scholarly journals Angular distributions and angular momentum alignment of O(3PJ) atoms formed in the photolysis of O2via the Herzberg continuum

2010 ◽  
Vol 12 (48) ◽  
pp. 15715 ◽  
Author(s):  
Dmitri Chestakov ◽  
Wim J. van der Zande ◽  
David H. Parker ◽  
Claire Vallance
Keyword(s):  
Angular Momentum ◽  
Angular Distributions ◽  
Herzberg Continuum

QUASICLASSICAL TRAJECTORY STUDY OF PRODUCT POLARIZATIONS IN THE H(2S) + NH → N(4S) + H2 REACTION

2012 ◽  
Vol 11 (06) ◽  
pp. 1297-1310 ◽  
Author(s):  
LIN LI ◽  
SHUNLE DONG
Keyword(s):  
Angular Momentum ◽  
Cross Sections ◽  
Differential Cross ◽  
Ground State ◽  
Calculation Method ◽  
Collision Energy ◽  
Potential Surface ◽  
Angular Distributions ◽  
Title Reaction ◽  
Energy Dependent

Based on the DMBE potential surface of the 4 A ″ ground-state, the product rotational polarizations in the title reaction are studied by using quasiclassical trajectory (QCT) calculation method. Three angular distributions of P(θr), P(Φr), P(θr, Φr) and the four polarization-dependent differential cross sections (PDDCSs) were calculated for the collision energy range of 1–20 kcal/mol. The results revealed that the product is backward-scattering and the product rotational angular momentum j′ is aligned and oriented. With the increment of collision energy, the degree of the product alignment and orientation is enhanced, showing the collision energy-dependent behaviors of the product polarizations.

QUASICLASSICAL TRAJECTORY STUDY OF STEREODYNAMICS FOR THE REACTIONS Li+HF/DF/TF

2013 ◽  
Vol 12 (03) ◽  
pp. 1350008
Author(s):  
JIE CHENG ◽  
XIAN-FANG YUE
Keyword(s):  
Angular Momentum ◽  
Cross Sections ◽  
Collision Energy ◽  
Energy Surface ◽  
Center Of Mass ◽  
Angular Distributions ◽  
Direct Reaction ◽  
Generalized Polarization ◽  
State 1 ◽  
Rotational Angular Momentum

Stereodynamics of the reaction Li + HF (v = 0,j = 0) → LiF + H and its isotopic variants on the ground electronic state (12A′) potential energy surface (PES) are studied by employing the quasiclassical trajectory (QCT) method. At a collision energy of 2.2 kcal/mol, product rotational angular momentum distributions, P(θr) and P(ϕr), are calculated in the center-of-mass (CM) frame. The results demonstrate that the product rotational angular momentum j′ is not only aligned along the direction perpendicular to the reagent relative velocity vector k, but also oriented along the negative y-axis. The four generalized polarization-dependent differential cross sections (PDDCSs) are also computed. The PDDCS00 distribution shows a sideways scattering for the reaction Li + HF and a strongly backward scattering for the reaction Li + DF . However, it displays both the forward and backward scatterings for the reaction Li + TF . These features demonstrate that the Li + HF and Li + DF reactions proceed predominantly through the direct reaction mechanism. However, the Li + TF reaction undergoes both the direct and indirect reaction mechanisms. The PDDCS21- distribution indicates that the product angular distributions are anisotropic.

DYNAMIC APPROACH TO ANALYSIS OF ANGULAR DISTRIBUTIONS OF FISSION AND QUASIFISSION FRAGMENTS

2010 ◽  
Vol 19 (05n06) ◽  
pp. 1125-1133 ◽  
Author(s):  
V. A. DROZDOV ◽  
D. O. EREMENKO ◽  
O. V. FOTINA ◽  
S. Yu. PLATONOV ◽  
O. A. YUMINOV ◽  
...  
Keyword(s):  
Relaxation Time ◽  
Angular Momentum ◽  
Dynamic Model ◽  
Angular Distributions ◽  
Dynamic Approach ◽  
Dinuclear System ◽  
New Model ◽  
Angular Correlations

The dynamic model is proposed for description of the angular distributions of quasifission fragments. The model is able to describe experimental anisotropy of the angular distributions of fissionlike fragments for the 32 S , 28 Si +208 Pb reactions. It is also shown that the new model allows the description of the experimental mass-angular correlations in the quasifission fragment yields for the 64 Ni +197 Au reaction at 383 and 418 MeV of incident energies. The analysis was performed with the angular momentum and deformation dependent relaxation time of the tilting mode. Information on the dinuclear system lifetimes were obtained.

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