scholarly journals Size-resolved characterization of organic aerosol in the North China Plain: new insights from high resolution spectral analysis

2021 ◽  
Author(s):  
Weiqi Xu ◽  
Chun Chen ◽  
Yanmei Qiu ◽  
Conghui Xie ◽  
Yunle Chen ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
North China Plain ◽  
North China ◽  
Fine Particles ◽  
Large Fraction ◽  
Organic Aerosol ◽  
Size Distributions ◽  
The North ◽  
The Impact

Organic aerosol (OA), a large fraction of fine particles, has a large impact on climate radiative forcing and human health, and the impact depends strongly on size distributions. Here we...

McFAN experiment: An integrated analysis of the multiphase chemistry experiment in Fogs and Aerosols in the North China Plain

2020 ◽  
Author(s):  
Hang Su ◽  
Nan Ma ◽  
Yele Sun ◽  
Jiangchuan Tao ◽  
Pingqing Fu ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
Winter Season ◽  
Direct Determination ◽  
Organic Aerosol ◽  
Integrated Analysis ◽  
The North ◽  
The North China Plain ◽  
The Impact ◽  
Chemistry Experiment

<p>Fine-particle pollution associated with winter haze threatens the health of more than 400 million people in the North China Plain. The Multiphase chemistry experiment in Fogs and Aerosols in the North China Plain (McFAN) investigated the physical-chemical mechanisms leading to the haze formation with a focus on the contributions of multiphase processes in aerosol and fogs. We integrated multiple platform observations with regional and box models to identify the key oxidation process producing sulfate, nitrate and secondary organic aerosols, and their impact. A new environmental chamber was deployed to conduct kinetic experiments with real atmospheric compositions in comparison to literature kinetic data from laboratory studies. The experiments were carried out for multiple years since 2017 at the Gucheng site in the center of polluted areas and have performed experiments in the winter season. The location of the site minimizes fast transition between clean and polluted air masses (e.g., in Beijing), and helps to maintain a pollution regime representative for the North China Plain. The multi-year consecutive experiments documented the trend of PM2.5 pollution and corresponding change of aerosol physical and chemical properties, and allowed to investigate newly proposed mechanisms. The preliminary results show new proofs of the key role of aqueous phase reactions in regulating the aerosol compositions during haze events.</p><p>Reference:</p><p>Zheng et al., Exploring the severe winter haze in Beijing: the impact of synoptic weather, regional transport and heterogeneous reactions. Atmospheric Chemistry and Physics <strong>15</strong>, 2969-2983 (2015).</p><p>Cheng et al., Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China. Science Advances <strong>2</strong>,  (2016).</p><p>Li et al., Multifactor colorimetric analysis on pH-indicator papers: an optimized approach for direct determination of ambient aerosol pH. Atmos. Meas. Tech. Discuss. <strong>2019</strong>, 1-19 (2019).</p><p>Kuang et al., Distinct diurnal variation of organic aerosol hygroscopicity and its relationship with oxygenated organic aerosol. Atmos. Chem. Phys. Discuss. <strong>2019</strong>, 1-33 (2019).</p><p> </p>

scholarly journals Impact of crop field burning and mountains on heavy haze in the North China Plain: A case study

2016 ◽  
Author(s):  
X. Long ◽  
X. X. Tie ◽  
J. J. Cao ◽  
R. J. Huang ◽  
T. Feng ◽  
...  
Keyword(s):  
Air Pollution ◽  
North China Plain ◽  
North China ◽  
Wind Condition ◽  
Beijing City ◽  
The North ◽  
The North China Plain ◽  
Crop Field ◽  
The Impact ◽  
Field Burning

Abstract. Crop field burning (CFB) has important effects on air pollution in China, but it is seldom quantified and reported in a regional scale, which is of great importance for the control strategies of CFB in China, especially in the North China Plain (NCP). With the provincial statistical data and open crop fires captured by satellite (MODIS), we extracted a detailed emission inventory of CFB during a heavy haze event from 6th to 12th October 2014. A regional dynamical and chemical model (WRF-Chem) was applied to investigate the impact of CFB on air pollution in NCP. The model simulations were compared with the in situ measurements of PM2.5 (particular matter with radius less than 2.5 μm) concentrations. The model evaluation shows that the correlation coefficients (R) between measured and calculated values exceeds 0.80 and absolute normalized mean bias (NMB) is no more than 14 %. In addition, the simulated meteorological parameters such as winds and planetary boundary layer height (PBLH) are also in good agreement with observations. The model was intensive used to study (1) the impacts of CFB and (2) the effect of mountains on regional air quality. The results show that the CFB occurred in southern NCP (SNCP) had significant effect on PM2.5 concentrations locally, causing a maximum of 35 % PM2.5 increase in SNCP. Because of south wind condition, the CFB pollution plume is subjective a long transport to northern NCP (NNCP-with several mega cities, including Beijing of the capital city in China), where there are no significant CFB occurrences, causing a maximum of 32 % PM2.5 increase in NNCP. As a result, the heavy haze in Beijing is enhanced by the CFB occurred in SNCP. Further more, there are two major mountains located in the western and northern NCP. Under the south wind condition, these mountains play important roles in enhancing the PM2.5 pollution in NNCP through the blocking and guiding effects. This study suggests that the PM2.5 emissions in SNCP region should be significantly limited in order to reduce the occurrences of heavy haze events in NNCP region, including the Beijing City.

scholarly journals Summertime fine particulate nitrate pollution in the North China Plain: Increasing trends, formation mechanisms, and implications for control policy

2018 ◽  
Author(s):  
Liang Wen ◽  
Likun Xue ◽  
Xinfeng Wang ◽  
Caihong Xu ◽  
Tianshu Chen ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
Fine Particles ◽  
Nitrate Pollution ◽  
Effective Control ◽  
Formation Mechanisms ◽  
The North ◽  
The North China Plain ◽  
Holistic Understanding ◽  
Nitrate Aerosol

Abstract. Nitrate aerosol composes a significant fraction of fine particles and plays a key role in regional air quality and climate. To obtain a holistic understanding of the nitrate pollution and its formation mechanisms over the North China Plain (NCP) – the most industrialized and polluted region in northern China, intensive field observations were conducted at three sites during summertime in 2014–2015. The measurement sites include the downtown and downwind of Ji'nan, the capital city of Shandong Province, as well as the peak of NCP – Mt. Tai (1534 m a.s.l.), and hence cover representative urban, rural and remote areas of the region. Elevated nitrate concentrations were observed at all three sites despite distinct temporal and spatial variations. The nitrate / PM2.5 and nitrate / sulfate ratios have significantly increased in Ji'nan (2005–2015) and at Mt. Tai (from 2007 to 2014), indicating the worsening situation of regional nitrate pollution. A multi-phase chemical box model (RACM/CAPRAM) was deployed and constrained by observations to elucidate the nitrate formation mechanisms. The principal formation route is the partitioning of gaseous HNO3 to aerosol phase at daytime, whilst the nocturnal nitrate formation is dominated by the heterogeneous hydrolysis of N2O5. The daytime nitrate production in the NCP region is mainly limited by the availability of NO2 and to a lesser extent O3 and NH3, and the nighttime formation is controlled by both NO2 and O3. NH3 prompts significantly the nitrate formation at daytime but plays a slightly negative role in the nighttime. Our analyses suggest that controlling NOx and O3 is an efficient way at the moment to mitigate nitrate pollution in the NCP region, where NH3 is usually in excess in summer. This study provides observational evidence of rising trend of nitrate aerosol as well as scientific support for formulating effective control strategies for regional haze in China.

Photochemical Aqueous-Phase Reactions Induce Rapid Daytime Formation of Oxygenated Organic Aerosol on the North China Plain

2020 ◽  
Vol 54 (7) ◽  
pp. 3849-3860 ◽  
Author(s):  
Ye Kuang ◽  
Yao He ◽  
Wanyun Xu ◽  
Bin Yuan ◽  
Gen Zhang ◽  
...  
Keyword(s):  
Aqueous Phase ◽  
North China Plain ◽  
North China ◽  
Organic Aerosol ◽  
The North ◽  
The North China Plain

Aerosol chemical compositions in the North China Plain and the impact on the visibility in Beijing and Tianjin

2018 ◽  
Vol 201 ◽  
pp. 235-246 ◽  
Author(s):  
Jianan Zou ◽  
Zirui Liu ◽  
Bo Hu ◽  
Xiaojuan Huang ◽  
Tianxue Wen ◽  
...  
Keyword(s):  
North China Plain ◽  
North China ◽  
Chemical Compositions ◽  
The North ◽  
The North China Plain ◽  
The Impact

Impact of the methods of groundwater access on irrigation and crop yield in the North China Plain

2016 ◽  
Vol 8 (4) ◽  
pp. 613-633 ◽  
Author(s):  
Lijuan Zhang ◽  
Jinxia Wang ◽  
Guangsheng Zhang ◽  
Qiuqiong Huang
Keyword(s):  
Crop Yield ◽  
North China Plain ◽  
North China ◽  
Climate Factors ◽  
Groundwater Use ◽  
Content Type ◽  
The North ◽  
The North China Plain ◽  
Groundwater Markets ◽  
The Impact

Purpose The purpose of this paper is: to track the methods by which farmers access groundwater for irrigation in the North China Plain (NCP); to explore whether climate factors influence farmers’ decisions on the methods of groundwater access for irrigation; and to examine whether the amount of groundwater use for irrigation and crop yield systematically differ across groups of farmers using various methods of groundwater access, and how climate factors affect them. Design/methodology/approach Descriptive statistical analysis and econometric models are used on household survey data collected over several years and county-level climate data. Findings Over the past few decades, a significant share of farmers have switched the methods of groundwater access from collective tubewells to own tubewells or groundwater markets. Farmers who bought water from groundwater markets applied less water to wheat plots than those who had their own tubewells. However, wheat yield was not negatively affected. Both average climate conditions and long-term variations were found to be related to farmers’ choice of methods of groundwater access for irrigation. More frequent droughts and increasingly volatile temperatures both increased the likelihood of farmers gaining groundwater irrigation from markets. Originality/value The analysis results suggest farmers are using groundwater markets to help them adapt to climate change. Applying empirical analysis to identify the impact of the methods by which farmers access groundwater for irrigation on the amount of groundwater use and crop yield will help policy makers design reasonable adaptation policies for the NCP.

Carbonaceous components in particulate matter during a haze episode at a typical industrial area in the North China Plain

2020 ◽  
Vol ahead-of-print (ahead-of-print) ◽  
Author(s):  
Hongya Niu ◽  
Zhaoce Liu ◽  
Wei Hu ◽  
Wenjing Cheng ◽  
Mengren Li ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Organic Carbon ◽  
North China Plain ◽  
North China ◽  
Large Fraction ◽  
Industrial Emissions ◽  
Content Type ◽  
The North ◽  
The North China Plain ◽  
The Mean

Purpose Severe airborne particulate pollution frequently occurs over the North China Plain (NCP) region in recent years. To better understand the characteristics of carbonaceous components in particulate matter (PM) over the NCP region. Design/methodology/approach PM samples were collected at a typical area affected by industrial emissions in Handan, in January 2016. The concentrations of organic carbon (OC) and elemental carbon (EC) in PM of different size ranges (i.e. PM2.5, PM10 and TSP) were measured. The concentrations of secondary organic carbon (SOC) were estimated by the EC tracer method. Findings The results show that the concentration of OC ranged from 14.9 μg m−3 to 108.4 μg m−3, and that of EC ranged from 4.0 μg m−3 to 19.4μg m−3, when PM2.5 changed from 58.0μg m−3 to 251.1μg m−3 during haze days, and the carbonaceous aerosols most distributed in PM2.5 rather than large fraction. The concentrations of OC and EC PM2.5 correlated better (r = 0.7) than in PM2.5−10 and PM>10, implying that primary emissions were dominant sources of OC and EC in PM2.5. The mean ratios of OC/EC in PM2.5, PM2.5–10 and PM>10 were 4.4 ± 2.1, 3.6 ± 0.9 and 1.9 ± 0.7, respectively. Based on estimation, SOC accounted for 16.3%, 22.0% and 9.1% in PM2.5, PM2.5–10 and PM>10 respectively. Originality/value The ratio of SOC/OC (48.2%) in PM2.5 was higher in Handan than those (28%–32%) in other megacities, e.g. Beijing, Tianjin and Shijiazhuang in the NCP, suggesting that the formation of SOC contributed significantly to OC. The mean mass absorption efficiencies of EC (MACEC) in PM10 and TSP were 3.4 m2 g−1 (1.9–6.6 m2 g−1) and 2.9 m2 g−1 (1.6–5.6 m2 g−1), respectively, both of which had similar variation patterns to those of OC/EC and SOC/OC.

scholarly journals Study on the Change Characteristics of and Population Exposure to Heatwave Events on the North China Plain

2019 ◽  
Vol 2019 ◽  
pp. 1-10
Author(s):  
Long-Fei Zhan ◽  
Yanjun Wang ◽  
Hemin Sun ◽  
Jianqing Zhai ◽  
Mingjin Zhan
Keyword(s):  
North China Plain ◽  
North China ◽  
Climatic Factors ◽  
Demographic Data ◽  
Population Exposure ◽  
Central Position ◽  
Daily Maximum ◽  
The North ◽  
The North China Plain ◽  
The Impact

In accordance with the China Meteorological Administration definition, this study considered a weather process with a maximum surface temperature of ≥35°C for more than three consecutive days as a heatwave event. Based on a dataset of daily maximum temperatures from meteorological stations on the North China Plain, including ordinary and national basic/reference surface stations, the intensity-area-duration method was used to analyze the spatiotemporal distribution characteristics of heatwave events on the North China Plain (1961–2017). Moreover, based on demographic data from the Statistical Yearbook and Greenhouse Gas Initiative (GGI) Population Scenario Database of the Austrian Institute for International Applied Systems Analysis (IIASA), population exposure to heatwave events was also studied. The results showed that the frequency, intensity, and area of impact of heatwave events on the North China Plain initially decreased (becoming weaker and less extensive) and then increased (becoming stronger and more extensive). Similarly, the trend of population exposure to heatwave events initially decreased and then increased, and the central position of exposure initially moved southward and then returned northward. Population exposure in the eastern Taihang Mountains was found significantly higher than in the western Taihang Mountains. In relation to the change of population exposure to heatwave events on the North China Plain, the influence of climatic factors was found dominant with an absolute contribution rate of >75%. Except for 2011–2017, increase in population also increased the exposure to heatwaves, particularly in the first half of the study period. Interaction between climatic and population factors generally had less impact on population exposure than either climatic factors or population factors alone. This study demonstrated a method for assessing the impact of heatwave events on population exposure, which could form a scientific basis for the development of government policy regarding adaption to climate change.

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