Atomistic mechanism of charge separation upon photoexcitation at the dye–semiconductor interface for photovoltaic applications

2011 ◽  
Vol 13 (29) ◽  
pp. 13196 ◽  
Author(s):  
Yang Jiao ◽  
Zijing Ding ◽  
Sheng Meng
2012 ◽  
Vol 51 (37) ◽  
pp. 11841-11849 ◽  
Author(s):  
He He ◽  
Chao Liu ◽  
Kevin D. Dubois ◽  
Tong Jin ◽  
Michael E. Louis ◽  
...  

Author(s):  
Qirong Yang ◽  
Jianxin Guan ◽  
Jingwen Deng ◽  
Zihan Xu ◽  
Zhihao Yu ◽  
...  

2021 ◽  
Author(s):  
Seiichiro Izawa ◽  
Masahiro Hiramoto

We realized solid-state UC with 100 times higher efficiency than a conventional system by discovering a novel UC mechanism in bilayer organic semiconductor heterojunctions. The UC occurred through spin inversion during the charge separation and recombination at the interface. The key to the success was the triplet formation at the interface, as this could avoid the loss process during triplet diffusion, which is a problematic issue in conventional systems. As a result of this finding, efficient UC from near-infrared to visible light on flexible thin films under LED light excitation was made possible.


2008 ◽  
Vol 101 (19) ◽  
Author(s):  
Matthias Muntwiler ◽  
Qingxin Yang ◽  
William A. Tisdale ◽  
X.-Y. Zhu

Nanomaterials ◽  
2019 ◽  
Vol 9 (3) ◽  
pp. 359 ◽  
Author(s):  
Yong-sheng Fu ◽  
Jun Li ◽  
Jianguo Li

Due to the capability of utilizing light energy to drive chemical reactions, photocatalysis has been widely accepted as a green technology to help us address the increasingly severe environment and energy issues facing human society. To date, a large amount of research has been devoted to enhancing the properties of photocatalysts. As reported, coupling semiconductors with metals is one of the most effective methods to achieve high-performance photocatalysts. The excellent properties of metal/semiconductor (M/S) nanocomposite photocatalysts originate in two aspects: (i) improved charge separation at the metal-semiconductor interface; and (ii) increased absorption of visible light due to the surface plasmon resonance of metals. So far, many M/S nanocomposite photocatalysts with different structures have been developed for the application in environmental remediation, selective organic transformation, hydrogen evolution, and disinfection. Herein, we will give a review on the M/S nanocomposite photocatalysts, regarding their fundamentals, structures (as well as their typical synthetic approaches), applications and properties. Finally, we will also present our perspective on the future development of M/S nanocomposite photocatalysts.


RSC Advances ◽  
2015 ◽  
Vol 5 (15) ◽  
pp. 11084-11090 ◽  
Author(s):  
Ke Cheng ◽  
Xiao Han ◽  
Jian Meng ◽  
Shujie Wang ◽  
Zuliang Du

The mechanism for enhanced charge separation was discussed and the charge transport model was established.


2021 ◽  
Author(s):  
Seiichiro Izawa ◽  
Masahiro Hiramoto

We realized solid-state UC with 100 times higher efficiency than a conventional system by discovering a novel UC mechanism in bilayer organic semiconductor heterojunctions. The UC occurred through spin inversion during the charge separation and recombination at the interface. The key to the success was the triplet formation at the interface, as this could avoid the loss process during triplet diffusion, which is a problematic issue in conventional systems. As a result of this finding, efficient UC from near-infrared to visible light on flexible thin films under LED light excitation was made possible.


2011 ◽  
Vol 133 (50) ◽  
pp. 20468-20475 ◽  
Author(s):  
Bridget Carsten ◽  
Jodi M. Szarko ◽  
Hae Jung Son ◽  
Wei Wang ◽  
Luyao Lu ◽  
...  

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