Cotton pad-derived large-area 3D N-doped graphene-like full carbon cathode with an O-rich functional group for flexible all solid Zn–air batteries

2020 ◽  
Vol 8 (22) ◽  
pp. 11202-11209 ◽  
Author(s):  
Xiangjun Zheng ◽  
Xuecheng Cao ◽  
Kai Zeng ◽  
Zhihui Sun ◽  
Jin Yan ◽  
...  

A flexible 3D N, O-doped graphene-like full carbon cathode has been synthesized with a cotton pad as a template via a scalable and one-step pyrolysis process, and can be directly used as an efficient air cathode for flexible all solid-state ZABs.

Nanoscale ◽  
2018 ◽  
Vol 10 (9) ◽  
pp. 4391-4397 ◽  
Author(s):  
Ivan Esteve-Adell ◽  
Jinbao He ◽  
Fernando Ramiro ◽  
Pedro Atienzar ◽  
Ana Primo ◽  
...  

A procedure for the one-step preparation of films of few-layer N-doped graphene on top of nanometric hexagonal boron nitride sheets based on the pyrolysis at 900 °C under an inert atmosphere is reported.


2019 ◽  
Vol 7 (13) ◽  
pp. 7591-7603 ◽  
Author(s):  
Liya Ma ◽  
Jin Liu ◽  
Song Lv ◽  
Qin Zhou ◽  
Xinyu Shen ◽  
...  

N,S co-doped graphene-enhanced HPC is prepared by a facile one-step method, and exhibits superior electrochemical performances as a solid-state supercapacitor electrode.


RSC Advances ◽  
2021 ◽  
Vol 11 (63) ◽  
pp. 40059-40071
Author(s):  
Hurmus Gursu ◽  
Yağmur Guner ◽  
Melih Besir Arvas ◽  
Kamil Burak Dermenci ◽  
Umut Savaci ◽  
...  

In this study, the one-step electrochemical preparation of chlorine doped and chlorine-oxygen containing functional group doped graphene-based powders was carried out by Yucel's method, with the resultant materials used as anode materials for lithium (Li)-ion batteries.


2014 ◽  
Vol 2 (14) ◽  
pp. 2510-2516 ◽  
Author(s):  
Amrita Kumar ◽  
Michael T. Otley ◽  
Fahad Alhasmi Alamar ◽  
Yumin Zhu ◽  
Blaise G. Arden ◽  
...  

The establishment of a relationship between device performance parameters is reported here for a versatile one-step preparation method of a large area solid-state electrochromic device.


2018 ◽  
Vol 2 (9) ◽  
pp. 1692-1699 ◽  
Author(s):  
Xiao-Man Cao ◽  
Zhi-Jia Sun ◽  
Si-Yu Zhao ◽  
Bing Wang ◽  
Zheng-Bo Han

Novel 3D sponge-like hierarchical porous carbons using different-sized MOFs (Zn(tbip)) as precursors are successfully prepared via a one-step pyrolysis process, and are promising for application in high-performance flexible all-solid-state supercapacitors.


2020 ◽  
Author(s):  
Baojian Xiong ◽  
Yue Li ◽  
Yin Wei ◽  
Søren Kramer ◽  
Zhong Lian

Cross-coupling between substrates that can be easily derived from phenols is highly attractive due to the abundance and low cost of phenols. Here, we report a dual nickel/palladium-catalyzed reductive cross-coupling between aryl tosylates and aryl triflates; both substrates can be accessed in just one step from readily available phenols. The reaction has a broad functional group tolerance and substrate scope (>60 examples). Furthermore, it displays low sensitivity to steric effects demonstrated by the synthesis of a 2,2’disubstituted biaryl and a fully substituted aryl product. The widespread presence of phenols in natural products and pharmaceuticals allow for straightforward late-stage functionalization, illustrated with examples such as Ezetimibe and tyrosine. NMR spectroscopy and DFT calculations indicate that the nickel catalyst is responsible for activating the aryl triflate, while the palladium catalyst preferentially reacts with the aryl tosylate.


2021 ◽  
Vol 129 (24) ◽  
pp. 245303
Author(s):  
Fan Xu ◽  
Yujiao Li ◽  
Beilei Yuan ◽  
Yongzheng Zhang ◽  
Haoming Wei ◽  
...  

Nanomaterials ◽  
2021 ◽  
Vol 11 (1) ◽  
pp. 202
Author(s):  
Yexin Dai ◽  
Jie Ding ◽  
Jingyu Li ◽  
Yang Li ◽  
Yanping Zong ◽  
...  

In this work, reduced graphene oxide (rGO) nanocomposites doped with nitrogen (N), sulfur (S) and transitional metal (Ni, Co, Fe) were synthesized by using a simple one-step in-situ hydrothermal approach. Electrochemical characterization showed that rGO-NS-Ni was the most prominent catalyst for glucose oxidation. The current density of the direct glucose alkaline fuel cell (DGAFC) with rGO-NS-Ni as the anode catalyst reached 148.0 mA/cm2, which was 40.82% higher than the blank group. The DGAFC exhibited a maximum power density of 48 W/m2, which was more than 2.08 folds than that of blank group. The catalyst was further characterized by SEM, XPS and Raman. It was speculated that the boosted performance was due to the synergistic effect of N, S-doped rGO and the metallic redox couples, (Ni2+/Ni3+, Co2+/Co3+ and Fe2+/Fe3+), which created more active sites and accelerated electron transfer. This research can provide insights for the development of environmental benign catalysts and promote the application of the DGAFCs.


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