Vertical growth of SnS2 nanobelt arrays on CuSbS2 nanosheets for enhanced photocatalytic reduction of CO2

2021 ◽  
Vol 57 (80) ◽  
pp. 10419-10422
Author(s):  
Wenhao Li ◽  
Quanlong Xu ◽  
Wei Chen ◽  
Faliang Gou ◽  
Shujing Zhou ◽  
...  

Two-dimensional SnS2 nanobelt arrays vertically grown on two-dimensional CuSbS2 nanosheet heterostructures showed enhanced photocatalytic activity for CO2 reduction.

2018 ◽  
Vol 6 (11) ◽  
pp. 4768-4775 ◽  
Author(s):  
Mang Wang ◽  
Jinxuan Liu ◽  
Chunmei Guo ◽  
Xiaosu Gao ◽  
Chenghuan Gong ◽  
...  

The two-dimensional ZIF-67 with a leaf-like morphology exhibited the best photocatalytic activity and stability due to the highest CO2 adsorption capability and efficient electron transfer from the excited [Ru(bpy)3]2+ to ZIF-67.


Catalysts ◽  
2018 ◽  
Vol 8 (12) ◽  
pp. 581 ◽  
Author(s):  
Sonam Goyal ◽  
Maizatul Shaharun ◽  
Chong Kait ◽  
Bawadi Abdullah ◽  
Mariam Ameen

The efficient reduction of CO2 into valuable products such as methanol, over metal-organic frameworks (MOFs) based catalyst, has received much attention. The photocatalytic reduction is considered the most economical method due to the utilization of solar energy. In this study, Copper (II)/Zeolitic Imidazolate Framework-8 (Cu/ZIF-8) catalysts were synthesized via a hydrothermal method for photocatalytic reduction of CO2 to methanol. The synthesized catalysts were characterized by X-ray Photoelectron Spectroscopy (XPS), Field Emission Scanning Electron Microscopy (FESEM) coupled with Energy Dispersive X-ray (EDX), Ultraviolet-visible (UV-vis) spectroscopy, and X-Ray Diffraction (XRD). The host ZIF-8, treated with 2 mmol copper prepared in 2M ammonium hydroxide solution showed the highest photocatalytic activity. The crystal structures of ZIF-8 and 2Cu/ZIF-8N2 catalysts were observed as cubic and orthorhombic, respectively and the XPS analysis confirmed the deposition of Cu (II) ions over ZIF-8 surface among all the prepared catalysts. The orthorhombic structure, nano-sized crystals, morphology and Cu loading of the 2Cu/ZIF-8N2 catalyst were the core factors to influence the photocatalytic activity. The yield of Methanol was found to be 35.82 µmol/L·g after 6 h of irradiations on 2Cu/ZIF-8N2 catalyst in the wavelength range between 530–580 nm. The copper-based ZIF-8 catalyst has proven as an alternative approach for the economical photocatalytic reduction of CO2 to CH3OH.


2015 ◽  
Vol 51 (36) ◽  
pp. 7645-7648 ◽  
Author(s):  
Mu Li ◽  
Peng Li ◽  
Kun Chang ◽  
Tao Wang ◽  
Lequan Liu ◽  
...  

An efficient and stable photocatalytic activity was obtained over NaTaO3 by introducing electron donor (H2) into the CO2 reduction process with water and loaded Ru as cocatalysts. The main effect of the electron donor was found to release the peroxide intermediates of the half reaction for water oxidation.


2021 ◽  
Author(s):  
Shiyan Wang ◽  
Xiaowan Bai ◽  
Qiang Li ◽  
Yixin Ouyang ◽  
Li Shi ◽  
...  

Solar-driven high-efficient photocatalytic reduction of CO2 into value-added fuel has been regarded as a promising strategy to assuage current global warming and energy crisis, while developing highly product-selective, long-term stable...


2020 ◽  
Vol 8 (37) ◽  
pp. 19156-19195 ◽  
Author(s):  
Deyu Qin ◽  
Yin Zhou ◽  
Wenjun Wang ◽  
Chen Zhang ◽  
Guangming Zeng ◽  
...  

This review systematically summarizes the recent advances in two-dimensional nanomaterials for photocatalytic reduction of CO2 and its related mechanisms.


2018 ◽  
Vol 7 (1) ◽  
pp. 650-659 ◽  
Author(s):  
Houde She ◽  
Hua Zhou ◽  
Liangshan Li ◽  
Ziwei Zhao ◽  
Man Jiang ◽  
...  

2019 ◽  
Vol 55 (77) ◽  
pp. 11523-11526 ◽  
Author(s):  
Zi-Cheng Fu ◽  
Joshua T. Moore ◽  
Fei Liang ◽  
Wen-Fu Fu

Hybrid catalysts that cobalt oxide nanoparticles immobilized on outside surfaces of spherical SBA-15 presented unexpected photocatalytic activity towards CO2-to-CO conversion.


2017 ◽  
Vol 41 (13) ◽  
pp. 5660-5668 ◽  
Author(s):  
Quang Duc Truong ◽  
Huu Thu Hoa ◽  
Dai-Viet N. Vo ◽  
Thanh Son Le

Anatase titania with tunable shapes has been synthesized by a facile hydrothermal method using peroxotitanic acid as a precursor. The results of investigations showed that the photocatalytic activity in the reduction of CO2 to methanol increased with an increase in the percentage of {001} surfaces.


2016 ◽  
Vol 18 (5) ◽  
pp. 1355-1363 ◽  
Author(s):  
Shuying Zhu ◽  
Shijing Liang ◽  
Jinhong Bi ◽  
Minghua Liu ◽  
Limin Zhou ◽  
...  

Ultrathin SnNb2O6 2D nanosheets could be used as an efficient photocatalyst for the reduction of CO2 to methane and exhibit much higher photocatalytic activity than that of the bulk counterpart due to the unique structural features.


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