DEPOLARIZED RAYLEIGH SCATTERINGDEPOLARIZED RAYLEIGH AND RAMAN SCATTERING : MECHANISM OF ORIENTATIONAL MOTION IN LIQUIDS

1972 ◽  
Vol 33 (C1) ◽  
pp. C1-181-C1-181
Author(s):  
T. A. LITOVITZ
1998 ◽  
Vol 58 (20) ◽  
pp. 13619-13626 ◽  
Author(s):  
H. Siegle ◽  
A. Kaschner ◽  
A. Hoffmann ◽  
I. Broser ◽  
C. Thomsen ◽  
...  

1991 ◽  
Vol 10 (3) ◽  
pp. 389-394 ◽  
Author(s):  
D. Schwarze ◽  
H. Stolz ◽  
W. von der Osten ◽  
G. Weimann ◽  
J. Röseler ◽  
...  

A detailed theoretical treatment of the hyper Raman effect is presented. Using the density matrix treatment we derive general formulae which give information on the frequencies of the scattered radiation, the scattering mechanism and resonance processes. A hyperpolarizability theory analogous to the Placzek polarizability theory is developed and the conditions under which it is valid are established. The enhancement of intensity of hyper Raman scattering through resonance processes is discussed.


1973 ◽  
Vol 51 (15) ◽  
pp. 1657-1663 ◽  
Author(s):  
N. Krishnamurthy ◽  
B. H. Torrie

Raman scattering from single crystals of TlCl0.6Br0.4 has been observed both as a function of temperature and excitation wavelength. The spectra exhibit strong one-phonon Raman scattering at 17 and 37 cm−1 and a weak two-phonon band centered at 296 cm−1, close to twice the LO frequency (q = 0) of the mixed crystal. From the temperature dependence and the calculated one- and two-phonon densities of states, it is shown that the 37 cm−1 line and the tail following it are an admixture of first- and second-order Raman scattering. The enhancement of the intensity of the 296 cm−1 band when the exciting wavelength is decreased from 5145 Å to 4545 Å is attributed to the resonant-scattering mechanism proposed by Fontana and Mulazzi.


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