A green and facile method to prepare graphitic carbon nitride nanosheets with outstanding photocatalytic H2O2 production ability via NaClO hydrothermal treatment

2018 ◽  
Vol 42 (22) ◽  
pp. 18335-18341 ◽  
Author(s):  
Hui Wang ◽  
Lei Fang ◽  
Shaozheng Hu ◽  
Yanbo Pei ◽  
Wentao Ma
Keyword(s):  
Surface Area ◽  
Charge Separation ◽  
Carbon Nitride ◽  
Separation Efficiency ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
H2o2 Production ◽  
Photocatalytic Process ◽  
Charge Separation Efficiency ◽  
Carbon Nitride Nanosheets

Transportation and transformation of photogenerated carriers during the photocatalytic process of graphitic carbon nitride (g-C3N4) are restricted by the low surface area and insufficient charge separation efficiency.

scholarly journals Band Engineering and Morphology Control of Oxygen-Incorporated Graphitic Carbon Nitride Porous Nanosheets for Highly Efficient Photocatalytic Hydrogen Evolution

2021 ◽  
Vol 13 (1) ◽  
Author(s):  
Yunyan Wu ◽  
Pan Xiong ◽  
Jianchun Wu ◽  
Zengliang Huang ◽  
Jingwen Sun ◽  
...  
Keyword(s):  
Surface Area ◽  
Hydrogen Evolution ◽  
Carbon Nitride ◽  
Separation Efficiency ◽  
Physical Adsorption ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
Photocatalytic Hydrogen Evolution ◽  
Band Engineering ◽  
Highly Efficient

AbstractGraphitic carbon nitride (g-C3N4)-based photocatalysts have shown great potential in the splitting of water. However, the intrinsic drawbacks of g-C3N4, such as low surface area, poor diffusion, and charge separation efficiency, remain as the bottleneck to achieve highly efficient hydrogen evolution. Here, a hollow oxygen-incorporated g-C3N4 nanosheet (OCN) with an improved surface area of 148.5 m2 g−1 is fabricated by the multiple thermal treatments under the N2/O2 atmosphere, wherein the C–O bonds are formed through two ways of physical adsorption and doping. The physical characterization and theoretical calculation indicate that the O-adsorption can promote the generation of defects, leading to the formation of hollow morphology, while the O-doping results in reduced band gap of g-C3N4. The optimized OCN shows an excellent photocatalytic hydrogen evolution activity of 3519.6 μmol g−1 h−1 for ~ 20 h, which is over four times higher than that of g-C3N4 (850.1 μmol g−1 h−1) and outperforms most of the reported g-C3N4 catalysts.

Nanoporous photocatalysts developed through heat-driven stacking of graphitic carbon nitride nanosheets

RSC Advances ◽  
2015 ◽  
Vol 5 (18) ◽  
pp. 14027-14033 ◽  
Author(s):  
Zhijun Huang ◽  
Fengbo Li ◽  
Bingfeng Chen ◽  
Guoqing Yuan
Keyword(s):  
Heat Treatment ◽  
Optical Properties ◽  
Photocatalytic Activity ◽  
Surface Area ◽  
Carbon Nitride ◽  
High Surface ◽  
High Surface Area ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
Carbon Nitride Nanosheets

Nanostructured g-C3N4 with high surface area from heat treatment of guanidinium cyanurate exhibits better optical properties and enhanced photocatalytic activity.

Enhanced peroxidase-like activity of AuNPs loaded graphitic carbon nitride nanosheets for colorimetric biosensing

2019 ◽  
Vol 1091 ◽  
pp. 69-75 ◽  
Author(s):  
Na Wu ◽  
Yi-Ting Wang ◽  
Xiao-Yan Wang ◽  
Feng-Na Guo ◽  
Hui Wen ◽  
...  
Keyword(s):  
Carbon Nitride ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
Carbon Nitride Nanosheets ◽  
Colorimetric Biosensing

A simple tactic synthesis of hollow porous graphitic carbon nitride with significantly enriched photocatalytic performance

2021 ◽  
Author(s):  
Vellaichamy Balakumar ◽  
Manivannan Ramalingam ◽  
Chitiphon Chuaicham ◽  
KARTHIKEYAN SEKAR ◽  
K. Sasaki
Keyword(s):  
Crystal Structure ◽  
Surface Area ◽  
Carbon Nitride ◽  
Photocatalytic Performance ◽  
Porous Graphitic Carbon ◽  
Graphitic Carbon ◽  
Graphitic Carbon Nitride ◽  
Modified Surface

Hollow porous graphitic carbon nitride (porous CN) was synthesized via a simple tactic method, and the resulting porous CN showed an effectively modified surface area, crystal structure and enhanced photocatalytic...

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