Carbon nitride as a new way to facilitate the next generation of carbon-based supercapacitors

2019 ◽  
Vol 3 (9) ◽  
pp. 2176-2204 ◽  
Author(s):  
Mostafa Ghaemmaghami ◽  
Rahim Mohammadi

As an earth-abundant material, graphitic carbon nitride has become a new research hotspot and drawn broad interdisciplinary attention in the area of energy storage and conversion and it showed great potential for application in supercapacitors.

2013 ◽  
Vol 117 (12) ◽  
pp. 6055-6059 ◽  
Author(s):  
Menghao Wu ◽  
Qian Wang ◽  
Qiang Sun ◽  
Puru Jena

Materials ◽  
2020 ◽  
Vol 13 (13) ◽  
pp. 3038
Author(s):  
Michal Baudys ◽  
Šárka Paušová ◽  
Petr Praus ◽  
Vlasta Brezová ◽  
Dana Dvoranová ◽  
...  

Graphitic carbon nitride (g-C3N4) is a conjugated polymer, which recently drew a lot of attention as a metal-free and UV and visible light responsive photocatalyst in the field of solar energy conversion and environmental remediation. This is due to its appealing electronic band structure, high physicochemical stability and earth-abundant nature. In the present work, bulk g-C3N4 was synthesized by thermal decomposition of melamine. This material was further exfoliated by thermal treatment. S-doped samples were prepared from thiourea or further treatment of exfoliated g-C3N4 by mesylchloride. Synthesized materials were applied for photocatalytic removal of air pollutants (acetaldehyde and NOx) according to the ISO 22197 and ISO 22197-1 methodology. The efficiency of acetaldehyde removal under UV irradiation was negligible for all g-C3N4 samples. This can be explained by the fact that g-C3N4 under irradiation does not directly form hydroxyl radicals, which are the primary oxidation species in acetaldehyde oxidation. It was proved by electron paramagnetic resonance (EPR) spectroscopy that the dominant species formed on the irradiated surface of g-C3N4 was the superoxide radical. Its production was responsible for a very high NOx removal efficiency not only under UV irradiation (which was comparable with that of TiO2), but also under visible irradiation.


2019 ◽  
Vol 30 (5) ◽  
pp. 5109-5119 ◽  
Author(s):  
Xiaoyang Xu ◽  
Qianqian Liu ◽  
Ting Wei ◽  
Ying Zhao ◽  
Xiangjing Zhang

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