Toward high thermoelectric performance p-type FeSb2.2Te0.8via in situ formation of InSb nanoinclusions

2015 ◽  
Vol 3 (32) ◽  
pp. 8372-8380 ◽  
Author(s):  
Gangjian Tan ◽  
Hang Chi ◽  
Wei Liu ◽  
Yun Zheng ◽  
Xinfeng Tang ◽  
...  

The InSb nanoinclusions formed in situ at the grain boundaries of FeSb2.2Te0.8 mitigates the mobility degradation while the added grain boundaries effectively scatter heat-carrying phonons. This novel “electron-channel phonon-barrier” nanocompositing approach opens a new route to design high performance thermoelectric materials.

2017 ◽  
Vol 29 (8) ◽  
pp. 3572-3579 ◽  
Author(s):  
Haiping Wu ◽  
Yue Cao ◽  
Linxiao Geng ◽  
Chao Wang

Nano Letters ◽  
2014 ◽  
Vol 14 (2) ◽  
pp. 716-723 ◽  
Author(s):  
Tadhg Kennedy ◽  
Emma Mullane ◽  
Hugh Geaney ◽  
Michal Osiak ◽  
Colm O’Dwyer ◽  
...  

2021 ◽  
Author(s):  
Qi Zhang ◽  
Hengda Sun ◽  
Meifang Zhu

Abstract Organic thermoelectric (OTE) materials have been regarded as a potential candidate to harvest waste heat from complex, low temperature surfaces of objects and convert it into electricity. Recently, n-type conjugated polymers as organic thermoelectric materials have aroused intensive research in order to improve their performance to match up with their p-type counterpart. In this review, we discuss aspects that affect the performance of n-type OTEs, and further focus on the effect of planarity of backbone on doping efficiency and eventually the TE performance. We then summarize strategies such as implementing rigid n-type polymer backbone or modifying conventional polymer building blocks for more planar conformation. In the outlook part, we conclude forementioned devotions and point out new possibility that may promote the future development of this field.


2018 ◽  
Vol 6 (41) ◽  
pp. 20454-20462 ◽  
Author(s):  
Juan Li ◽  
Shuai Zhang ◽  
Boyi Wang ◽  
Shichao Liu ◽  
Luo Yue ◽  
...  

Thermoelectric performance can be largely enhanced by forming solid solutions and biaxial strain.


2018 ◽  
Vol 6 (45) ◽  
pp. 22381-22390 ◽  
Author(s):  
Yufeng Xue ◽  
Chunmei Gao ◽  
Lirong Liang ◽  
Xin Wang ◽  
Guangming Chen

This review discusses recent advances in controlled fabrication of nanostructures and the enhanced thermoelectric performance of polymers and their composites.


Nano Energy ◽  
2016 ◽  
Vol 27 ◽  
pp. 282-297 ◽  
Author(s):  
Sajid Ahmad ◽  
Ajay Singh ◽  
Anil Bohra ◽  
Ranita Basu ◽  
Shovit Bhattacharya ◽  
...  

Science ◽  
2019 ◽  
Vol 365 (6460) ◽  
pp. 1418-1424 ◽  
Author(s):  
Wenke He ◽  
Dongyang Wang ◽  
Haijun Wu ◽  
Yu Xiao ◽  
Yang Zhang ◽  
...  

Thermoelectric technology allows conversion between heat and electricity. Many good thermoelectric materials contain rare or toxic elements, so developing low-cost and high-performance thermoelectric materials is warranted. Here, we report the temperature-dependent interplay of three separate electronic bands in hole-doped tin sulfide (SnS) crystals. This behavior leads to synergistic optimization between effective mass (m*) and carrier mobility (μ) and can be boosted through introducing selenium (Se). This enhanced the power factor from ~30 to ~53 microwatts per centimeter per square kelvin (μW cm−1 K−2 at 300 K), while lowering the thermal conductivity after Se alloying. As a result, we obtained a maximum figure of merit ZT (ZTmax) of ~1.6 at 873 K and an average ZT (ZTave) of ~1.25 at 300 to 873 K in SnS0.91Se0.09 crystals. Our strategy for band manipulation offers a different route for optimizing thermoelectric performance. The high-performance SnS crystals represent an important step toward low-cost, Earth-abundant, and environmentally friendly thermoelectrics.


2020 ◽  
Vol 8 (24) ◽  
pp. 12156-12168
Author(s):  
Decheng An ◽  
Shaoping Chen ◽  
Xin Zhai ◽  
Yuan Yu ◽  
Wenhao Fan ◽  
...  

An outstanding figure-of-merit zT ≈ 1.06 at 600 K for p-type elemental Te thermoelectrics is realized by synergistically tuning their carrier and phonon transport behaviors via a multicomponent alloying strategy.


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