Monitoring of atmospheric nitrogen dioxide by long-path pulsed differential optical absorption spectroscopy using two different light paths

2012 ◽  
Vol 14 (3) ◽  
pp. 944 ◽  
Author(s):  
Yasuaki Kambe ◽  
Yotsumi Yoshii ◽  
Kenshi Takahashi ◽  
Kenichi Tonokura
Keyword(s):  
Optical Absorption ◽  
Nitrogen Dioxide ◽  
Absorption Spectroscopy ◽  
Differential Optical Absorption Spectroscopy ◽  
Optical Absorption Spectroscopy ◽  
Atmospheric Nitrogen

scholarly journals Spatially resolved measurements of nitrogen dioxide in an urban environment using concurrent multi-axis differential optical absorption spectroscopy

2006 ◽  
Vol 6 (6) ◽  
pp. 12671-12700
Author(s):  
R. J. Leigh ◽  
G. K. Corlett ◽  
U. Frieß ◽  
P. S. Monks
Keyword(s):  
Remote Sensing ◽  
Optical Absorption ◽  
Nitrogen Dioxide ◽  
Urban Environment ◽  
Absorption Spectroscopy ◽  
Differential Optical Absorption Spectroscopy ◽  
Optical Absorption Spectroscopy ◽  
High Time Resolution ◽  
In Situ Techniques

Abstract. A novel system using the technique of concurrent multi-axis differential optical absorption spectroscopy system has been developed and applied to the measurement of nitrogen dioxide in an urban environment. Using five fixed telescopes, slant columns of nitrogen dioxide, ozone, water vapour, and the oxygen dimer, O4, are simultaneously retrieved in five vertically separated viewing directions. The application of this remote sensing technique in the urban environment is explored. Through, the application of several simplifying assumptions a tropospheric concentration of NO2 is derived and compared with an urban background in-situ chemiluminescence detector. The remote sensing and in-situ techniques show good agreement. Owing to the high time resolution of the measurements, the ability to image and quantify plumes within the urban environment is demonstrated. The CMAX-DOAS measurements provide a useful measure of overall NO2 concentrations on a city-wide scale.

scholarly journals Spatially resolved measurements of nitrogen dioxide in an urban environment using concurrent multi-axis differential optical absorption spectroscopy

2007 ◽  
Vol 7 (18) ◽  
pp. 4751-4762 ◽  
Author(s):  
R. J. Leigh ◽  
G. K. Corlett ◽  
U. Frieß ◽  
P. S. Monks
Keyword(s):  
Remote Sensing ◽  
Optical Absorption ◽  
Nitrogen Dioxide ◽  
Urban Environment ◽  
Absorption Spectroscopy ◽  
Differential Optical Absorption Spectroscopy ◽  
Optical Absorption Spectroscopy ◽  
High Time Resolution ◽  
In Situ Techniques

Abstract. A novel system using the technique of concurrent multi-axis differential optical absorption spectroscopy system has been developed and applied to the measurement of nitrogen dioxide in an urban environment. Using five fixed telescopes, slant columns of nitrogen dioxide, ozone, water vapour, and the oxygen dimer, O4, are simultaneously retrieved in five vertically separated viewing directions. The application of this remote sensing technique in the urban environment is explored. Through the application of several simplifying assumptions a tropospheric concentration of NO2 is derived and compared with an urban background in-situ chemiluminescence detector. Trends derived from remote sensing and in-situ techniques show agreement to within 15 to 40% depending on conditions. Owing to the high time resolution of the measurements, the ability to image and quantify plumes within the urban environment is demonstrated. The CMAX-DOAS measurements provide a useful measure of overall NO2 concentrations on a city-wide scale.

scholarly journals Total Ozone Columns from the Environmental Trace Gases Monitoring Instrument (EMI) Using the DOAS Method

2021 ◽  
Vol 13 (11) ◽  
pp. 2098
Author(s):  
Yuanyuan Qian ◽  
Yuhan Luo ◽  
Fuqi Si ◽  
Haijin Zhou ◽  
Taiping Yang ◽  
...  
Keyword(s):  
Optical Absorption ◽  
Absorption Spectroscopy ◽  
Total Ozone ◽  
Scattered Light ◽  
Trace Gases ◽  
Rapid Change ◽  
Differential Optical Absorption Spectroscopy ◽  
Optical Absorption Spectroscopy ◽  
Monitoring Instrument ◽  
Monthly Average

Global measurements of total ozone are necessary to evaluate ozone hole recovery above Antarctica. The Environmental Trace Gases Monitoring Instrument (EMI) onboard GaoFen 5, launched in May 2018, was developed to measure and monitor the global total ozone column (TOC) and distributions of other trace gases. In this study, some of the first global TOC results of the EMI using the differential optical absorption spectroscopy (DOAS) method and validation with ground-based TOC measurements and data derived from Ozone Monitoring Instrument (OMI) and TROPOspheric Monitoring Instrument (TROPOMI) observations are presented. Results show that monthly average EMI TOC data had a similar spatial distribution and a high correlation coefficient (R ≥ 0.99) with both OMI and TROPOMI TOC. Comparisons with ground-based measurements from the World Ozone and Ultraviolet Radiation Data Centre also revealed strong correlations (R > 0.9). Continuous zenith sky measurements from zenith scattered light differential optical absorption spectroscopy instruments in Antarctica were also used for validation (R = 0.9). The EMI-derived observations were able to account for the rapid change in TOC associated with the sudden stratospheric warming event in October 2019; monthly average TOC in October 2019 was 45% higher compared to October 2018. These results indicate that EMI TOC derived using the DOAS method is reliable and has the potential to be used for global TOC monitoring.

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