scholarly journals A classical treatment of optical tunneling in plasmonic gaps: extending the quantum corrected model to practical situations

2015 ◽  
Vol 178 ◽  
pp. 151-183 ◽  
Author(s):  
Rubén Esteban ◽  
Asier Zugarramurdi ◽  
Pu Zhang ◽  
Peter Nordlander ◽  
Francisco J. García-Vidal ◽  
...  

The optical response of plasmonic nanogaps is challenging to address when the separation between the two nanoparticles forming the gap is reduced to a few nanometers or even subnanometer distances. We have compared results of the plasmon response within different levels of approximation, and identified a classical local regime, a nonlocal regime and a quantum regime of interaction. For separations of a few Ångstroms, in the quantum regime, optical tunneling can occur, strongly modifying the optics of the nanogap. We have considered a classical effective model, so called Quantum Corrected Model (QCM), that has been introduced to correctly describe the main features of optical transport in plasmonic nanogaps. The basics of this model are explained in detail, and its implementation is extended to include nonlocal effects and address practical situations involving different materials and temperatures of operation.

2010 ◽  
Author(s):  
Christin David ◽  
F. Javier García de Abajo ◽  
Dmitry N. Chigrin

1995 ◽  
Vol 122 (1-3) ◽  
pp. 9-15 ◽  
Author(s):  
S. Wang ◽  
J. Siqueiros ◽  
R. Machorro

2005 ◽  
Vol 133 (5) ◽  
pp. 315-320 ◽  
Author(s):  
Railing Chang ◽  
H.-P. Chiang ◽  
P.T. Leung ◽  
D.P. Tsai ◽  
W.S. Tse

Photonics ◽  
2019 ◽  
Vol 6 (2) ◽  
pp. 39 ◽  
Author(s):  
Muhammad Khalid ◽  
Cristian Ciracì

Nonlocal and quantum effects play an important role in accurately modeling the optical response of nanometer-sized metallic nanoparticles. These effects cannot be described by conventional classical theories, as they neglect essential microscopic details. Quantum hydrodynamic theory (QHT) has emerged as an excellent tool to correctly predict the nonlocal and quantum effects by taking into account the spatial dependence of the charge density. In this article, we used a QHT to investigate the impact of nonlocality and electron spill-out on the plasmonic behavior of spherical Na and Au nanoshells. We adopted a self-consistent way to compute the equilibrium charge density. The results predicted by QHT were compared with those obtained with the local response approximation (LRA) and the Thomas–Fermi hydrodynamic theory (TFHT). We found that nonlocal effects have a strong impact on both the near- and far-field optical properties of nanoshells, in particular, for the antibonding resonant mode. We also investigated the optical response of these systems for different thicknesses of the shell, both for Na and Au metals.


Author(s):  
J. E. Doherty ◽  
A. F. Giamei ◽  
B. H. Kear ◽  
C. W. Steinke

Recently we have been investigating a class of nickel-base superalloys which possess substantial room temperature ductility. This improvement in ductility is directly related to improvements in grain boundary strength due to increased boundary cohesion through control of detrimental impurities and improved boundary shear strength by controlled grain boundary micros true tures.For these investigations an experimental nickel-base superalloy was doped with different levels of sulphur impurity. The micros tructure after a heat treatment of 1360°C for 2 hr, 1200°C for 16 hr consists of coherent precipitates of γ’ Ni3(Al,X) in a nickel solid solution matrix.


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