Pyrite-type ruthenium disulfide with tunable disorder and defects enables ultra-efficient overall water splitting

2019 ◽  
Vol 7 (23) ◽  
pp. 14222-14232 ◽  
Author(s):  
Yinlong Zhu ◽  
Hassan A. Tahini ◽  
Yang Wang ◽  
Qian Lin ◽  
Yan Liang ◽  
...  

Synergistic disorder and defect engineering in ruthenium disulfide enables efficient water splitting with an ultralow cell voltage of 1.527 V.

2021 ◽  
Vol 13 (35) ◽  
pp. 41545-41554
Author(s):  
Xuesong Liu ◽  
Peng Liu ◽  
Feifei Wang ◽  
Xingbin Lv ◽  
Tao Yang ◽  
...  

2021 ◽  
Vol 45 (1) ◽  
pp. 351-357
Author(s):  
Dandan Chen ◽  
Yingdong Chen ◽  
Wei Zhang ◽  
Rui Cao

The prepared electrode (NiSe-TMEDA/CC) from single-molecule electrodeposition is functional for both the OER and HER and shows a superior performance for overall water splitting with a low cell voltage in alkaline medium.


2019 ◽  
Vol 7 (19) ◽  
pp. 12325-12332 ◽  
Author(s):  
Xiuming Bu ◽  
Renjie Wei ◽  
Wei Gao ◽  
Changyong Lan ◽  
Johnny C. Ho

A unique sandwich structure of CoMnP/Ni2P/NiFe is successfully achieved by introducing a Ni2P interlayer between CoMnP nanosheets and NiFe foam to achieve an excellent bifunctional electrocatalyst, yielding a low cell voltage of only 1.48 V at 10 mA cm−2 for overall water splitting in alkaline media.


2020 ◽  
Vol 4 (1) ◽  
pp. 312-323 ◽  
Author(s):  
Harsharaj S. Jadhav ◽  
Animesh Roy ◽  
Bezawit Z. Desalegan ◽  
Jeong Gil Seo

A room-temperature synthesized NiFeCe2 electrocatalyst delivered a current density of 10 mA cm−2 at a cell voltage of 1.59 V when used as the electrolyzer.


Author(s):  
Wei Ma ◽  
Jiajia Ge ◽  
Jin You Zheng ◽  
Jiangwei Zhang ◽  
Suyu Jiang ◽  
...  

Exploring efficient electrocatalysts through controllable defect engineering in materials with low-cost and earth-abundant elements is highly desired for overall water splitting. Herein, a hybrid electrocatalyst was accomplished by growing layered...


Materials ◽  
2019 ◽  
Vol 12 (18) ◽  
pp. 3028 ◽  
Author(s):  
Hai-Bin Wang ◽  
Jia-Qi Wang ◽  
Neli Mintcheva ◽  
Min Wang ◽  
Shuang Li ◽  
...  

Engineering surface structure of catalysts is an efficient way towards high catalytic performance. Here, we report on the synthesis of regular iridium nanospheres (Ir NSs), with abundant atomic steps prepared by a laser ablation technique. Atomic steps, consisting of one-atom level covering the surface of such Ir NSs, were observed by aberration-corrected high-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM). The prepared Ir NSs exhibited remarkably enhanced activity both for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) in acidic medium. As a bifunctional catalyst for overall water splitting, they achieved a cell voltage of 1.535 V @ 10 mA/cm2, which is much lower than that of Pt/C-Ir/C couple (1.630 V @ 10 mA/cm2).


Author(s):  
Ali Saad ◽  
Zhixing Cheng ◽  
Hangjia Shen ◽  
Haichuan Guo ◽  
John Paul Attfield ◽  
...  

3-D mesoporous triphasic cobalt–copper phosphides is used as highly efficient bifunctional, stable electrocatalyst for water-alkali electrolyzers. This offers a lower cell voltage when compared to noble-metal-based Pt/C–IrO2/C.


2019 ◽  
Vol 7 (20) ◽  
pp. 12440-12445 ◽  
Author(s):  
Weiju Hao ◽  
Renbing Wu ◽  
Hongyuan Yang ◽  
Yanhui Guo

An overall water splitting device assembled using a photothermal effect coupled Ni–W–B/carbon cloth electrode could deliver a current density of 25 mA cm−2 at an ultralow cell voltage of 1.524 V without heating the whole system, which is comparable to its performance at an elevated cell temperature of 50 °C.


ACS Catalysis ◽  
2021 ◽  
pp. 11429-11439
Author(s):  
Yalei Qin ◽  
Fan Fang ◽  
Zhengzheng Xie ◽  
Huiwen Lin ◽  
Kai Zhang ◽  
...  

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