scholarly journals Initial time‐resolved particle beam profile measurements at the Advanced Photon Source

1996 ◽  
Vol 67 (9) ◽  
pp. 3367-3368 ◽  
Author(s):  
B. X. Yang ◽  
A. H. Lumpkin
2021 ◽  
Author(s):  
Luisa Watkins ◽  
Sheila W. Seidel ◽  
Minxu Peng ◽  
Akshay Agarwal ◽  
Christopher C. Yu ◽  
...  

Author(s):  
J. Dietrich ◽  
C. Boehme ◽  
T. Weis ◽  
A.H. Botha ◽  
J.L. Conradie ◽  
...  

2014 ◽  
Vol 70 (a1) ◽  
pp. C776-C776 ◽  
Author(s):  
Elzbieta Trzop ◽  
Bertrand Fournier ◽  
Katarzyna Jarzembska ◽  
Jesse Sokolow ◽  
Radoslaw Kaminski ◽  
...  

Thanks to their potential applications as light-emitting devices, chemical sensors and dye-sensitized solar cells, heteroleptic copper (I) complexes have been extensively studied. Cu(DPPE)(DMP)·PF6(dppe= 1,2-bis(diphenylphosphino)ethane; dmp = 2,9-dimethyl-1,10-phenanthroline) crystallizes in the monoclinic system, P21/c, with two independent molecules in the asymmetric unit. Previous studies on this system [1,2] show strong temperature-dependent emission. The complex was studied at 90K under 355nm laser excitation. At this temperature, the luminescence decay for Cu(DPPE)(DMP)·PF6is biexponential with lifetimes of ~3μs and ~28μs. Two time-resolved X-ray diffraction techniques were applied for studies: (1) a Laue technique at BioCARS ID-14 beamline at the Advanced Photon Source, and (2) monochromatic diffraction at a newly constructed in-house pump-probe monochromatic facility at the University at Buffalo. Structural changes determined with the two methods are in qualitative agreement; discrepancies in position of the Cu and P atoms were observed. The molecular distortions were smaller than those determined at 16K in the earlier synchrotron study by Vorontsov et al. [2]. Photodeformation maps (see Figure below), in which the increase in temperature on photoexcitation has been eliminated, clearly illustrate the photoinduced atomic shifts for both data sets. Results will be compared with those obtained for other studied heteroleptic copper (I) complexes, for instance Cu[(1,10-phenanthroline-N,N′) bis(triphenylphosphine)]·BF4[3]. The in-house pump-probe facility is discussed by Radoslaw Kaminski at this meeting. Research funded by the National Science Foundation (CHE1213223). BioCARS Sector 14 at APS is supported by NIH (RR007707). The Advanced Photon Source is funded by the Office of Basic Energy Sciences, U.S. Department of Energy, (W-31-109-ENG-38). KNJ is supported by the Polish Ministry of Science and Higher Education through the "Mobility Plus" program.


1992 ◽  
Author(s):  
A. H. Lumpkin ◽  
G. Decker ◽  
E. Kahana ◽  
D. Patterson ◽  
W. Sellyey ◽  
...  

2010 ◽  
Author(s):  
Eric M. Dufresne ◽  
Bernhard Adams ◽  
Dohn A. Arms ◽  
Matthieu Chollet ◽  
Eric C. Landahl ◽  
...  
Keyword(s):  

2014 ◽  
Vol 70 (a1) ◽  
pp. C855-C855
Author(s):  
Karena Chapman

In the last decade, the potential of the pair distribution function (PDF) method as a versatile tool for materials characterization has expanded enormously, driven by accelerated data acquisition (from hours to sub-second) and the advent of dedicated PDF instruments, such as 11-ID-B at the Advanced Photon Source. New time-resolved, in-situ/operando, parametric, and combined experimental capabilities coupled with innovative model-independent approaches to data analysis are being developed to harness the growing potential of this methodology. For example, while the complex multicomponent architecture of batteries and their coupled electronic, chemical and structural transformations complicate investigations of functionality, through the development of new insitu PDF measurement capabilities and analytical approaches, we have been able to gain insight into the structure and reactivity of these electrochemical energy storage systems.[1] This presentation will describe recent studies of electrode reactions during cycling and the atomic structure of electrolytes.[2]


2020 ◽  
Vol 27 (1) ◽  
pp. 217-221
Author(s):  
Bi-Hsuan Lin ◽  
Yu-Hao Wu ◽  
Xiao-Yun Li ◽  
Hsu-Cheng Hsu ◽  
Yu-Cheng Chiu ◽  
...  

Time-resolved X-ray excited optical luminescence (TR-XEOL) was developed successfully for the 23A X-ray nanoprobe beamline located at the Taiwan Photon Source (TPS). The advantages of the TR-XEOL facility include (i) a nano-focused X-ray beam (<60 nm) with excellent spatial resolution and (ii) a streak camera that can simultaneously record the XEOL spectrum and decay time. Three time spans, including normal (30 ps to 2 ns), hybrid (30 ps to 310 ns) and single (30 ps to 1.72 µs) bunch modes, are available at the TPS, which can fulfil different experimental conditions involving samples with various lifetimes. It is anticipated that TR-XEOL at the TPS X-ray nanoprobe could provide great characterization capabilities for investigating the dynamics of photonic materials.


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