Rational design of electrocatalysts and photo(electro)catalysts for nitrogen reduction to ammonia (NH3) under ambient conditions

2018 ◽  
Vol 11 (1) ◽  
pp. 45-56 ◽  
Author(s):  
Chunxian Guo ◽  
Jingrun Ran ◽  
Anthony Vasileff ◽  
Shi-Zhang Qiao
Keyword(s):  
Rational Design ◽  
Ambient Conditions ◽  
Nitrogen Reduction

This perspective highlights the rational design of efficient electrocatalysts and photo(electro)catalysts for N2 reduction to ammonia (NH3) under ambient conditions.

Rational Design of Fe–N/C Hybrid for Enhanced Nitrogen Reduction Electrocatalysis under Ambient Conditions in Aqueous Solution

ACS Catalysis ◽  
2018 ◽  
Vol 9 (1) ◽  
pp. 336-344 ◽  
Author(s):  
Ying Wang ◽  
Xiaoqiang Cui ◽  
Jingxiang Zhao ◽  
Guangri Jia ◽  
Lin Gu ◽  
...  
Keyword(s):  
Aqueous Solution ◽  
Rational Design ◽  
Ambient Conditions ◽  
Nitrogen Reduction

Rational design of boron contained co-doped graphene as high efficient electro-catalysts for nitrogen reduction reaction

2021 ◽  
Author(s):  
Wencheng Ouyang ◽  
Qiuming Zhi ◽  
LeLe Gong ◽  
Hao Sun ◽  
Minghui Liu ◽  
...  
Keyword(s):  
Nitrogen Fixation ◽  
Renewable Energy ◽  
Rational Design ◽  
Reduction Reaction ◽  
Ammonia Production ◽  
Ambient Conditions ◽  
Nitrogen Reduction ◽  
High Efficient ◽  
Doped Graphene ◽  
Co Doped

Electrocatalytic nitrogen reduction reaction (NRR) under ambient conditions has been proposed as a sustainable alternative for nitrogen fixation and ammonia production in environment and renewable energy fields. Carbon-based materials have...

Efficient photocatalytic nitrogen fixation under ambient conditions enabled by the heterojunctions of n-type Bi2MoO6 and oxygen-vacancy-rich p-type BiOBr

Nanoscale ◽  
2019 ◽  
Vol 11 (21) ◽  
pp. 10439-10445 ◽  
Author(s):  
Xiaolan Xue ◽  
Renpeng Chen ◽  
Changzeng Yan ◽  
Yi Hu ◽  
Wenjun Zhang ◽  
...  
Keyword(s):  
Nitrogen Fixation ◽  
Oxygen Vacancy ◽  
Ambient Conditions ◽  
Nitrogen Reduction ◽  
Photocatalytic Activities ◽  
P Type

Bi2MoO6/OV-BiOBr heterojunctions are synthesized and show good photocatalytic activities for nitrogen reduction to ammonia under ambient conditions.

p-Block Element-doped Silicon Nanowires for Nitrogen Reduction Reaction: A DFT Study

Nanoscale ◽  
2021 ◽  
Author(s):  
Zhongyuan Guo ◽  
Lakshitha Jasin Arachchige ◽  
Siyao Qiu ◽  
Xiao Li Zhang ◽  
Yongjun Xu ◽  
...  
Keyword(s):  
Silicon Nanowires ◽  
Reduction Reaction ◽  
Dft Study ◽  
Block Element ◽  
Ambient Conditions ◽  
Nitrogen Reduction ◽  
Green Route ◽  
Doped Silicon

Photocatalytic nitrogen reduction reaction (NRR) is a promising, green route to chemically reducing N2 into NH3 under ambient conditions, correlating to the N2 fixation process of nitrogenase enzymes. To achieve...

Sulfur vacancy-rich N-doped MoS2 nanoflowers for highly boosting electrocatalytic N2 fixation to NH3 under ambient conditions

2019 ◽  
Vol 55 (51) ◽  
pp. 7386-7389 ◽  
Author(s):  
Libin Zeng ◽  
Shuai Chen ◽  
Joshua van der Zalm ◽  
Xinyong Li ◽  
Aicheng Chen
Keyword(s):  
N2 Fixation ◽  
Ambient Conditions ◽  
Sulfur Vacancy ◽  
Nitrogen Reduction ◽  
Highly Effective ◽  
Electrochemical Catalysts

Sulfur vacancy-rich N-doped MoS2 nanoflowers act as highly effective electrochemical catalysts for efficient nitrogen reduction.

Highly efficient electrochemical ammonia synthesis via nitrogen reduction reactions on a VN nanowire array under ambient conditions

2018 ◽  
Vol 54 (42) ◽  
pp. 5323-5325 ◽  
Author(s):  
Xiaoping Zhang ◽  
Rong-Mei Kong ◽  
Huitong Du ◽  
Lian Xia ◽  
Fengli Qu
Keyword(s):  
High Performance ◽  
Ammonia Synthesis ◽  
Nanowire Array ◽  
Reduction Reaction ◽  
Carbon Cloth ◽  
Ambient Conditions ◽  
Faradaic Efficiency ◽  
Nitrogen Reduction ◽  
Highly Efficient ◽  
High Ammonia

A VN nanowire array on carbon cloth (VN/CC) as a high-performance catalyst for the nitrogen reduction reaction (NRR) affords high ammonia yield (2.48 × 10−10 mol−1 s−1 cm−2) and faradaic efficiency (3.58%) at −0.3 V versus RHE in 0.1 M HCl.

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