Mechanical Tough yet Self-Healing Transparent Conductive Elastomers through Synergic Dual Cross-Linking Strategy

2021 ◽  
Author(s):  
Qiankun Zhang ◽  
Guangxue Chen ◽  
Ren'ai Li ◽  
Liang Lin ◽  
He minghui

Simultaneous achieving transparency, high mechanical strength and self-healing in conductive elastomers with simple and green features is a challenge. Here we develop a novel strategy for a tough yet self-healing...

Sensors ◽  
2021 ◽  
Vol 21 (11) ◽  
pp. 3574
Author(s):  
Pejman Heidarian ◽  
Hossein Yousefi ◽  
Akif Kaynak ◽  
Mariana Paulino ◽  
Saleh Gharaie ◽  
...  

Electroconductive hydrogels with stimuli-free self-healing and self-recovery (SELF) properties and high mechanical strength for wearable strain sensors is an area of intensive research activity at the moment. Most electroconductive hydrogels, however, consist of static bonds for mechanical strength and dynamic bonds for SELF performance, presenting a challenge to improve both properties into one single hydrogel. An alternative strategy to successfully incorporate both properties into one system is via the use of stiff or rigid, yet dynamic nano-materials. In this work, a nano-hybrid modifier derived from nano-chitin coated with ferric ions and tannic acid (TA/Fe@ChNFs) is blended into a starch/polyvinyl alcohol/polyacrylic acid (St/PVA/PAA) hydrogel. It is hypothesized that the TA/Fe@ChNFs nanohybrid imparts both mechanical strength and stimuli-free SELF properties to the hydrogel via dynamic catecholato-metal coordination bonds. Additionally, the catechol groups of TA provide mussel-inspired adhesion properties to the hydrogel. Due to its electroconductivity, toughness, stimuli-free SELF properties, and self-adhesiveness, a prototype soft wearable strain sensor is created using this hydrogel and subsequently tested.


Author(s):  
Chunyang Bao ◽  
Xuhao Zhang ◽  
Pengdong Yu ◽  
Qingzhong Li ◽  
Yusheng Qin ◽  
...  

Degradable polymers that play an increasingly important role in the development of sustainable society are highly demanded to feature not only high mechanical strength, but also exhibit superior toughness. Herein,...


Author(s):  
Liangliang Xia ◽  
Ming Zhou ◽  
Hongjun Tu ◽  
wen Zeng ◽  
xiaoling Yang ◽  
...  

The preparation of room-temperature self-healing polymeric materials with good healing efficiency and high mechanical strength is challenging. Two processes are essential to realise the room-temperature self-healing of materials: (a) a...


2019 ◽  
Vol 3 (3) ◽  
pp. 464-471 ◽  
Author(s):  
Jing Cui ◽  
Zhe Ma ◽  
Li Pan ◽  
Chun-Hua An ◽  
Jing Liu ◽  
...  

Synergistic hard/soft gradient distribution and dynamic ionic interactions impart high mechanical strength, toughness, stretchability and tenacious self-healing ability to copolymers.


Author(s):  
Kaili Zhang ◽  
Ren'ai Li ◽  
Guangxue Chen ◽  
Yang Jimin ◽  
Junfei Tian ◽  
...  

Conductive elastomers (CEs)with strong mechanical properties have been fabricated and used in flexible electronics. However, the development of CEs with both super-high mechanical strength and extreme stretchability remains challenging. This...


2016 ◽  
Vol 49 (19) ◽  
pp. 7442-7449 ◽  
Author(s):  
Cigdem Bilici ◽  
Volkan Can ◽  
Ulrich Nöchel ◽  
Marc Behl ◽  
Andreas Lendlein ◽  
...  

2020 ◽  
Vol 8 (7) ◽  
pp. 3667-3675 ◽  
Author(s):  
Siheng Li ◽  
Hongyu Pan ◽  
Yuting Wang ◽  
Junqi Sun

Hydrogel-based self-healing ionic skins possess high mechanical strength, excellent resilience, anti-freezing properties and high sensitivity and can heal fatigue and mechanical damage to restore the original sensing performance.


2018 ◽  
Vol 57 (29) ◽  
pp. 9008-9012 ◽  
Author(s):  
Zhifang Wang ◽  
Yipeng Ren ◽  
Ye Zhu ◽  
Lijing Hao ◽  
Yunhua Chen ◽  
...  

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