pp. 229
Author(s):  
P.E. Garrett ◽  
K.G. Leach ◽  
A.D. MacLean ◽  
G.C. Ball ◽  
P.C. Bender ◽  
...  

2013 ◽  
Vol 12 (04) ◽  
pp. 1350027 ◽  
Author(s):  
A. M. KOKHKHAROV ◽  
E. A. ZAKHIDOV ◽  
SH. P. GOFUROV ◽  
S. A. BAKHRAMOV ◽  
U. K. MAKHMANOV

Nonlinear optical rotation of elliptically polarized laser pulses (λ = 532 nm, τFWHM ~ 12 ns) in benzene, toluene and binary (toluene+acetonitrile) solutions of fullerene C 70–D5h(6) has been investigated experimentally. High-resolution transmission electron microscope studies of C 70-solutions showed stable ball-shaped C 70-clusters formation in toluene+acetonitrile mixtures. It has been demonstrated, that the C 70-clusters sizes depend on initial concentration of C 70, as well as volume fraction of acetonitrile in solvent mixture. The most probable model of C 70-clusterization in solutions was proposed. Correlations between the processes of nonlinear rotation of polarization ellipse, change of electronic absorption spectra and C 70-clusters formation in solutions have been demonstrated. Physical mechanisms of laser-induced optical activity in C 70-solutions have been discussed. The values of the nonlinear Kerr coefficient (n2) and nonlinear susceptibility component [Formula: see text] of C 70-solutions in: toluene, benzene with various polarization ellipticity (θ = 0.2-0.8), and toluene+acetonitrile at different concentrations of C 70 for various volume fractions of acetonitrile have been determined.


Physics ◽  
2021 ◽  
Vol 14 ◽  
Author(s):  
Ronald F. Garcia Ruiz

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