Surface chemistry and catalysis confined under two-dimensional materials

2017 ◽  
Vol 46 (7) ◽  
pp. 1842-1874 ◽  
Author(s):  
Qiang Fu ◽  
Xinhe Bao

Interfaces between 2D material overlayers and solid surfaces provide confined spaces for chemical processes, which have stimulated new chemistry under a 2D cover.

RSC Advances ◽  
2020 ◽  
Vol 10 (15) ◽  
pp. 8618-8627 ◽  
Author(s):  
Long Zhou ◽  
Guanglong Zhang ◽  
Fangyuan Xiu ◽  
Shuwei Xia ◽  
Liangmin Yu

The tesseract contained 2D material, C24Se12, is an effective molecular sieve with high selectivity to recover helium from natural gas under ambient conditions.


2019 ◽  
Vol 48 (21) ◽  
pp. 5310-5349 ◽  
Author(s):  
Liming Wang ◽  
Wenlong Chen ◽  
Doudou Zhang ◽  
Yaping Du ◽  
Rose Amal ◽  
...  

This work constructively reviewed and predicted the surface strategies for catalytic CO2 reduction with 2D material, nanocluster and single-atom catalysts


Nanoscale ◽  
2020 ◽  
Vol 12 (48) ◽  
pp. 24503-24509
Author(s):  
Eunpyo Park ◽  
Minkyung Kim ◽  
Tae Soo Kim ◽  
In Soo Kim ◽  
Jongkil Park ◽  
...  

A three-terminal top-gated flash device based on two-dimensional materials with a high coupling ratio exhibits highly linear synaptic weight updates.


Catalysts ◽  
2018 ◽  
Vol 8 (12) ◽  
pp. 590 ◽  
Author(s):  
Yu Ren ◽  
Yuze Dong ◽  
Yaqing Feng ◽  
Jialiang Xu

Energy shortage and environmental pollution problems boost in recent years. Photocatalytic technology is one of the most effective ways to produce clean energy—hydrogen and degrade pollutants under moderate conditions and thus attracts considerable attentions. TiO2 is considered one of the best photocatalysts because of its well-behaved photo-corrosion resistance and catalytic activity. However, the traditional TiO2 photocatalyst suffers from limitations of ineffective use of sunlight and rapid carrier recombination rate, which severely suppress its applications in photocatalysis. Surface modification and hybridization of TiO2 has been developed as an effective method to improve its photocatalysis activity. Due to superior physical and chemical properties such as high surface area, suitable bandgap, structural stability and high charge mobility, two-dimensional (2D) material is an ideal modifier composited with TiO2 to achieve enhanced photocatalysis process. In this review, we summarized the preparation methods of 2D material/TiO2 hybrid and drilled down into the role of 2D materials in photocatalysis activities.


2017 ◽  
Vol 7 (1) ◽  
Author(s):  
Zhengrong Guo ◽  
Tienchong Chang ◽  
Xingming Guo ◽  
Huajian Gao

2018 ◽  
Author(s):  
Penny Perlepe ◽  
Rodolphe Clérac ◽  
Itziar Oyarzabal ◽  
Corine Mathonière

Nanophotonics ◽  
2020 ◽  
Vol 9 (16) ◽  
pp. 4719-4728
Author(s):  
Tao Deng ◽  
Shasha Li ◽  
Yuning Li ◽  
Yang Zhang ◽  
Jingye Sun ◽  
...  

AbstractThe molybdenum disulfide (MoS2)-based photodetectors are facing two challenges: the insensitivity to polarized light and the low photoresponsivity. Herein, three-dimensional (3D) field-effect transistors (FETs) based on monolayer MoS2 were fabricated by applying a self–rolled-up technique. The unique microtubular structure makes 3D MoS2 FETs become polarization sensitive. Moreover, the microtubular structure not only offers a natural resonant microcavity to enhance the optical field inside but also increases the light-MoS2 interaction area, resulting in a higher photoresponsivity. Photoresponsivities as high as 23.8 and 2.9 A/W at 395 and 660 nm, respectively, and a comparable polarization ratio of 1.64 were obtained. The fabrication technique of the 3D MoS2 FET could be transferred to other two-dimensional materials, which is very promising for high-performance polarization-sensitive optical and optoelectronic applications.


RSC Advances ◽  
2021 ◽  
Vol 11 (15) ◽  
pp. 8654-8663
Author(s):  
Fatima Zahra Ramadan ◽  
Flaviano José dos Santos ◽  
Lalla Btissam Drissi ◽  
Samir Lounis

Based on density functional theory combined with low-energy models, we explore the magnetic properties of a hybrid atomic-thick two-dimensional (2D) material made of germanene doped with fluorine atoms in a half-fluorinated configuration (Ge2F).


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