Two-dimensional materials as catalysts for solar fuels: hydrogen evolution reaction and CO2 reduction

2019 ◽  
Vol 7 (2) ◽  
pp. 430-454 ◽  
Author(s):  
Amirhossein Hasani ◽  
Mahider Tekalgne ◽  
Quyet Van Le ◽  
Ho Won Jang ◽  
Soo Young Kim

The issues of global warming and fossil fuel shortage have increased the demand for clean and renewable energy.

Author(s):  
Jing Ji ◽  
Cunjin Zhang ◽  
Shuaibo Qin ◽  
Peng Jin

The oxygen evolution reaction (OER), oxygen reduction reaction (ORR), and hydrogen evolution reaction (HER) all have attracted much attention due to their utmost importance for clean and renewable energy applications....


Nanomaterials ◽  
2020 ◽  
Vol 10 (12) ◽  
pp. 2337
Author(s):  
Yanying Yu ◽  
Jie Xu ◽  
Jianwei Zhang ◽  
Fan Li ◽  
Jiantao Fu ◽  
...  

Transition-metal dichalcogenides (TMDs) materials have attracted much attention for hydrogen evolution reaction (HER) as a new catalyst, but they still have challenges in poor stability and high reaction over-potential. In this study, Ultra-thin SnS2 nanocatalysts were synthesized by simple hydrothermal method, and low load of Pt was added to form stable SnS2-Pt-3 (the content of platinum is 0.5 wt %). The synergistic effect between ultra-thin SnS2 rich in active sites and individual dispersed Pt nanoclusters can significantly reduce the reaction barrier and further accelerate HER reaction kinetics. Hence, SnS2-Pt-3 exhibits a low overpotential of 210 mV at the current density of 10 mA cm−2. It is worth noting that SnS2-Pt-3 has a small Tafel slope (126 mV dec−1) in 0.5 M H2SO4, as well as stability. This work provides a new option for the application of TMDs materials in efficient hydrogen evolution reaction. Moreover, this method can be easily extended to other catalysts with desired two-dimensional materials.


2018 ◽  
Vol 20 (29) ◽  
pp. 19390-19397 ◽  
Author(s):  
Xiaowei Yang ◽  
Nan Gao ◽  
Si Zhou ◽  
Jijun Zhao

MXenes, a new class of two-dimensional materials, arouse great interest due to their diverse chemistries, superior electrical conductivity and stability.


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