Phonon dynamics and electron–phonon coupling in pristine picene

2012 ◽  
Vol 14 (5) ◽  
pp. 1694-1699 ◽  
Author(s):  
Alberto Girlando ◽  
Matteo Masino ◽  
Ivano Bilotti ◽  
Aldo Brillante ◽  
Raffaele G. Della Valle ◽  
...  
2018 ◽  
Vol 20 (3) ◽  
pp. 1642-1652 ◽  
Author(s):  
André Anda ◽  
Darius Abramavičius ◽  
Thorsten Hansen

Two-dimensional electronic spectroscopy (2DES) is a powerful tool in the study of coupled electron–phonon dynamics, yet very little is known about how nonlinearities in the electron–phonon coupling, arising from anharmonicities in the nuclear potentials, affect the spectra.


2020 ◽  
Vol 124 (7) ◽  
Author(s):  
Dino Novko ◽  
Fabio Caruso ◽  
Claudia Draxl ◽  
Emmanuele Cappelluti

2019 ◽  
Vol 205 ◽  
pp. 08013
Author(s):  
Mark J. Stern ◽  
Laurent P. René de Cotret ◽  
Martin R. Otto ◽  
Robert P. Chatelain ◽  
Jean-Philippe Boisvert ◽  
...  

We show that ultrafast electron diffuse (inelastic) scattering provides a detailed, momentum-resolved view of electron-phonon and phonon-phonon coupling across the entire Brillouin zone. Ultrafast time-resolution and scattering selection rules can distinguish between phonon branches without energy-resolution.


2009 ◽  
Vol 102 (12) ◽  
Author(s):  
Larry Lüer ◽  
Christoph Gadermaier ◽  
Jared Crochet ◽  
Tobias Hertel ◽  
Daniele Brida ◽  
...  

2018 ◽  
Vol 20 (16) ◽  
pp. 10677-10685 ◽  
Author(s):  
Mirko Scholz ◽  
Kawon Oum ◽  
Thomas Lenzer

Long-lived coherent oscillations in transient absorption signals of BiI3 suggest strong electron–phonon coupling in this material for photovoltaics.


2018 ◽  
Vol 97 (16) ◽  
Author(s):  
Mark J. Stern ◽  
Laurent P. René de Cotret ◽  
Martin R. Otto ◽  
Robert P. Chatelain ◽  
Jean-Philippe Boisvert ◽  
...  

2021 ◽  
Vol 12 (6) ◽  
pp. 1690-1695
Author(s):  
Zhongyu Liu ◽  
Yingwei Li ◽  
Wonyong Shin ◽  
Rongchao Jin

2021 ◽  
Vol 103 (2) ◽  
Author(s):  
I.Yu. Sklyadneva ◽  
R. Heid ◽  
P. M. Echenique ◽  
E. V. Chulkov

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Rui Su ◽  
Zhaojian Xu ◽  
Jiang Wu ◽  
Deying Luo ◽  
Qin Hu ◽  
...  

AbstractThe performance of perovskite photovoltaics is fundamentally impeded by the presence of undesirable defects that contribute to non-radiative losses within the devices. Although mitigating these losses has been extensively reported by numerous passivation strategies, a detailed understanding of loss origins within the devices remains elusive. Here, we demonstrate that the defect capturing probability estimated by the capture cross-section is decreased by varying the dielectric response, producing the dielectric screening effect in the perovskite. The resulting perovskites also show reduced surface recombination and a weaker electron-phonon coupling. All of these boost the power conversion efficiency to 22.3% for an inverted perovskite photovoltaic device with a high open-circuit voltage of 1.25 V and a low voltage deficit of 0.37 V (a bandgap ~1.62 eV). Our results provide not only an in-depth understanding of the carrier capture processes in perovskites, but also a promising pathway for realizing highly efficient devices via dielectric regulation.


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