Visible-light-responsive Z-scheme system for photocatalytic lignocelluloses-to-H2 conversion

2021 ◽  
Author(s):  
Qing-Yu Liu ◽  
Hao-dong Wang ◽  
Yong-Jun Yuan ◽  
Rui Tang ◽  
Liang Bao ◽  
...  

Z-scheme system was successfully constructed for visible light driven photocatalytic H2 production from lignocelluloses, the highest H2 evolution rate of this Z-scheme system achieves 5.3 and 1.6 μmol•h-1 in α-celluloses...

2021 ◽  
Vol 11 (22) ◽  
pp. 10854
Author(s):  
Jingyun Mao ◽  
Huiling Zhong ◽  
Xinpin Liu ◽  
Qingrong Qian ◽  
Yongjin Luo ◽  
...  

The development of a facile method for the synthesis of GaN:ZnO solid solution, an attractive material with a wurtzite-type structure, is vital to enhance its photocatalytic activity toward H2 evolution. Herein, GaN:ZnO solid solution nanorods with diameters of around 180 nm were fabricated by combining the electro-spun method with a sequentially calcinating process. Photocatalytic water-splitting activities of the as-obtained samples loaded with Rh2−yCryO3 co-catalyst were estimated by H2 evolution under visible-light irradiation. The as-prepared GaN:ZnO nanorods at a nitridation temperature of 850 °C showed the optimal performance. Careful characterization of the GaN:ZnO solid solution nanorods indicated that the nitridation temperature is an important parameter affecting the photocatalytic performance, which is related to the specific surface area and the absorbable visible-light wavelength range. Finally, the mechanism of the GaN:ZnO solid solution nanorods was also investigated. The proposed synthesis strategy paves a new way to realize excellent activity and recyclability of GaN:ZnO solid solution nanorod photocatalysts for hydrogen generation.


2021 ◽  
Vol MA2021-01 (39) ◽  
pp. 1244-1244
Author(s):  
Zejie Chen ◽  
Kenta Watanabe ◽  
Robert Stinson ◽  
Luisa Barrera ◽  
Sam Keene ◽  
...  

2018 ◽  
Vol 130 (50) ◽  
pp. 16685-16689 ◽  
Author(s):  
Jin Wang ◽  
Tong Xia ◽  
Lei Wang ◽  
Xusheng Zheng ◽  
Zeming Qi ◽  
...  

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