scholarly journals Tunable preparation of highly dispersed NixMn-LDO catalysts derived from NixMn-LDHs precursors and application in low-temperature NH3-SCR reactions

RSC Advances ◽  
2019 ◽  
Vol 9 (42) ◽  
pp. 24377-24385 ◽  
Author(s):  
Benhui Hou ◽  
Yali Du ◽  
Xuezhen Liu ◽  
Chao Ci ◽  
Xu Wu ◽  
...  
Keyword(s):  
Low Temperature ◽  
Uniform Distribution ◽  
Active Species ◽  
Nh3 Scr ◽  
Highly Dispersed

The NixMn-LDO catalysts derived from NixMn-LDHs precursors with uniform distribution of active species particles exhibited outstanding DeNOx performance.

Highly dispersed surface active species of Mn/Ce/TiW catalysts for high performance at low temperature NH3-SCR

2017 ◽  
Vol 330 ◽  
pp. 1195-1202 ◽  
Author(s):  
Hongfeng Chen ◽  
Yang Xia ◽  
Hui Huang ◽  
Yongping Gan ◽  
Xinyong Tao ◽  
...  
Keyword(s):  
Low Temperature ◽  
High Performance ◽  
Active Species ◽  
Nh3 Scr ◽  
Highly Dispersed ◽  
Surface Active

Enhancing catalytic activity and stability for CO2 methanation on Ni@MOF-5 via control of active species dispersion

2015 ◽  
Vol 51 (9) ◽  
pp. 1728-1731 ◽  
Author(s):  
Wenlong Zhen ◽  
Bo Li ◽  
Gongxuan Lu ◽  
Jiantai Ma
Keyword(s):  
Catalytic Activity ◽  
Low Temperature ◽  
High Stability ◽  
Active Catalyst ◽  
Active Species ◽  
Co2 Methanation ◽  
Long Term Stability ◽  
Uniform State ◽  
Highly Dispersed

A novel high active catalyst Ni@MOF-5 showed unexpected higher activity under the low temperature for CO2 methanation. The characterization results indicated that Ni was in highly dispersed uniform state over MOF-5. This catalyst performed high stability and showed almost no deactivation in long term stability tests up to 100 h.

scholarly journals Insight into the Promoting Role of Er Modification on SO2 Resistance for NH3-SCR at Low Temperature over FeMn/TiO2 Catalysts

Catalysts ◽  
2021 ◽  
Vol 11 (5) ◽  
pp. 618
Author(s):  
Huan Du ◽  
Zhitao Han ◽  
Xitian Wu ◽  
Chenglong Li ◽  
Yu Gao ◽  
...  
Keyword(s):  
Low Temperature ◽  
Catalyst Surface ◽  
Impregnation Method ◽  
In Situ Drifts ◽  
Tio2 Catalyst ◽  
Nh3 Scr ◽  
Nh3 Adsorption ◽  
So2 Resistance ◽  
Fast Scr

Er-modified FeMn/TiO2 catalysts were prepared through the wet impregnation method, and their NH3-SCR activities were tested. The results showed that Er modification could obviously promote SO2 resistance of FeMn/TiO2 catalysts at a low temperature. The promoting effect and mechanism were explored in detail using various techniques, such as BET, XRD, H2-TPR, XPS, TG, and in-situ DRIFTS. The characterization results indicated that Er modification on FeMn/TiO2 catalysts could increase the Mn4+ concentration and surface chemisorbed labile oxygen ratio, which was favorable for NO oxidation to NO2, further accelerating low-temperature SCR activity through the “fast SCR” reaction. As fast SCR reaction could accelerate the consumption of adsorbed NH3 species, it would benefit to restrain the competitive adsorption of SO2 and limit the reaction between adsorbed SO2 and NH3 species. XPS results indicated that ammonium sulfates and Mn sulfates formed were found on Er-modified FeMn/TiO2 catalyst surface seemed much less than those on FeMn/TiO2 catalyst surface, suggested that Er modification was helpful for reducing the generation or deposition of sulfate salts on the catalyst surface. According to in-situ DRIFTS the results of, the presence of SO2 in feeding gas imposed a stronger impact on the NO adsorption than NH3 adsorption on Lewis acid sites of Er-modified FeMn/TiO2 catalysts, gradually making NH3-SCR reaction to proceed in E–R mechanism rather than L–H mechanism. DRIFTS.

Lead poisoning and regeneration of Mn-Ce/TiO2 catalysts for NH3-SCR of NO at low temperature

2021 ◽  
Vol 49 (1) ◽  
pp. 113-120
Author(s):  
Dong-jie YAN ◽  
Tong GUO ◽  
Ya YU ◽  
Zhao-hui CHEN
Keyword(s):  
Low Temperature ◽  
Lead Poisoning ◽  
Nh3 Scr ◽  
Scr Of No

Improved NH3-SCR deNOx activity and tolerance to H2O & SO2 at low temperature over the NbmCu0.1-mCe0.9Ox catalysts: Role of acidity by niobium doping

Fuel ◽  
2021 ◽  
Vol 303 ◽  
pp. 121239
Author(s):  
Zhiping Zhang ◽  
Yingying Li ◽  
Piaoping Yang ◽  
Yushi Li ◽  
Chen Zhao ◽  
...  
Keyword(s):  
Low Temperature ◽  
Niobium Doping ◽  
Nh3 Scr

Nb2O5-modified Mn-Ce/AC catalyst with high ZnCl2 and SO2 tolerance for low-temperature NH3-SCR of NO

2021 ◽  
Vol 9 (5) ◽  
pp. 106323
Author(s):  
Yuhan Zhou ◽  
Buxin Su ◽  
Shan Ren ◽  
Zhichao Chen ◽  
Zenghui Su ◽  
...  
Keyword(s):  
Low Temperature ◽  
Nh3 Scr ◽  
Scr Of No ◽  
So2 Tolerance
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