Creation of carbon-defects and in-plane holes with the assistance of NH4Br to enhance the photocatalytic activity of g-C3N4

Author(s):  
Guiyang Yu ◽  
Haitao Zhao ◽  
Chuanwang Xing ◽  
Luyan Guo ◽  
Xiyou Li

Microstructure modulation is an effective strategy to improve photocatalytic efficiency of graphitic carbon nitride (g-C3N4) for solar energy conversion. In the present work, abundant carbon defects and holes in g-C3N4...

Author(s):  
Huilin Hou ◽  
Gang Shao ◽  
Weiyou Yang

As one of fascinating visible-light-responsive photocatalysts, the two-dimensional (2D) graphitic carbon nitride (g-C3N4) has drawn broad attention in the field of solar energy conversion and environmental remediation. However, its intrinsic...


RSC Advances ◽  
2016 ◽  
Vol 6 (89) ◽  
pp. 86688-86694 ◽  
Author(s):  
Lan-Rong Zou ◽  
Gui-Fang Huang ◽  
Dong-Feng Li ◽  
Jin-Hua Liu ◽  
An-Lian Pan ◽  
...  

A graphitic carbon nitride (g-C3N4) nanosheet and its nanocomposites have recently attracted increasing interest due to their massive potentials in applications ranging from fluorescence imaging to solar energy conversion.


2018 ◽  
Vol 8 (18) ◽  
pp. 4576-4599 ◽  
Author(s):  
Waheed Iqbal ◽  
Bo Yang ◽  
Xu Zhao ◽  
Muhammad Rauf ◽  
Muhammad Waqas ◽  
...  

This review discusses advances in the synthesis and design of g-C3N4-based nanomaterials and their various photocatalytic and photoredox applications.


2021 ◽  
Vol 22 (23) ◽  
pp. 13096
Author(s):  
Daria Baranowska ◽  
Tomasz Kędzierski ◽  
Małgorzata Aleksandrzak ◽  
Ewa Mijowska ◽  
Beata Zielińska

In this contribution, the effect of hydrogenation conditions atmosphere (temperature and time) on physicochemical properties and photocatalytic efficiency of graphitic carbon nitride (g-C3N4, gCN) was studied in great details. The changes in the morphology, chemical structure, optical and electrochemical properties were carefully investigated. Interestingly, the as-modified samples exhibited boosted photocatalytic degradation of Rhodamine B (RhB) with the assistance of visible light irradiation. Among modified gCN, the sample annealed at 500 °C for 4 h (500-4) in H2 atmosphere exhibited the highest photocatalytic activity—1.76 times higher compared to pristine gCN. Additionally, this sample presented high stability and durability after four cycles. It was noticed that treating gCN with hydrogen at elevated temperatures caused the creation of nitrogen vacancies on gCN surfaces acting as highly active sites enhancing the specific surface area and improving the mobility of photogenerated charge carriers leading to accelerating the photocatalytic activity. Therefore, it is believed that detailed optimization of thermal treatment in a hydrogen atmosphere is a facile approach to boost the photoactivity of gCN.


RSC Advances ◽  
2017 ◽  
Vol 7 (25) ◽  
pp. 15390-15396 ◽  
Author(s):  
Yasir A. Haleem ◽  
Qun He ◽  
Daobin Liu ◽  
Changda Wang ◽  
Weiyu Xu ◽  
...  

The hydrogen evolution reaction (HER) may contribute substantially to energy resources in the future through solar energy conversion.


EnergyChem ◽  
2021 ◽  
Vol 3 (2) ◽  
pp. 100051
Author(s):  
Chuanbiao Bie ◽  
Bei Cheng ◽  
Jiajie Fan ◽  
Wingkei Ho ◽  
Jiaguo Yu

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